Oxidation of Spent Nuclear Fuel from Flawed RBMK-1000 Fuel Rods under Dry Storage Conditions
The effect of a humid nitrogen atmosphere with an oxygen content of 0.08, 0.48, 1.30 vol % and a temperature of 300°С on the change in the structure of the RBMK-1000 fuel composition vs. the size of the defect in the fuel cladding was investigated. It was demonstrated that in the case of fuel claddi...
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| Veröffentlicht in: | Radiochemistry (New York, N.Y.) N.Y.), 2022-06, Vol.64 (3), p.284-293 |
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| container_title | Radiochemistry (New York, N.Y.) |
| container_volume | 64 |
| creator | Beznosyuk, V. I. Krinitsyn, A. P. Mishin, K. Ya Metalidi, M. M. Nikandrova, M. V. |
| description | The effect of a humid nitrogen atmosphere with an oxygen content of 0.08, 0.48, 1.30 vol % and a temperature of 300°С on the change in the structure of the RBMK-1000 fuel composition vs. the size of the defect in the fuel cladding was investigated. It was demonstrated that in the case of fuel cladding damage with an area of more than 0.8 mm
2
, SNF storage in a nitrogen atmosphere with an oxygen content of more than 0.5 vol % at a temperature of 300°C brings about a rather rapid oxidation of the fuel composition to U
3
O
8
. Thus, dry storage of SNF should be carried out without access to oxygen. |
| doi_str_mv | 10.1134/S1066362222030043 |
| format | Article |
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2
, SNF storage in a nitrogen atmosphere with an oxygen content of more than 0.5 vol % at a temperature of 300°C brings about a rather rapid oxidation of the fuel composition to U
3
O
8
. Thus, dry storage of SNF should be carried out without access to oxygen.</description><identifier>ISSN: 1066-3622</identifier><identifier>EISSN: 1608-3288</identifier><identifier>DOI: 10.1134/S1066362222030043</identifier><language>eng</language><publisher>Moscow: Pleiades Publishing</publisher><subject>Chemistry ; Chemistry and Materials Science ; Chemistry/Food Science ; Composition ; Nitrogen ; Nuclear Chemistry ; Nuclear fuel elements ; Oxidation ; Oxygen ; Oxygen content ; RBMK ; Spent nuclear fuels</subject><ispartof>Radiochemistry (New York, N.Y.), 2022-06, Vol.64 (3), p.284-293</ispartof><rights>Pleiades Publishing, Ltd. 2022</rights><rights>Pleiades Publishing, Ltd. 2022.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c198t-6a048f4dd04676bba75e9627e16771cad25a4b73d6533450b132d32a09b09a213</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1134/S1066362222030043$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1134/S1066362222030043$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,781,785,27929,27930,41493,42562,51324</link.rule.ids></links><search><creatorcontrib>Beznosyuk, V. I.</creatorcontrib><creatorcontrib>Krinitsyn, A. P.</creatorcontrib><creatorcontrib>Mishin, K. Ya</creatorcontrib><creatorcontrib>Metalidi, M. M.</creatorcontrib><creatorcontrib>Nikandrova, M. V.</creatorcontrib><title>Oxidation of Spent Nuclear Fuel from Flawed RBMK-1000 Fuel Rods under Dry Storage Conditions</title><title>Radiochemistry (New York, N.Y.)</title><addtitle>Radiochemistry</addtitle><description>The effect of a humid nitrogen atmosphere with an oxygen content of 0.08, 0.48, 1.30 vol % and a temperature of 300°С on the change in the structure of the RBMK-1000 fuel composition vs. the size of the defect in the fuel cladding was investigated. It was demonstrated that in the case of fuel cladding damage with an area of more than 0.8 mm
2
, SNF storage in a nitrogen atmosphere with an oxygen content of more than 0.5 vol % at a temperature of 300°C brings about a rather rapid oxidation of the fuel composition to U
3
O
8
