Structural, dielectric, impedance and modulus studies of lead-free (1 − x)Bi0.5Na0.5TiO3−xBaTiO3(x = 0,0.06,0.08)-based ceramics
Lead free (1 − x )Bi 0.5 Na 0.5 TiO 3 − x BaTiO 3 ; x = 0.0, 0.06 and 0.08 solid solution in the proximity of morphotropic phase boundary were synthesized by conventional solid state technique. The addition of BaTiO 3 is found to affect the structural and dielectric properties of Bi 0.5 Na 0.5 T...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2022-05, Vol.33 (15), p.12281-12294 |
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| container_title | Journal of materials science. Materials in electronics |
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| creator | Kaur, Kamal deep Gautam, Anamol Shakti, Nanda Uniyal, Poonam |
| description | Lead free (1 −
x
)Bi
0.5
Na
0.5
TiO
3
−
x
BaTiO
3
;
x
= 0.0, 0.06 and 0.08 solid solution in the proximity of morphotropic phase boundary were synthesized by conventional solid state technique. The addition of BaTiO
3
is found to affect the structural and dielectric properties of Bi
0.5
Na
0.5
TiO
3.
It was evidenced by X-ray diffraction that the samples exhibit the combination of two phases orthorhombic (major) and minor traits of tetragonal phase. Scanning electron micrograph revealed the regular-shaped grains with dense microstructure. The dielectric properties of the synthesized samples were studied in wide frequency range (100 Hz–1 MHz) at various temperatures upto 450 °C. From impedance and modulus spectroscopy it has been found that there exists a non-Debye relaxation in the synthesized samples. The contribution of capacitance of grain and grain boundary in the conduction mechanism of the synthesized samples at higher temperatures is reported. The synthesized ceramics show the negative temperature coefficient of resistivity. The studied material shows a relaxor behavior with wide operating temperature window for various dielectric, piezoelectric and ferroelectric applications. |
| doi_str_mv | 10.1007/s10854-022-08187-9 |
| format | Article |
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x
)Bi
0.5
Na
0.5
TiO
3
−
x
BaTiO
3
;
x
= 0.0, 0.06 and 0.08 solid solution in the proximity of morphotropic phase boundary were synthesized by conventional solid state technique. The addition of BaTiO
3
is found to affect the structural and dielectric properties of Bi
0.5
Na
0.5
TiO
3.
It was evidenced by X-ray diffraction that the samples exhibit the combination of two phases orthorhombic (major) and minor traits of tetragonal phase. Scanning electron micrograph revealed the regular-shaped grains with dense microstructure. The dielectric properties of the synthesized samples were studied in wide frequency range (100 Hz–1 MHz) at various temperatures upto 450 °C. From impedance and modulus spectroscopy it has been found that there exists a non-Debye relaxation in the synthesized samples. The contribution of capacitance of grain and grain boundary in the conduction mechanism of the synthesized samples at higher temperatures is reported. The synthesized ceramics show the negative temperature coefficient of resistivity. The studied material shows a relaxor behavior with wide operating temperature window for various dielectric, piezoelectric and ferroelectric applications.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-022-08187-9</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Barium titanates ; Bismuth titanate ; Ceramics ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Dielectric properties ; Electron micrographs ; Ferroelectricity ; Frequency ranges ; Grain boundaries ; Impedance ; Lead free ; Materials Science ; Operating temperature ; Optical and Electronic Materials ; Piezoelectricity ; Solid solutions ; Synthesis</subject><ispartof>Journal of materials science. Materials in electronics, 2022-05, Vol.33 (15), p.12281-12294</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022</rights><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c2349-b76fb6f13e6a6dea5412994e813142dbd713cce3956fac800a3969ef91766ce53</citedby><cites>FETCH-LOGICAL-c2349-b76fb6f13e6a6dea5412994e813142dbd713cce3956fac800a3969ef91766ce53</cites><orcidid>0000-0002-2779-9647</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-022-08187-9$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-022-08187-9$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Kaur, Kamal deep</creatorcontrib><creatorcontrib>Gautam, Anamol</creatorcontrib><creatorcontrib>Shakti, Nanda</creatorcontrib><creatorcontrib>Uniyal, Poonam</creatorcontrib><title>Structural, dielectric, impedance and modulus studies of lead-free (1 − x)Bi0.5Na0.5TiO3−xBaTiO3(x = 0,0.06,0.08)-based ceramics</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>Lead free (1 −
x
)Bi
0.5
Na
0.5
TiO
3
−
x
BaTiO
3
;
x
= 0.0, 0.06 and 0.08 solid solution in the proximity of morphotropic phase boundary were synthesized by conventional solid state technique. The addition of BaTiO
3
is found to affect the structural and dielectric properties of Bi
0.5
Na
0.5
TiO
3.
