Assessment of Natural Radionuclide Distribution Pattern and Radiological Risk from Rocks in Precambrian Oban Massif, Southeastern Nigeria
A gamma spectrometric analysis of rock samples collected from the Precambrian Oban Massif, southeastern Nigeria, was performed to determine some primordial radioelements’ activity concentrations: U-238, Th-232, and K-40, and their associated radiological hazards. The mean activity of the primordial...
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creator | E. Ekpe, Ekpenyong Ben, Ubong C. Ekwok, Stephen E. Ebong, Ebong D. Akpan, Anthony E. Eldosouky, Ahmed M. Abdelrahman, Kamal Gómez-Ortiz, David |
description | A gamma spectrometric analysis of rock samples collected from the Precambrian Oban Massif, southeastern Nigeria, was performed to determine some primordial radioelements’ activity concentrations: U-238, Th-232, and K-40, and their associated radiological hazards. The mean activity of the primordial radionuclides was determined to be 1073.06 ± 0.65, 160.74 ± 1.32, and 250.76 ± 0.91 Bq·kg−1 for 40K, 238U, and 232Th, respectively, showing that they are inhomogeneously distributed, with activity changing with the rock type and location. The activity concentrations are highest in biotite garnet schist, quartz diorite, and biotite gneiss rock domains. The mean values of the radiological hazards are 0.08 Bq·kg−1 (alpha index), 2.15 Bq·kg−1(gamma index), 2.06 Bq·kg−1(internal) and 1.63 Bq·kg−1 (external4.30 Bq·kg−1(representative level index6), 602.23 Bq·kg−1, (radium equivalent), 780 nGy·h−1 (total absorbed dose rate), 270.91 nGy·h−1 (indoor), 509.78 nGy·h−1 (outdoor), 624.99, 1329.07 and 1954.06 mSv·yr−1 (outdoor, indoor and total annual effective dose equivalent, respectively), 6448.40 (cumulative excess lifetime cancer risk) and 248.94–3761.47 Bq·kg−1 (annual gonadal dose equivalent). These results are higher than their various permissible limits (except at Ako Community) and suggest that rocks in the area may be unsuitable for constructing dwelling places. It is strongly advised that basic safety standards and precautionary measures recommended by the European Commission should be strictly adhered to while dealing with these rocks. |
doi_str_mv | 10.3390/min12030312 |
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Ekpe, Ekpenyong ; Ben, Ubong C. ; Ekwok, Stephen E. ; Ebong, Ebong D. ; Akpan, Anthony E. ; Eldosouky, Ahmed M. ; Abdelrahman, Kamal ; Gómez-Ortiz, David</creator><creatorcontrib>E. Ekpe, Ekpenyong ; Ben, Ubong C. ; Ekwok, Stephen E. ; Ebong, Ebong D. ; Akpan, Anthony E. ; Eldosouky, Ahmed M. ; Abdelrahman, Kamal ; Gómez-Ortiz, David</creatorcontrib><description>A gamma spectrometric analysis of rock samples collected from the Precambrian Oban Massif, southeastern Nigeria, was performed to determine some primordial radioelements’ activity concentrations: U-238, Th-232, and K-40, and their associated radiological hazards. The mean activity of the primordial radionuclides was determined to be 1073.06 ± 0.65, 160.74 ± 1.32, and 250.76 ± 0.91 Bq·kg−1 for 40K, 238U, and 232Th, respectively, showing that they are inhomogeneously distributed, with activity changing with the rock type and location. The activity concentrations are highest in biotite garnet schist, quartz diorite, and biotite gneiss rock domains. The mean values of the radiological hazards are 0.08 Bq·kg−1 (alpha index), 2.15 Bq·kg−1(gamma index), 2.06 Bq·kg−1(internal) and 1.63 Bq·kg−1 (external4.30 Bq·kg−1(representative level index6), 602.23 Bq·kg−1, (radium equivalent), 780 nGy·h−1 (total absorbed dose rate), 270.91 nGy·h−1 (indoor), 509.78 nGy·h−1 (outdoor), 624.99, 1329.07 and 1954.06 mSv·yr−1 (outdoor, indoor and total annual effective dose equivalent, respectively), 6448.40 (cumulative excess lifetime cancer risk) and 248.94–3761.47 Bq·kg−1 (annual gonadal dose equivalent). These results are higher than their various permissible limits (except at Ako Community) and suggest that rocks in the area may be unsuitable for constructing dwelling places. It is strongly advised that basic safety standards and precautionary measures recommended by the European Commission should be strictly adhered to while dealing with these rocks.