Tailoring Coordination Microenvironment of Cu(I) in Metal–Organic Frameworks for Enhancing Electroreduction of CO2 to CH4

The coordination microenvironment of metal active sites in metal–organic frameworks (MOFs) plays a crucial role in its performance for electrochemical CO2 reduction reaction (CO2RR). However, it remains a challenge to clarify the structure–performance relationship for CO2RR catalyzed by MOFs. Herein...

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Veröffentlicht in:	Advanced functional materials 2022-09, Vol.32 (36), p.n/a
Hauptverfasser:	Zhang, Ya, Zhou, Qiang, Qiu, Zhao‐Feng, Zhang, Xiao‐Yu, Chen, Jia‐Qi, Zhao, Yue, Gong, Feng, Sun, Wei‐Yin
Format:	Artikel
Sprache:	eng
Schlagworte:	Carbon dioxide Chemical reduction CO 2 electroreduction Coordination coordination microenvironments Copper Cu sites density functional theory Electrowinning Free energy Heat of formation Materials science Metal-organic frameworks Methane Selectivity
Online-Zugang:	Volltext
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