Ultra-small Pd Nanoparticles Supported on Porous g-C3N4 Nanosheet for Efficient Hydrogenation Reaction
Heterogeneous catalytic hydrogenation reactions are of great significance in chemical industry. In this work, ultrasmall Pd nanoparticles (NPs) supported on porous g-C 3 N 4 nanosheets (Pd/CN) have been prepared for efficient hydrogenation reactions. The special structure of the catalytic metal–semi...
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| Veröffentlicht in: | Catalysis letters 2022-07, Vol.152 (7), p.2200-2205 |
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| creator | Yang, Liuqing Yu, Mengjie Fu, Xianglong Xie, Tongtong Pang, Zhiyuan Liu, Yanan Wang, Yangang |
| description | Heterogeneous catalytic hydrogenation reactions are of great significance in chemical industry. In this work, ultrasmall Pd nanoparticles (NPs) supported on porous g-C
3
N
4
nanosheets (Pd/CN) have been prepared for efficient hydrogenation reactions. The special structure of the catalytic metal–semiconductor heterojunction not only stabilize the Pd NPs but also improve their electronic activation. In addition, the high surface area of Pd/CN provides a large numbers of adsorption sites for styrene and H
2
. As a result, the optimized Pd/CN-0.5 nanocomposites achieved 100% conversion of styrene in 60 min under mild conditions.
Graphic Abstract |
| doi_str_mv | 10.1007/s10562-021-03812-4 |
| format | Article |
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3
N
4
nanosheets (Pd/CN) have been prepared for efficient hydrogenation reactions. The special structure of the catalytic metal–semiconductor heterojunction not only stabilize the Pd NPs but also improve their electronic activation. In addition, the high surface area of Pd/CN provides a large numbers of adsorption sites for styrene and H
2
. As a result, the optimized Pd/CN-0.5 nanocomposites achieved 100% conversion of styrene in 60 min under mild conditions.
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3
N
4
nanosheets (Pd/CN) have been prepared for efficient hydrogenation reactions. The special structure of the catalytic metal–semiconductor heterojunction not only stabilize the Pd NPs but also improve their electronic activation. In addition, the high surface area of Pd/CN provides a large numbers of adsorption sites for styrene and H
2
. As a result, the optimized Pd/CN-0.5 nanocomposites achieved 100% conversion of styrene in 60 min under mild conditions.
Graphic Abstract</description><subject>Activated carbon</subject><subject>Atoms & subatomic particles</subject><subject>Binding sites</subject><subject>Carbon nitride</subject><subject>Catalysis</subject><subject>Chemical industry</subject><subject>Chemical reactions</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Ethanol</subject><subject>Heterojunctions</subject><subject>Hydrogenation</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Nanocomposites</subject><subject>Nanoparticles</subject><subject>Nanosheets</subject><subject>Organometallic Chemistry</subject><subject>Palladium</subject><subject>Physical Chemistry</subject><subject>Styrenes</subject><issn>1011-372X</issn><issn>1572-879X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kM9LwzAYhoMoOKf_gKeA52h-tE1ylDGdMHSog91C2iSzo2tqkh7239utgjdP33t4nveDF4Bbgu8JxvwhEpwXFGFKEGaCUJSdgQnJOUWCy835kDEhiHG6uQRXMe4wxpITOQFu3aSgUdzrpoErA1916zsdUl01NsKPvut8SNZA38KVD76PcItm7DU7gfHL2gSdD3DuXF3Vtk1wcTDBb22rUz0471ZXx3ANLpxuor35vVOwfpp_zhZo-fb8MntcoooRmZA1RuSkLArDKS2YxIaIomTSuIKUmaScM1I6mVmRM4t1xThjkkpi8lxIziWbgruxtwv-u7cxqZ3vQzu8VLQQLMeZyPBA0ZGqgo8xWKe6UO91OCiC1XFPNe6phj3VaU-VDRIbpTjA7daGv-p_rB_e3HeA</recordid><startdate>20220701</startdate><enddate>20220701</enddate><creator>Yang, Liuqing</creator><creator>Yu, Mengjie</creator><creator>Fu, Xianglong</creator><creator>Xie, Tongtong</creator><creator>Pang, Zhiyuan</creator><creator>Liu, Yanan</creator><creator>Wang, Yangang</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope></search><sort><creationdate>20220701</creationdate><title>Ultra-small Pd Nanoparticles Supported on Porous g-C3N4 Nanosheet for Efficient Hydrogenation Reaction</title><author>Yang, Liuqing ; Yu, Mengjie ; Fu, Xianglong ; Xie, Tongtong ; Pang, Zhiyuan ; Liu, Yanan ; Wang, Yangang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-edd851b66d7226390d186b39df61b4927731bf94e853e0ac37339291d55897793</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Activated carbon</topic><topic>Atoms & subatomic particles</topic><topic>Binding sites</topic><topic>Carbon nitride</topic><topic>Catalysis</topic><topic>Chemical industry</topic><topic>Chemical reactions</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Ethanol</topic><topic>Heterojunctions</topic><topic>Hydrogenation</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Nanocomposites</topic><topic>Nanoparticles</topic><topic>Nanosheets</topic><topic>Organometallic Chemistry</topic><topic>Palladium</topic><topic>Physical Chemistry</topic><topic>Styrenes</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Liuqing</creatorcontrib><creatorcontrib>Yu, Mengjie</creatorcontrib><creatorcontrib>Fu, Xianglong</creatorcontrib><creatorcontrib>Xie, Tongtong</creatorcontrib><creatorcontrib>Pang, Zhiyuan</creatorcontrib><creatorcontrib>Liu, Yanan</creatorcontrib><creatorcontrib>Wang, Yangang</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials science collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><jtitle>Catalysis letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yang, Liuqing</au><au>Yu, Mengjie</au><au>Fu, Xianglong</au><au>Xie, Tongtong</au><au>Pang, Zhiyuan</au><au>Liu, Yanan</au><au>Wang, Yangang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ultra-small Pd Nanoparticles Supported on Porous g-C3N4 Nanosheet for Efficient Hydrogenation Reaction</atitle><jtitle>Catalysis letters</jtitle><stitle>Catal Lett</stitle><date>2022-07-01</date><risdate>2022</risdate><volume>152</volume><issue>7</issue><spage>2200</spage><epage>2205</epage><pages>2200-2205</pages><issn>1011-372X</issn><eissn>1572-879X</eissn><abstract>Heterogeneous catalytic hydrogenation reactions are of great significance in chemical industry. In this work, ultrasmall Pd nanoparticles (NPs) supported on porous g-C
3
N
4
nanosheets (Pd/CN) have been prepared for efficient hydrogenation reactions. The special structure of the catalytic metal–semiconductor heterojunction not only stabilize the Pd NPs but also improve their electronic activation. In addition, the high surface area of Pd/CN provides a large numbers of adsorption sites for styrene and H
2
. As a result, the optimized Pd/CN-0.5 nanocomposites achieved 100% conversion of styrene in 60 min under mild conditions.
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| subjects | Activated carbon Atoms & subatomic particles Binding sites Carbon nitride Catalysis Chemical industry Chemical reactions Chemistry Chemistry and Materials Science Ethanol Heterojunctions Hydrogenation Industrial Chemistry/Chemical Engineering Nanocomposites Nanoparticles Nanosheets Organometallic Chemistry Palladium Physical Chemistry Styrenes |
| title | Ultra-small Pd Nanoparticles Supported on Porous g-C3N4 Nanosheet for Efficient Hydrogenation Reaction |
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