</description><identifier>ISSN: 2075-163X</identifier><identifier>EISSN: 2075-163X</identifier><identifier>DOI: 10.3390/min12030312</identifier><language>eng</language><publisher>Basel: MDPI AG</publisher><subject>Aggregates ; Biotite ; Civil engineering ; Composite materials ; Construction ; Diorite ; Dosage ; Equivalence ; Gamma rays ; Garnet ; Geology ; Gneiss ; Hazards ; Health risks ; Massifs ; Potassium ; Precambrian ; Radiation ; Radioisotopes ; Radionuclide kinetics ; Radium ; Rock ; Rocks ; Schist ; Schists ; Sediment samples ; Spectrometry</subject><ispartof>Minerals (Basel), 2022-03, Vol.12 (3), p.312</ispartof><rights>2022 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c298t-f19788d8fed7c25aafc0323d721d0940f6e0cc9c0fcee52f98580195904607623</citedby><cites>FETCH-LOGICAL-c298t-f19788d8fed7c25aafc0323d721d0940f6e0cc9c0fcee52f98580195904607623</cites><orcidid>0000-0003-1928-9775 ; 0000-0002-5744-3887 ; 0000-0003-2528-310X ; 0000-0002-9473-6769</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>E. Ekpe, Ekpenyong</creatorcontrib><creatorcontrib>Ben, Ubong C.</creatorcontrib><creatorcontrib>Ekwok, Stephen E.</creatorcontrib><creatorcontrib>Ebong, Ebong D.</creatorcontrib><creatorcontrib>Akpan, Anthony E.</creatorcontrib><creatorcontrib>Eldosouky, Ahmed M.</creatorcontrib><creatorcontrib>Abdelrahman, Kamal</creatorcontrib><creatorcontrib>Gómez-Ortiz, David</creatorcontrib><title>Assessment of Natural Radionuclide Distribution Pattern and Radiological Risk from Rocks in Precambrian Oban Massif, Southeastern Nigeria</title><title>Minerals (Basel)</title><description>A gamma spectrometric analysis of rock samples collected from the Precambrian Oban Massif, southeastern Nigeria, was performed to determine some primordial radioelements’ activity concentrations: U-238, Th-232, and K-40, and their associated radiological hazards. The mean activity of the primordial radionuclides was determined to be 1073.06 ± 0.65, 160.74 ± 1.32, and 250.76 ± 0.91 Bq·kg−1 for 40K, 238U, and 232Th, respectively, showing that they are inhomogeneously distributed, with activity changing with the rock type and location. The activity concentrations are highest in biotite garnet schist, quartz diorite, and biotite gneiss rock domains. The mean values of the radiological hazards are 0.08 Bq·kg−1 (alpha index), 2.15 Bq·kg−1(gamma index), 2.06 Bq·kg−1(internal) and 1.63 Bq·kg−1 (external4.30 Bq·kg−1(representative level index6), 602.23 Bq·kg−1, (radium equivalent), 780 nGy·h−1 (total absorbed dose rate), 270.91 nGy·h−1 (indoor), 509.78 nGy·h−1 (outdoor), 624.99, 1329.07 and 1954.06 mSv·yr−1 (outdoor, indoor and total annual effective dose equivalent, respectively), 6448.40 (cumulative excess lifetime cancer risk) and 248.94–3761.47 Bq·kg−1 (annual gonadal dose equivalent). These results are higher than their various permissible limits (except at Ako Community) and suggest that rocks in the area may be unsuitable for constructing dwelling places. It is strongly advised that basic safety standards and precautionary measures recommended by the European Commission should be strictly adhered to while dealing with these rocks.