Multiple Response Optimization of Poly(vinyl alcohol)/Starch Based Bioactive Composite Films for Antimicrobial Packaging Applications
In this work, the incorporation of additives i.e. glycerol, citric acid and zinc oxide at four-levels into poly(vinyl alcohol)/starch (PSt) films containing extracted spent coffee ground (ex-SCG) was designed and optimized using Taguchi method combined with Grey relational analysis. Citric acid was...
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| Veröffentlicht in: | Journal of polymers and the environment 2022-05, Vol.30 (5), p.1787-1802 |
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| creator | Ounkaew, Artjima Kasemsiri, Pornnapa Pongsa, Uraiwan Hiziroglu, Salim Pasuwan, Patimakorn Boonlai, Yuwasiri Theerakulpisut, Somnuk |
| description | In this work, the incorporation of additives i.e. glycerol, citric acid and zinc oxide at four-levels into poly(vinyl alcohol)/starch (PSt) films containing extracted spent coffee ground (ex-SCG) was designed and optimized using Taguchi method combined with Grey relational analysis. Citric acid was the most significant parameter affecting the antibacterial activity against
Escherichia coli
(
E. coli
) and
Staphylococcus aureus
(
S. aureus
)
.
Addition of glycerol in PSt films enhanced water resistance and biodegradability of the samples, but decreased their tensile strength and modulus values. The presence of ZnO increased the tensile strength of PSt films. The Grey relational analysis showed that the optimal mix proportion for PSt film could be achieved at 10 wt% glycerol, 45 wt% citric acid and 1 wt% ZnO. The PSt films based on the optimized mix proportion of additives were used as packaging for fresh cherry tomatoes. The films remarkably inhibited growth of bacteria and maintained freshness of the packaged cherry tomatoes. Based on the finding in this work, experimentally made PSt films could have a potential for food preservation and antimicrobial packaging applications to enhance the quality and to extend the shelf-life of fresh fruits and vegetables.
Graphic Abstract |
| doi_str_mv | 10.1007/s10924-021-02308-x |
| format | Article |
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Escherichia coli
(
E. coli
) and
Staphylococcus aureus
(
S. aureus
)
.
Addition of glycerol in PSt films enhanced water resistance and biodegradability of the samples, but decreased their tensile strength and modulus values. The presence of ZnO increased the tensile strength of PSt films. The Grey relational analysis showed that the optimal mix proportion for PSt film could be achieved at 10 wt% glycerol, 45 wt% citric acid and 1 wt% ZnO. The PSt films based on the optimized mix proportion of additives were used as packaging for fresh cherry tomatoes. The films remarkably inhibited growth of bacteria and maintained freshness of the packaged cherry tomatoes. Based on the finding in this work, experimentally made PSt films could have a potential for food preservation and antimicrobial packaging applications to enhance the quality and to extend the shelf-life of fresh fruits and vegetables.
Graphic Abstract</description><identifier>ISSN: 1566-2543</identifier><identifier>EISSN: 1572-8919</identifier><identifier>DOI: 10.1007/s10924-021-02308-x</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Additives ; Antibacterial activity ; Antimicrobial agents ; Biocompatibility ; Biodegradability ; Biodegradation ; Biomedical materials ; Chemistry ; Chemistry and Materials Science ; Citric acid ; Coffee ; Composite materials ; E coli ; Environmental Chemistry ; Environmental Engineering/Biotechnology ; Food packaging ; Food preservation ; Freshness ; Fruits ; Glycerol ; Industrial Chemistry/Chemical Engineering ; Materials Science ; Optimization ; Original Paper ; Packaging ; Polymer Sciences ; Polyvinyl alcohol ; Shelf life ; Starch ; Taguchi methods ; Tensile strength ; Tomatoes ; Water resistance ; Zinc oxide ; Zinc oxides</subject><ispartof>Journal of polymers and the environment, 2022-05, Vol.30 (5), p.1787-1802</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-9c5e5d4c1c346d2188106bce52e6114bf1ee64035ca8fd7eb78a24f0c165dafb3</citedby><cites>FETCH-LOGICAL-c319t-9c5e5d4c1c346d2188106bce52e6114bf1ee64035ca8fd7eb78a24f0c165dafb3</cites><orcidid>0000-0002-0834-708X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10924-021-02308-x$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10924-021-02308-x$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Ounkaew, Artjima</creatorcontrib><creatorcontrib>Kasemsiri, Pornnapa</creatorcontrib><creatorcontrib>Pongsa, Uraiwan</creatorcontrib><creatorcontrib>Hiziroglu, Salim</creatorcontrib><creatorcontrib>Pasuwan, Patimakorn</creatorcontrib><creatorcontrib>Boonlai, Yuwasiri</creatorcontrib><creatorcontrib>Theerakulpisut, Somnuk</creatorcontrib><title>Multiple Response Optimization of Poly(vinyl alcohol)/Starch Based Bioactive Composite Films for Antimicrobial Packaging Applications</title><title>Journal of polymers and the environment</title><addtitle>J Polym Environ</addtitle><description>In this work, the incorporation of additives i.e. glycerol, citric acid and zinc oxide at four-levels into poly(vinyl alcohol)/starch (PSt) films containing extracted spent coffee ground (ex-SCG) was designed and optimized using Taguchi method combined with Grey relational analysis. Citric acid was the most significant parameter affecting the antibacterial activity against
Escherichia coli
(
E. coli
) and
Staphylococcus aureus
(
S. aureus
)
.