It was evidenced by X-ray diffraction that the samples exhibit the combination of two phases orthorhombic (major) and minor traits of tetragonal phase. Scanning electron micrograph revealed the regular-shaped grains with dense microstructure. The dielectric properties of the synthesized samples were studied in wide frequency range (100 Hz–1 MHz) at various temperatures upto 450 °C. From impedance and modulus spectroscopy it has been found that there exists a non-Debye relaxation in the synthesized samples. The contribution of capacitance of grain and grain boundary in the conduction mechanism of the synthesized samples at higher temperatures is reported. The synthesized ceramics show the negative temperature coefficient of resistivity. The studied material shows a relaxor behavior with wide operating temperature window for various dielectric, piezoelectric and ferroelectric applications.</description><subject>Barium titanates</subject><subject>Bismuth titanate</subject><subject>Ceramics</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Dielectric properties</subject><subject>Electron micrographs</subject><subject>Ferroelectricity</subject><subject>Frequency ranges</subject><subject>Grain boundaries</subject><subject>Impedance</subject><subject>Lead free</subject><subject>Materials Science</subject><subject>Operating temperature</subject><subject>Optical and Electronic Materials</subject><subject>Piezoelectricity</subject><subject>Solid solutions</subject><subject>Synthesis</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9UD1rHDEQFSGGXOz8gVSCNDaczqOP1UpFCtv4I2DsIg6kEzppNqzZu71Iu3DuXNrgyj_Rv8S6XMCdi3kzzLz3Bh4hXznMOEB9mDmYSjEQgoHhpmb2A5nwqpZMGfH7I5mArWqmKiE-kc853wKAVtJMyNPPIY1hGJPvpjS22GEYUhumtF2sMPplQOqXkS76OHZjpnkYCynTvqEd-siahEj3-cv948vDc8H1wXELs-rKF7hpr2XZro_9Ztpfl_P3UjCFGegNmAM29xkjDZj8og15j-w0vsv45X_fJb_OTm9OLtjl9fmPk6NLFoRUls1r3cx1wyVqryP6SnFhrULDJVcizmPNZQgobaUbHwyAl1ZbbCyvtQ5YyV3ybeu7Sv3fEfPgbvsxLctLJ7RWApQwprDElhVSn3PCxq1Su_DpznFwm9TdNnVXUnf_Une2iORWlAt5-QfTm_U7qlf3tYdv</recordid><startdate>20220501</startdate><enddate>20220501</enddate><creator>Kaur, Kamal deep</creator><creator>Gautam, Anamol</creator><creator>Shakti, Nanda</creator><creator>Uniyal, Poonam</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0002-2779-9647</orcidid></search><sort><creationdate>20220501</creationdate><title>Structural, dielectric, impedance and modulus studies of lead-free (1 − x)Bi0.5Na0.5TiO3−xBaTiO3(x = 0,0.06,0.08)-based ceramics</title><author>Kaur, Kamal deep ; Gautam, Anamol ; Shakti, Nanda ; Uniyal, Poonam</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c2349-b76fb6f13e6a6dea5412994e813142dbd713cce3956fac800a3969ef91766ce53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Barium titanates</topic><topic>Bismuth titanate</topic><topic>Ceramics</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Dielectric properties</topic><topic>Electron micrographs</topic><topic>Ferroelectricity</topic><topic>Frequency ranges</topic><topic>Grain boundaries</topic><topic>Impedance</topic><topic>Lead free</topic><topic>Materials Science</topic><topic>Operating temperature</topic><topic>Optical and Electronic Materials</topic><topic>Piezoelectricity</topic><topic>Solid solutions</topic><topic>Synthesis</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Kaur, Kamal deep</creatorcontrib><creatorcontrib>Gautam, Anamol</creatorcontrib><creatorcontrib>Shakti, Nanda</creatorcontrib><creatorcontrib>Uniyal, Poonam</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Kaur, Kamal deep</au><au>Gautam, Anamol</au><au>Shakti, Nanda</au><au>Uniyal, Poonam</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Structural, dielectric, impedance and modulus studies of lead-free (1 − x)Bi0.5Na0.5TiO3−xBaTiO3(x = 0,0.06,0.08)-based ceramics</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2022-05-01</date><risdate>2022</risdate><volume>33</volume><issue>15</issue><spage>12281</spage><epage>12294</epage><pages>12281-12294</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>Lead free (1 −
x
)Bi
0.5
Na
0.5
TiO
3
−
x
BaTiO
3
;
x
= 0.0, 0.06 and 0.08 solid solution in the proximity of morphotropic phase boundary were synthesized by conventional solid state technique. The addition of BaTiO
3
is found to affect the structural and dielectric properties of Bi
0.5
Na
0.5
TiO
3.
It was evidenced by X-ray diffraction that the samples exhibit the combination of two phases orthorhombic (major) and minor traits of tetragonal phase. Scanning electron micrograph revealed the regular-shaped grains with dense microstructure. The dielectric properties of the synthesized samples were studied in wide frequency range (100 Hz–1 MHz) at various temperatures upto 450 °C. From impedance and modulus spectroscopy it has been found that there exists a non-Debye relaxation in the synthesized samples. The contribution of capacitance of grain and grain boundary in the conduction mechanism of the synthesized samples at higher temperatures is reported. The synthesized ceramics show the negative temperature coefficient of resistivity. The studied material shows a relaxor behavior with wide operating temperature window for various dielectric, piezoelectric and ferroelectric applications.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-022-08187-9</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0002-2779-9647</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0957-4522 |
| ispartof | Journal of materials science. Materials in electronics, 2022-05, Vol.33 (15), p.12281-12294 |
| issn | 0957-4522 1573-482X |
| language | eng |
| recordid | cdi_proquest_journals_2664204288 |
| source | SpringerNature Journals |
| subjects | Barium titanates Bismuth titanate Ceramics Characterization and Evaluation of Materials Chemistry and Materials Science Dielectric properties Electron micrographs Ferroelectricity Frequency ranges Grain boundaries Impedance Lead free Materials Science Operating temperature Optical and Electronic Materials Piezoelectricity Solid solutions Synthesis |
| title | Structural, dielectric, impedance and modulus studies of lead-free (1 − x)Bi0.5Na0.5TiO3−xBaTiO3(x = 0,0.06,0.08)-based ceramics |
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