Synthesis of amidoximated polyacrylonitrile/sodium alginate composite hydrogel beed and its use in selective and recyclable removal of U(VI)
In this study, a novel type of composite hydrogel bead (PSH) was prepared by mixing of amidoximated polyacrylonitrile (PAO) and sodium alginate (SA). The structure of PSH was characterized with FT-IR, SEM and XPS. The influences of adsorption conditions on uranium(VI) adsorption by PSH were investig...
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Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2022-04, Vol.331 (4), p.1669-1682 |
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container_title | Journal of radioanalytical and nuclear chemistry |
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creator | Zhu, Bingyu Li, Le Dai, Zhongran Tang, Shuangyang Zhen, Deshuai Sun, Lin Chen, Lei Tuo, Chen Tang, Ziwei |
description | In this study, a novel type of composite hydrogel bead (PSH) was prepared by mixing of amidoximated polyacrylonitrile (PAO) and sodium alginate (SA). The structure of PSH was characterized with FT-IR, SEM and XPS. The influences of adsorption conditions on uranium(VI) adsorption by PSH were investigated by batch experiments. The kinetic and isotherm data were consistent with pseudo-second-order and Langmuir models, respectively. PSH displayed high selective adsorption capacity for uranium(VI). The maximum adsorption amount can reach 133.33 mg g
−1
. PSH was separated from aqueous solution easy and showed an excellent regeneration capacity. This research demonstrated that PSH had a broad prospect of application in the field of repairing uranium-containing wastewater. |
doi_str_mv | 10.1007/s10967-022-08233-0 |
format | Article |
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−1
. PSH was separated from aqueous solution easy and showed an excellent regeneration capacity. This research demonstrated that PSH had a broad prospect of application in the field of repairing uranium-containing wastewater.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-022-08233-0</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Adsorption ; Analysis ; Aqueous solutions ; Chemistry ; Chemistry and Materials Science ; Diagnostic Radiology ; Hadrons ; Heavy Ions ; Hydrogels ; Inorganic Chemistry ; Nuclear Chemistry ; Nuclear Physics ; Physical Chemistry ; Polyacrylonitrile ; Selective adsorption ; Sodium alginate ; Uranium ; Wastewater ; X ray photoelectron spectroscopy</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2022-04, Vol.331 (4), p.1669-1682</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2022</rights><rights>COPYRIGHT 2022 Springer</rights><rights>Akadémiai Kiadó, Budapest, Hungary 2022.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c358t-4f7fb2672590ec3ec1c5023c20c4e3acafca8c9540a42a17ad33c7b7b023bfe13</citedby><cites>FETCH-LOGICAL-c358t-4f7fb2672590ec3ec1c5023c20c4e3acafca8c9540a42a17ad33c7b7b023bfe13</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-022-08233-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-022-08233-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,782,786,27933,27934,41497,42566,51328</link.rule.ids></links><search><creatorcontrib>Zhu, Bingyu</creatorcontrib><creatorcontrib>Li, Le</creatorcontrib><creatorcontrib>Dai, Zhongran</creatorcontrib><creatorcontrib>Tang, Shuangyang</creatorcontrib><creatorcontrib>Zhen, Deshuai</creatorcontrib><creatorcontrib>Sun, Lin</creatorcontrib><creatorcontrib>Chen, Lei</creatorcontrib><creatorcontrib>Tuo, Chen</creatorcontrib><creatorcontrib>Tang, Ziwei</creatorcontrib><title>Synthesis of amidoximated polyacrylonitrile/sodium alginate composite hydrogel beed and its use in selective and recyclable removal of U(VI)</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>In this study, a novel type of composite hydrogel bead (PSH) was prepared by mixing of amidoximated polyacrylonitrile (PAO) and sodium alginate (SA). The structure of PSH was characterized with FT-IR, SEM and XPS. The influences of adsorption conditions on uranium(VI) adsorption by PSH were investigated by batch experiments. The kinetic and isotherm data were consistent with pseudo-second-order and Langmuir models, respectively. PSH displayed high selective adsorption capacity for uranium(VI). The maximum adsorption amount can reach 133.33 mg g
−1