Addition of glycerol in PSt films enhanced water resistance and biodegradability of the samples, but decreased their tensile strength and modulus values. The presence of ZnO increased the tensile strength of PSt films. The Grey relational analysis showed that the optimal mix proportion for PSt film could be achieved at 10 wt% glycerol, 45 wt% citric acid and 1 wt% ZnO. The PSt films based on the optimized mix proportion of additives were used as packaging for fresh cherry tomatoes. The films remarkably inhibited growth of bacteria and maintained freshness of the packaged cherry tomatoes. Based on the finding in this work, experimentally made PSt films could have a potential for food preservation and antimicrobial packaging applications to enhance the quality and to extend the shelf-life of fresh fruits and vegetables.
Graphic Abstract</description><subject>Additives</subject><subject>Antibacterial activity</subject><subject>Antimicrobial agents</subject><subject>Biocompatibility</subject><subject>Biodegradability</subject><subject>Biodegradation</subject><subject>Biomedical materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Citric acid</subject><subject>Coffee</subject><subject>Composite materials</subject><subject>E coli</subject><subject>Environmental Chemistry</subject><subject>Environmental Engineering/Biotechnology</subject><subject>Food packaging</subject><subject>Food preservation</subject><subject>Freshness</subject><subject>Fruits</subject><subject>Glycerol</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Materials Science</subject><subject>Optimization</subject><subject>Original Paper</subject><subject>Packaging</subject><subject>Polymer Sciences</subject><subject>Polyvinyl alcohol</subject><subject>Shelf life</subject><subject>Starch</subject><subject>Taguchi methods</subject><subject>Tensile strength</subject><subject>Tomatoes</subject><subject>Water resistance</subject><subject>Zinc oxide</subject><subject>Zinc oxides</subject><issn>1566-2543</issn><issn>1572-8919</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kDtPwzAUhSMEEqXwB5gsscAQ6lecZGwrCkhFVDxmy3Gc1sWJg51WLTv_G7dFYmO4unc43zlXJ4ouEbxFEKYDj2COaQwxCkNgFm-Ooh5KUhxnOcqPdzdjMU4oOY3OvF9CCPMA9qLvp5XpdGsUeFG-tY1X4LntdK2_RKdtA2wFZtZsr9e62RogjLQLa24Gr51wcgFGwqsSjLQVstNrBca2bq3XnQITbWoPKuvAsNnZSWcLLQyYCfkh5rqZg2HbGi33Kf48OqmE8erid_ej98nd2_ghnj7fP46H01gSlHdxLhOVlFQiSSgrMcoyBFkhVYIVQ4gWFVKKUUgSKbKqTFWRZgLTCkrEklJUBelHVwff1tnPlfIdX9qVa0Ikx4yyjGSQ4KDCB1V42nunKt46XQu35QjyXd38UDcPdfN93XwTIHKAfBA3c-X-rP-hfgAwjYYi</recordid><startdate>20220501</startdate><enddate>20220501</enddate><creator>Ounkaew, Artjima</creator><creator>Kasemsiri, Pornnapa</creator><creator>Pongsa, Uraiwan</creator><creator>Hiziroglu, Salim</creator><creator>Pasuwan, Patimakorn</creator><creator>Boonlai, Yuwasiri</creator><creator>Theerakulpisut, Somnuk</creator><general>Springer US</general><general>Springer Nature 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Artjima ; Kasemsiri, Pornnapa ; Pongsa, Uraiwan ; Hiziroglu, Salim ; Pasuwan, Patimakorn ; Boonlai, Yuwasiri ; Theerakulpisut, Somnuk</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-9c5e5d4c1c346d2188106bce52e6114bf1ee64035ca8fd7eb78a24f0c165dafb3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Additives</topic><topic>Antibacterial activity</topic><topic>Antimicrobial agents</topic><topic>Biocompatibility</topic><topic>Biodegradability</topic><topic>Biodegradation</topic><topic>Biomedical materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Citric acid</topic><topic>Coffee</topic><topic>Composite materials</topic><topic>E coli</topic><topic>Environmental Chemistry</topic><topic>Environmental Engineering/Biotechnology</topic><topic>Food packaging</topic><topic>Food preservation</topic><topic>Freshness</topic><topic>Fruits</topic><topic>Glycerol</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Materials