. Thus, dry storage of SNF should be carried out without access to oxygen.</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chemistry/Food Science</subject><subject>Composition</subject><subject>Nitrogen</subject><subject>Nuclear Chemistry</subject><subject>Nuclear fuel elements</subject><subject>Oxidation</subject><subject>Oxygen</subject><subject>Oxygen content</subject><subject>RBMK</subject><subject>Spent nuclear fuels</subject><issn>1066-3622</issn><issn>1608-3288</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNp1kF9LwzAUxYMoOKcfwLeAz9WbP03TR51Oxelg1TehpE06OrqmJi26b29GBR_E-3IvnPM7Fw5C5wQuCWH8KiMgBBM0DDAAzg7QhAiQEaNSHoY7yNFeP0Yn3m8AQBIhJ-h9-VVr1de2xbbCWWfaHr8MZWOUw_PBNLhydovnjfo0Gq9unp8iEthRWlnt8dBq4_Ct2-Gst06tDZ7ZVtf7RH-KjirVeHP2s6fobX73OnuIFsv7x9n1IipJKvtIKOCy4loDF4koCpXEJhU0MUQkCSmVprHiRcK0iBnjMRSEUc2ogrSAVFHCpuhizO2c_RiM7_ONHVwbXuZUpDFPJWVxcJHRVTrrvTNV3rl6q9wuJ5DvS8z_lBgYOjI-eNu1cb_J_0Pftb1wKw</recordid><startdate>20220601</startdate><enddate>20220601</enddate><creator>Beznosyuk, V. I.</creator><creator>Krinitsyn, A. P.</creator><creator>Mishin, K. Ya</creator><creator>Metalidi, M. M.</creator><creator>Nikandrova, M. V.</creator><general>Pleiades Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20220601</creationdate><title>Oxidation of Spent Nuclear Fuel from Flawed RBMK-1000 Fuel Rods under Dry Storage Conditions</title><author>Beznosyuk, V. I. ; Krinitsyn, A. P. ; Mishin, K. Ya ; Metalidi, M. M. ; Nikandrova, M. V.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c198t-6a048f4dd04676bba75e9627e16771cad25a4b73d6533450b132d32a09b09a213</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chemistry/Food Science</topic><topic>Composition</topic><topic>Nitrogen</topic><topic>Nuclear Chemistry</topic><topic>Nuclear fuel elements</topic><topic>Oxidation</topic><topic>Oxygen</topic><topic>Oxygen content</topic><topic>RBMK</topic><topic>Spent nuclear fuels</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Beznosyuk, V. I.</creatorcontrib><creatorcontrib>Krinitsyn, A. P.</creatorcontrib><creatorcontrib>Mishin, K. Ya</creatorcontrib><creatorcontrib>Metalidi, M. M.</creatorcontrib><creatorcontrib>Nikandrova, M. V.</creatorcontrib><collection>CrossRef</collection><jtitle>Radiochemistry (New York, N.Y.)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Beznosyuk, V. I.</au><au>Krinitsyn, A. P.</au><au>Mishin, K. Ya</au><au>Metalidi, M. M.</au><au>Nikandrova, M. V.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Oxidation of Spent Nuclear Fuel from Flawed RBMK-1000 Fuel Rods under Dry Storage Conditions</atitle><jtitle>Radiochemistry (New York, N.Y.)</jtitle><stitle>Radiochemistry</stitle><date>2022-06-01</date><risdate>2022</risdate><volume>64</volume><issue>3</issue><spage>284</spage><epage>293</epage><pages>284-293</pages><issn>1066-3622</issn><eissn>1608-3288</eissn><abstract>The effect of a humid nitrogen atmosphere with an oxygen content of 0.08, 0.48, 1.30 vol % and a temperature of 300°С on the change in the structure of the RBMK-1000 fuel composition vs. the size of the defect in the fuel cladding was investigated. It was demonstrated that in the case of fuel cladding damage with an area of more than 0.8 mm
2
, SNF storage in a nitrogen atmosphere with an oxygen content of more than 0.5 vol % at a temperature of 300°C brings about a rather rapid oxidation of the fuel composition to U
3
O
8
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| issn | 1066-3622 1608-3288 |
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| source | Springer Journals |
| subjects | Chemistry Chemistry and Materials Science Chemistry/Food Science Composition Nitrogen Nuclear Chemistry Nuclear fuel elements Oxidation Oxygen Oxygen content RBMK Spent nuclear fuels |
| title | Oxidation of Spent Nuclear Fuel from Flawed RBMK-1000 Fuel Rods under Dry Storage Conditions |
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