</description><subject>Aggregates</subject><subject>Biotite</subject><subject>Civil engineering</subject><subject>Composite materials</subject><subject>Construction</subject><subject>Diorite</subject><subject>Dosage</subject><subject>Equivalence</subject><subject>Gamma rays</subject><subject>Garnet</subject><subject>Geology</subject><subject>Gneiss</subject><subject>Hazards</subject><subject>Health risks</subject><subject>Massifs</subject><subject>Potassium</subject><subject>Precambrian</subject><subject>Radiation</subject><subject>Radioisotopes</subject><subject>Radionuclide kinetics</subject><subject>Radium</subject><subject>Rock</subject><subject>Rocks</subject><subject>Schist</subject><subject>Schists</subject><subject>Sediment samples</subject><subject>Spectrometry</subject><issn>2075-163X</issn><issn>2075-163X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNpNkMtOwzAQRS0EElXpih-wxBICfuRhL6vylEqLCkjsItexi9skLh5nwSfw16SURWcxczU6c0e6CJ1Tcs25JDeNaykjnHDKjtCAkSJLaM4_jg_0KRoBrElfknKRsQH6GQMYgMa0EXuLZyp2QdV4oSrn207XrjL41kEMbtnFfoVfVIwmtFi11Z6q_crp3YmDDbbBN3jh9Qaw69lgtGqWwakWz5d9e1YAzl7hV9_FT6Pgz2nmVqZHztCJVTWY0f8covf7u7fJYzKdPzxNxtNEMyliYqkshKiENVWhWaaU1YQzXhWMVkSmxOaGaC01sdqYjFkpMkGozCRJc1LkjA_Rxd53G_xXZyCWa9-Ftn9ZsjxlKRcypT11uad08ADB2HIbXKPCd0lJuYu7PIib_wJS53Q1</recordid><startdate>20220301</startdate><enddate>20220301</enddate><creator>E. 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Ekpe, Ekpenyong</au><au>Ben, Ubong C.</au><au>Ekwok, Stephen E.</au><au>Ebong, Ebong D.</au><au>Akpan, Anthony E.</au><au>Eldosouky, Ahmed M.</au><au>Abdelrahman, Kamal</au><au>Gómez-Ortiz, David</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Assessment of Natural Radionuclide Distribution Pattern and Radiological Risk from Rocks in Precambrian Oban Massif, Southeastern Nigeria</atitle><jtitle>Minerals (Basel)</jtitle><date>2022-03-01</date><risdate>2022</risdate><volume>12</volume><issue>3</issue><spage>312</spage><pages>312-</pages><issn>2075-163X</issn><eissn>2075-163X</eissn><abstract>A gamma spectrometric analysis of rock samples collected from the Precambrian Oban Massif, southeastern Nigeria, was performed to determine some primordial radioelements’ activity concentrations: U-238, Th-232, and K-40, and their associated radiological hazards. The mean activity of the primordial radionuclides was determined to be 1073.06 ± 0.65, 160.74 ± 1.32, and 250.76 ± 0.91 Bq·kg−1 for 40K, 238U, and 232Th, respectively, showing that they are inhomogeneously distributed, with activity changing with the rock type and location. The activity concentrations are highest in biotite garnet schist, quartz diorite, and biotite gneiss rock domains. The mean values of the radiological hazards are 0.08 Bq·kg−1 (alpha index), 2.15 Bq·kg−1(gamma index), 2.06 Bq·kg−1(internal) and 1.63 Bq·kg−1 (external4.30 Bq·kg−1(representative level index6), 602.23 Bq·kg−1, (radium equivalent), 780 nGy·h−1 (total absorbed dose rate), 270.91 nGy·h−1 (indoor), 509.78 nGy·h−1 (outdoor), 624.99, 1329.07 and 1954.06 mSv·yr−1 (outdoor, indoor and total annual effective dose equivalent, respectively), 6448.40 (cumulative excess lifetime cancer risk) and 248.94–3761.47 Bq·kg−1 (annual gonadal dose equivalent). These results are higher than their various permissible limits (except at Ako Community) and suggest that rocks in the area may be unsuitable for constructing dwelling places. It is strongly advised that basic safety standards and precautionary measures recommended by the European Commission should be strictly adhered to while dealing with these rocks.</abstract><cop>Basel</cop><pub>MDPI AG</pub><doi>10.3390/min12030312</doi><orcidid>https://orcid.org/0000-0003-1928-9775</orcidid><orcidid>https://orcid.org/0000-0002-5744-3887</orcidid><orcidid>https://orcid.org/0000-0003-2528-310X</orcidid><orcidid>https://orcid.org/0000-0002-9473-6769</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | Aggregates Biotite Civil engineering Composite materials Construction Diorite Dosage Equivalence Gamma rays Garnet Geology Gneiss Hazards Health risks Massifs Potassium Precambrian Radiation Radioisotopes Radionuclide kinetics Radium Rock Rocks Schist Schists Sediment samples Spectrometry |
title | Assessment of Natural Radionuclide Distribution Pattern and Radiological Risk from Rocks in Precambrian Oban Massif, Southeastern Nigeria |
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