Science</topic><topic>Optimization</topic><topic>Original Paper</topic><topic>Packaging</topic><topic>Polymer Sciences</topic><topic>Polyvinyl alcohol</topic><topic>Shelf life</topic><topic>Starch</topic><topic>Taguchi methods</topic><topic>Tensile strength</topic><topic>Tomatoes</topic><topic>Water resistance</topic><topic>Zinc oxide</topic><topic>Zinc oxides</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ounkaew, Artjima</creatorcontrib><creatorcontrib>Kasemsiri, Pornnapa</creatorcontrib><creatorcontrib>Pongsa, Uraiwan</creatorcontrib><creatorcontrib>Hiziroglu, Salim</creatorcontrib><creatorcontrib>Pasuwan, Patimakorn</creatorcontrib><creatorcontrib>Boonlai, Yuwasiri</creatorcontrib><creatorcontrib>Theerakulpisut, 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Basic</collection><jtitle>Journal of polymers and the environment</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ounkaew, Artjima</au><au>Kasemsiri, Pornnapa</au><au>Pongsa, Uraiwan</au><au>Hiziroglu, Salim</au><au>Pasuwan, Patimakorn</au><au>Boonlai, Yuwasiri</au><au>Theerakulpisut, Somnuk</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Multiple Response Optimization of Poly(vinyl alcohol)/Starch Based Bioactive Composite Films for Antimicrobial Packaging Applications</atitle><jtitle>Journal of polymers and the environment</jtitle><stitle>J Polym Environ</stitle><date>2022-05-01</date><risdate>2022</risdate><volume>30</volume><issue>5</issue><spage>1787</spage><epage>1802</epage><pages>1787-1802</pages><issn>1566-2543</issn><eissn>1572-8919</eissn><abstract>In this work, the incorporation of additives i.e. glycerol, citric acid and zinc oxide at four-levels into poly(vinyl alcohol)/starch (PSt) films containing extracted spent coffee ground (ex-SCG) was designed and optimized using Taguchi method combined with Grey relational analysis. Citric acid was the most significant parameter affecting the antibacterial activity against
Escherichia coli
(
E. coli
) and
Staphylococcus aureus
(
S. aureus
)
.
Addition of glycerol in PSt films enhanced water resistance and biodegradability of the samples, but decreased their tensile strength and modulus values. The presence of ZnO increased the tensile strength of PSt films. The Grey relational analysis showed that the optimal mix proportion for PSt film could be achieved at 10 wt% glycerol, 45 wt% citric acid and 1 wt% ZnO. The PSt films based on the optimized mix proportion of additives were used as packaging for fresh cherry tomatoes. The films remarkably inhibited growth of bacteria and maintained freshness of the packaged cherry tomatoes. Based on the finding in this work, experimentally made PSt films could have a potential for food preservation and antimicrobial packaging applications to enhance the quality and to extend the shelf-life of fresh fruits and vegetables.
Graphic Abstract</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10924-021-02308-x</doi><tpages>16</tpages><orcidid>https://orcid.org/0000-0002-0834-708X</orcidid></addata></record> |
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| issn | 1566-2543 1572-8919 |
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| subjects | Additives Antibacterial activity Antimicrobial agents Biocompatibility Biodegradability Biodegradation Biomedical materials Chemistry Chemistry and Materials Science Citric acid Coffee Composite materials E coli Environmental Chemistry Environmental Engineering/Biotechnology Food packaging Food preservation Freshness Fruits Glycerol Industrial Chemistry/Chemical Engineering Materials Science Optimization Original Paper Packaging Polymer Sciences Polyvinyl alcohol Shelf life Starch Taguchi methods Tensile strength Tomatoes Water resistance Zinc oxide Zinc oxides |
| title | Multiple Response Optimization of Poly(vinyl alcohol)/Starch Based Bioactive Composite Films for Antimicrobial Packaging Applications |
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