. PSH was separated from aqueous solution easy and showed an excellent regeneration capacity. This research demonstrated that PSH had a broad prospect of application in the field of repairing uranium-containing wastewater.</description><subject>Adsorption</subject><subject>Analysis</subject><subject>Aqueous solutions</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Diagnostic Radiology</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Hydrogels</subject><subject>Inorganic Chemistry</subject><subject>Nuclear Chemistry</subject><subject>Nuclear Physics</subject><subject>Physical Chemistry</subject><subject>Polyacrylonitrile</subject><subject>Selective adsorption</subject><subject>Sodium alginate</subject><subject>Uranium</subject><subject>Wastewater</subject><subject>X ray photoelectron spectroscopy</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNp9kc1u3SAQRlHVSr1N8gJZIXXTLpwMYBu8jKL-RIrURZNuEcbDDRGGW_CN6nfoQ5fElbrripE4ZwbmI-ScwQUDkJeFwdDLBjhvQHEhGnhFdqxTquFSwWuyAy76ppOCvSXvSnkEgEEpsSO_v69xecDiC02OmtlP6ZefzYITPaSwGpvXkKJfsg94WdLkjzM1Ye9jRahN8yEVX6uHdcppj4GOWE0TJ-qXQo8FqY-0YEC7-Cd8uchoVxvMGLCWc3oy4Xny_YcfNx9PyRtnQsGzv-cJuf_86e76a3P77cvN9dVtY0WnlqZ10o28l7wbAK1Ay2xX_2c52BaFscZZo-zQtWBabpg0kxBWjnKs0OiQiRPyfut7yOnnEcuiH9MxxzpS877jPQPRdpW62Ki9Cah9dGnJtbk1E87epoiu7kRfSWDAlRiGKvBNsDmVktHpQ667zKtmoJ9j0ltMusakX2LSUCWxSaXCcY_531v-Y_0BFH2YGA</recordid><startdate>20220401</startdate><enddate>20220401</enddate><creator>Zhu, Bingyu</creator><creator>Li, Le</creator><creator>Dai, Zhongran</creator><creator>Tang, Shuangyang</creator><creator>Zhen, Deshuai</creator><creator>Sun, Lin</creator><creator>Chen, Lei</creator><creator>Tuo, Chen</creator><creator>Tang, Ziwei</creator><general>Springer International Publishing</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20220401</creationdate><title>Synthesis of amidoximated polyacrylonitrile/sodium alginate composite hydrogel beed and its use in selective and recyclable removal of U(VI)</title><author>Zhu, Bingyu ; Li, Le ; Dai, Zhongran ; Tang, Shuangyang ; Zhen, Deshuai ; Sun, Lin ; Chen, Lei ; Tuo, Chen ; Tang, Ziwei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c358t-4f7fb2672590ec3ec1c5023c20c4e3acafca8c9540a42a17ad33c7b7b023bfe13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Adsorption</topic><topic>Analysis</topic><topic>Aqueous solutions</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Diagnostic Radiology</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Hydrogels</topic><topic>Inorganic Chemistry</topic><topic>Nuclear Chemistry</topic><topic>Nuclear Physics</topic><topic>Physical Chemistry</topic><topic>Polyacrylonitrile</topic><topic>Selective adsorption</topic><topic>Sodium alginate</topic><topic>Uranium</topic><topic>Wastewater</topic><topic>X ray photoelectron spectroscopy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhu, Bingyu</creatorcontrib><creatorcontrib>Li, Le</creatorcontrib><creatorcontrib>Dai, Zhongran</creatorcontrib><creatorcontrib>Tang, Shuangyang</creatorcontrib><creatorcontrib>Zhen, Deshuai</creatorcontrib><creatorcontrib>Sun, Lin</creatorcontrib><creatorcontrib>Chen, Lei</creatorcontrib><creatorcontrib>Tuo, Chen</creatorcontrib><creatorcontrib>Tang, Ziwei</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhu, Bingyu</au><au>Li, Le</au><au>Dai, Zhongran</au><au>Tang, Shuangyang</au><au>Zhen, Deshuai</au><au>Sun, Lin</au><au>Chen, Lei</au><au>Tuo, Chen</au><au>Tang, Ziwei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis of amidoximated polyacrylonitrile/sodium alginate composite hydrogel beed and its use in selective and recyclable removal of U(VI)</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2022-04-01</date><risdate>2022</risdate><volume>331</volume><issue>4</issue><spage>1669</spage><epage>1682</epage><pages>1669-1682</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>In this study, a novel type of composite hydrogel bead (PSH) was prepared by mixing of amidoximated polyacrylonitrile (PAO) and sodium alginate (SA). 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−1
. PSH was separated from aqueous solution easy and showed an excellent regeneration capacity. This research demonstrated that PSH had a broad prospect of application in the field of repairing uranium-containing wastewater.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10967-022-08233-0</doi><tpages>14</tpages></addata></record> |
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subjects | Adsorption Analysis Aqueous solutions Chemistry Chemistry and Materials Science Diagnostic Radiology Hadrons Heavy Ions Hydrogels Inorganic Chemistry Nuclear Chemistry Nuclear Physics Physical Chemistry Polyacrylonitrile Selective adsorption Sodium alginate Uranium Wastewater X ray photoelectron spectroscopy |
title | Synthesis of amidoximated polyacrylonitrile/sodium alginate composite hydrogel beed and its use in selective and recyclable removal of U(VI) |
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