Effects of cerium on structures and electrical properties of (Nb, Ta) modified Bi4Ti3O12 piezoelectric ceramics
Bi4Ti3O12 high‐temperature piezoelectric ceramics composed of 0.03 mol (Nb, Ta)5+ substituting B site and x mol CeO2 (x = 0–0.05, abbreviated as BCTNT100x) substituting A site were synthesized by the conventional solid‐state reaction method. The effects of Ce additive on the structures and electrica...
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| Veröffentlicht in: | Journal of the American Ceramic Society 2022-06, Vol.105 (6), p.4161-4170 |
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| container_title | Journal of the American Ceramic Society |
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| creator | Zhang, Feifei Xu, Yugen Yang, Heng Guan, Shangyi Shi, Wei Chen, Yulin Huang, Chenting Xing, Jie Liu, Hong Chen, Qiang |
| description | Bi4Ti3O12 high‐temperature piezoelectric ceramics composed of 0.03 mol (Nb, Ta)5+ substituting B site and x mol CeO2 (x = 0–0.05, abbreviated as BCTNT100x) substituting A site were synthesized by the conventional solid‐state reaction method. The effects of Ce additive on the structures and electrical properties of resulting Bi4Ti3O12‐based ceramics were systematically investigated. In‐situ temperature‐dependent X‐ray diffraction (XRD) confirmed that the phase structure of BCTNT100x ceramics change from orthorhombic structure to tetragonal structure as temperature increased. The ceramics at Ce content x = 0.03 illustrated optimal performances with superior piezoelectric constant (d33 = 36.5 pC/N), high Curie temperature (TC = 649 °C), and large remanent polarization (2Pr = 21.6 μC/cm2). BCTNT3 ceramics also possessed high d33 of 32.5 pC/N at an annealing temperature of 600°C, with electrical resistivity preserved at 106 Ω cm at 500 °C. These results demonstrate that BCTNT100x ceramics can be used as high‐temperature piezoelectric devices. |
| doi_str_mv | 10.1111/jace.18393 |
| format | Article |
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The effects of Ce additive on the structures and electrical properties of resulting Bi4Ti3O12‐based ceramics were systematically investigated. In‐situ temperature‐dependent X‐ray diffraction (XRD) confirmed that the phase structure of BCTNT100x ceramics change from orthorhombic structure to tetragonal structure as temperature increased. The ceramics at Ce content x = 0.03 illustrated optimal performances with superior piezoelectric constant (d33 = 36.5 pC/N), high Curie temperature (TC = 649 °C), and large remanent polarization (2Pr = 21.6 μC/cm2). BCTNT3 ceramics also possessed high d33 of 32.5 pC/N at an annealing temperature of 600°C, with electrical resistivity preserved at 106 Ω cm at 500 °C. These results demonstrate that BCTNT100x ceramics can be used as high‐temperature piezoelectric devices.</description><identifier>ISSN: 0002-7820</identifier><identifier>EISSN: 1551-2916</identifier><identifier>DOI: 10.1111/jace.18393</identifier><language>eng</language><publisher>Columbus: Wiley Subscription Services, Inc</publisher><subject>Bi4Ti3O12 ; Bismuth titanate ; Cerium oxides ; Curie temperature ; Electrical properties ; high curie temperature ; Niobium ; Piezoelectric ceramics ; Solid phases ; Tantalum ; Temperature dependence</subject><ispartof>Journal of the American Ceramic Society, 2022-06, Vol.105 (6), p.4161-4170</ispartof><rights>2022 The American Ceramic Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><orcidid>0000-0003-2260-246X ; 0000-0001-6805-4185 ; 0000-0001-8187-4583 ; 