Effects of defect on thermal stability and photoluminescence in quenched Ho‐doped 0.94Na0.5Bi0.5TiO3–0.06BaTiO3 lead‐free ceramics

Solid solution 0.94Na 0.5 Bi 0.5 TiO 3 –6BaTiO 3 (NBT–6BT) is considered to be one kind of lead‐free piezoelectric materials with excellent electrical properties due to the existence of morphotropic phase boundary (MPB). However, its relatively lower depolarization temperature is a long‐standing bot...

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Veröffentlicht in:Journal of materials research 2021-03, Vol.36 (5), p.1125-1133
Hauptverfasser: Zheng, Lai‐Qi, Chen, Chao, Jiang, Xiang‐Ping, Jiang, Xing‐An, Huang, Xiao‐Kun, Nie, Xin, Liu, Jun‐Ming
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container_issue 5
container_start_page 1125
container_title Journal of materials research
container_volume 36
creator Zheng, Lai‐Qi
Chen, Chao
Jiang, Xiang‐Ping
Jiang, Xing‐An
Huang, Xiao‐Kun
Nie, Xin
Liu, Jun‐Ming
description Solid solution 0.94Na 0.5 Bi 0.5 TiO 3 –6BaTiO 3 (NBT–6BT) is considered to be one kind of lead‐free piezoelectric materials with excellent electrical properties due to the existence of morphotropic phase boundary (MPB). However, its relatively lower depolarization temperature is a long‐standing bottleneck for the application of NBT‐based piezoelectric ceramics. In this work, the influence of thermal quenching on depolarization temperature and electrical properties of rare‐earth Ho‐doped NBT–6BT lead‐free ceramics was investigated. It was shown that the relative high piezoelectric performance, as well as an improvement of depolarization temperature ( T d ), can be realized by thermal quenching. The results showed that the quenching process induced high concentration of oxygen vacancy, giving rise to the change of octahedra mode and enhanced lattice distortion, which is benefit to the temperature stability of piezoelectric and ferroelectric properties. Furthermore, up‐conversion photoluminescence (PL) of Ho‐doped NBT–6BT could be effectively tuned by the introduction of oxygen vacancy, suggesting a promising potential in optical–electrical multifunctional devices.
doi_str_mv 10.1557/s43578-020-00076-3
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subjects Applied and Technical Physics
Biomaterials
Chemistry and Materials Science
Depolarization
Electrical properties
Ferroelectricity
Inorganic Chemistry
Invited Paper
Lattice vacancies
Materials Engineering
Materials research
Materials Science
Nanotechnology
Oxygen
Photoluminescence
Piezoelectric ceramics
Quenching
Solid solutions
Thermal stability
title Effects of defect on thermal stability and photoluminescence in quenched Ho‐doped 0.94Na0.5Bi0.5TiO3–0.06BaTiO3 lead‐free ceramics
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