0000-0003-2800-5519</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1111%2Fjace.18393$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1111%2Fjace.18393$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27903,27904,45553,45554</link.rule.ids></links><search><creatorcontrib>Zhang, Feifei</creatorcontrib><creatorcontrib>Xu, Yugen</creatorcontrib><creatorcontrib>Yang, Heng</creatorcontrib><creatorcontrib>Guan, Shangyi</creatorcontrib><creatorcontrib>Shi, Wei</creatorcontrib><creatorcontrib>Chen, Yulin</creatorcontrib><creatorcontrib>Huang, Chenting</creatorcontrib><creatorcontrib>Xing, Jie</creatorcontrib><creatorcontrib>Liu, Hong</creatorcontrib><creatorcontrib>Chen, Qiang</creatorcontrib><title>Effects of cerium on structures and electrical properties of (Nb, Ta) modified Bi4Ti3O12 piezoelectric ceramics</title><title>Journal of the American Ceramic Society</title><description>Bi4Ti3O12 high‐temperature piezoelectric ceramics composed of 0.03 mol (Nb, Ta)5+ substituting B site and x mol CeO2 (x = 0–0.05, abbreviated as BCTNT100x) substituting A site were synthesized by the conventional solid‐state reaction method. The effects of Ce additive on the structures and electrical properties of resulting Bi4Ti3O12‐based ceramics were systematically investigated. In‐situ temperature‐dependent X‐ray diffraction (XRD) confirmed that the phase structure of BCTNT100x ceramics change from orthorhombic structure to tetragonal structure as temperature increased. The ceramics at Ce content x = 0.03 illustrated optimal performances with superior piezoelectric constant (d33 = 36.5 pC/N), high Curie temperature (TC = 649 °C), and large remanent polarization (2Pr = 21.6 μC/cm2). BCTNT3 ceramics also possessed high d33 of 32.5 pC/N at an annealing temperature of 600°C, with electrical resistivity preserved at 106 Ω cm at 500 °C. These results demonstrate that BCTNT100x ceramics can be used as high‐temperature piezoelectric devices.</description><subject>Bi4Ti3O12</subject><subject>Bismuth titanate</subject><subject>Cerium oxides</subject><subject>Curie temperature</subject><subject>Electrical properties</subject><subject>high curie temperature</subject><subject>Niobium</subject><subject>Piezoelectric ceramics</subject><subject>Solid phases</subject><subject>Tantalum</subject><subject>Temperature dependence</subject><issn>0002-7820</issn><issn>1551-2916</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNo1kE1LAzEQhoMoWKsXf0HAi4Jb87nNHmupXxR7qeeQnSSQsttdk12k_fVuW53LzMDzvjO8CN1SMqFDPW0MuAlVvOBnaESlpBkraH6ORoQQlk0VI5foKqXNsNJCiRFqFt476BJuPAYXQ1_jZotTF3vo-ugSNluLXTUgMYCpcBub1sUuuKPi_rN8xGvzgOvGBh-cxc9BrANfUYbb4PbNv_LgbeoA6RpdeFMld_PXx-jrZbGev2XL1ev7fLbMWsYkz6wqAWRJnbDMcuYlSMkZUwosn1pvnS0UECqsED63AEb4kpa5K6koYQqUj9HdyXd4-Lt3qdObpo_b4aRmuchzRaQSA0VP1E-o3E63MdQm7jQl-pCmPqSpj2nqj9l8cZz4L5TxaxM</recordid><startdate>202206</startdate><enddate>202206</enddate><creator>Zhang, Feifei</creator><creator>Xu, Yugen</creator><creator>Yang, Heng</creator><creator>Guan, Shangyi</creator><creator>Shi, Wei</creator><creator>Chen, Yulin</creator><creator>Huang, Chenting</creator><creator>Xing, Jie</creator><creator>Liu, Hong</creator><creator>Chen, Qiang</creator><general>Wiley Subscription Services, Inc</general><scope>7QQ</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope><orcidid>https://orcid.org/0000-0003-2260-246X</orcidid><orcidid>https://orcid.org/0000-0001-6805-4185</orcidid><orcidid>https://orcid.org/0000-0001-8187-4583</orcidid><orcidid>https://orcid.org/0000-0003-2800-5519</orcidid></search><sort><creationdate>202206</creationdate><title>Effects of cerium on structures and electrical properties of (Nb, Ta) modified Bi4Ti3O12 piezoelectric ceramics</title><author>Zhang, Feifei ; Xu, Yugen ; Yang, Heng ; Guan, Shangyi ; Shi, Wei ; Chen, Yulin ; Huang, Chenting ; Xing, Jie ; Liu, Hong ; Chen, Qiang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p2253-d8bcc5b1e4d2d32f5c5532288cd37dfded98c014d44f6dcca4fb1b6eb14bc7c13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Bi4Ti3O12</topic><topic>Bismuth titanate</topic><topic>Cerium oxides</topic><topic>Curie temperature</topic><topic>Electrical properties</topic><topic>high curie temperature</topic><topic>Niobium</topic><topic>Piezoelectric ceramics</topic><topic>Solid phases</topic><topic>Tantalum</topic><topic>Temperature dependence</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Feifei</creatorcontrib><creatorcontrib>Xu, Yugen</creatorcontrib><creatorcontrib>Yang, Heng</creatorcontrib><creatorcontrib>Guan, Shangyi</creatorcontrib><creatorcontrib>Shi, Wei</creatorcontrib><creatorcontrib>Chen, Yulin</creatorcontrib><creatorcontrib>Huang, Chenting</creatorcontrib><creatorcontrib>Xing, Jie</creatorcontrib><creatorcontrib>Liu, Hong</creatorcontrib><creatorcontrib>Chen, Qiang</creatorcontrib><collection>Ceramic Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Journal of the American Ceramic Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Feifei</au><au>Xu, Yugen</au><au>Yang, Heng</au><au>Guan, Shangyi</au><au>Shi, Wei</au><au>Chen, Yulin</au><au>Huang, Chenting</au><au>Xing, Jie</au><au>Liu, Hong</au><au>Chen, Qiang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of cerium on structures and electrical properties of (Nb, Ta) modified Bi4Ti3O12 piezoelectric ceramics</atitle><jtitle>Journal of the American Ceramic Society</jtitle><date>2022-06</date><risdate>2022</risdate><volume>105</volume><issue>6</issue><spage>4161</spage><epage>4170</epage><pages>4161-4170</pages><issn>0002-7820</issn><eissn>1551-2916</eissn><abstract>Bi4Ti3O12 high‐temperature piezoelectric ceramics composed of 0.03 mol (Nb, Ta)5+ substituting B site and x mol CeO2 (x = 0–0.05, abbreviated as BCTNT100x) substituting A site were synthesized by the conventional solid‐state reaction method. The effects of Ce additive on the structures and electrical properties of resulting Bi4Ti3O12‐based ceramics were systematically investigated. In‐situ temperature‐dependent X‐ray diffraction (XRD) confirmed that the phase structure of BCTNT100x ceramics change from orthorhombic structure to tetragonal structure as temperature increased. The ceramics at Ce content x = 0.03 illustrated optimal performances with superior piezoelectric constant (d33 = 36.5 pC/N), high Curie temperature (TC = 649 °C), and large remanent polarization (2Pr = 21.6 μC/cm2). BCTNT3 ceramics also possessed high d33 of 32.5 pC/N at an annealing temperature of 600°C, with electrical resistivity preserved at 106 Ω cm at 500 °C. These results demonstrate that BCTNT100x ceramics can be used as high‐temperature piezoelectric devices.</abstract><cop>Columbus</cop><pub>Wiley Subscription Services, Inc</pub><doi>10.1111/jace.18393</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0003-2260-246X</orcidid><orcidid>https://orcid.org/0000-0001-6805-4185</orcidid><orcidid>https://orcid.org/0000-0001-8187-4583</orcidid><orcidid>https://orcid.org/0000-0003-2800-5519</orcidid></addata></record> |
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| subjects | Bi4Ti3O12 Bismuth titanate Cerium oxides Curie temperature Electrical properties high curie temperature Niobium Piezoelectric ceramics Solid phases Tantalum Temperature dependence |
| title | Effects of cerium on structures and electrical properties of (Nb, Ta) modified Bi4Ti3O12 piezoelectric ceramics |
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