Tunable band gap and transition between antiferromagnetism and ferromagnetism by surface adsorption in single-layer FePS3
The electronic and magnetic characteristics of two-dimensional materials have been the focus of attention in order to a wider range of spintronic applications. By using first-principles calculations, H atomic adsorption converts single-layer FePS 3 from semiconductor to half-metal while Li makes it...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2022-02, Vol.33 (4), p.1871-1876 |
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| container_issue | 4 |
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| container_title | Journal of materials science. Materials in electronics |
| container_volume | 33 |
| creator | Wu, Xiaoping Shen, Zhong Xiao, Wen Yang, Jiaquan Song, Changsheng |
| description | The electronic and magnetic characteristics of two-dimensional materials have been the focus of attention in order to a wider range of spintronic applications. By using first-principles calculations, H atomic adsorption converts single-layer FePS
3
from semiconductor to half-metal while Li makes it to metal. We also find that the magnetic ground state of intrinsic FePS
3
can be converted from antiferromagnetic to ferromagnetic by adsorbing H atoms, while alkali-metal atoms have no effect on it. Furthermore, the magnetic ground state is found sensitive to the numbers of H adatom on the surface of FePS
3
and demonstrates a vibration behavior. The present findings regarding a surface-adsorption-tuned bandgap and magnetism controlled by the adsorption concentration in a two-dimensional van der Waals magnets could lead to potential applications in next-generation magnetic memory storage, sensors and spintronic. |
| doi_str_mv | 10.1007/s10854-021-07386-0 |
| format | Article |
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3
from semiconductor to half-metal while Li makes it to metal. We also find that the magnetic ground state of intrinsic FePS
3
can be converted from antiferromagnetic to ferromagnetic by adsorbing H atoms, while alkali-metal atoms have no effect on it. Furthermore, the magnetic ground state is found sensitive to the numbers of H adatom on the surface of FePS
3
and demonstrates a vibration behavior. The present findings regarding a surface-adsorption-tuned bandgap and magnetism controlled by the adsorption concentration in a two-dimensional van der Waals magnets could lead to potential applications in next-generation magnetic memory storage, sensors and spintronic.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-021-07386-0</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Adatoms ; Adsorption ; Antiferromagnetism ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Energy gap ; Ferromagnetism ; First principles ; Ground state ; Magnetic properties ; Magnets ; Materials Science ; Optical and Electronic Materials ; Surface chemistry ; Two dimensional materials</subject><ispartof>Journal of materials science. Materials in electronics, 2022-02, Vol.33 (4), p.1871-1876</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-49ab0d5e9a51adcf751e8a8381b727c4ed7f71a8d310682e8bcb8f007709f4773</citedby><cites>FETCH-LOGICAL-c319t-49ab0d5e9a51adcf751e8a8381b727c4ed7f71a8d310682e8bcb8f007709f4773</cites><orcidid>0000-0001-7163-5765</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-021-07386-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-021-07386-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Wu, Xiaoping</creatorcontrib><creatorcontrib>Shen, Zhong</creatorcontrib><creatorcontrib>Xiao, Wen</creatorcontrib><creatorcontrib>Yang, Jiaquan</creatorcontrib><creatorcontrib>Song, Changsheng</creatorcontrib><title>Tunable band gap and transition between antiferromagnetism and ferromagnetism by surface adsorption in single-layer FePS3</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>The electronic and magnetic characteristics of two-dimensional materials have been the focus of attention in order to a wider range of spintronic applications. By using first-principles calculations, H atomic adsorption converts single-layer FePS
3
from semiconductor to half-metal while Li makes it to metal. We also find that the magnetic ground state of intrinsic FePS
3
can be converted from antiferromagnetic to ferromagnetic by adsorbing H atoms, while alkali-metal atoms have no effect on it. Furthermore, the magnetic ground state is found sensitive to the numbers of H adatom on the surface of FePS
3
and demonstrates a vibration behavior. The present findings regarding a surface-adsorption-tuned bandgap and magnetism controlled by the adsorption concentration in a two-dimensional van der Waals magnets could lead to potential applications in next-generation magnetic memory storage, sensors and spintronic.</description><subject>Adatoms</subject><subject>Adsorption</subject><subject>Antiferromagnetism</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Energy gap</subject><subject>Ferromagnetism</subject><subject>First principles</subject><subject>Ground state</subject><subject>Magnetic properties</subject><subject>Magnets</subject><subject>Materials Science</subject><subject>Optical and Electronic Materials</subject><subject>Surface chemistry</subject><subject>Two dimensional materials</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kE1LxDAURYMoOI7-AVcB19F8tUmXMjgqDCg4gruQtK-lQyetSYv039uZCoILVw8u594HB6FrRm8ZpeouMqoTSShnhCqhU0JP0IIlShCp-ccpWtAsUUQmnJ-jixh3lNJUCr1A43bw1jWAnfUFrmyHD7cP1se6r1uPHfRfAH6K-7qEENq9rTz0ddwfyT-RG3EcQmlzwLaIbeiOG7XHsfZVA6SxIwS8htc3cYnOSttEuPq5S_S-ftiunsjm5fF5db8huWBZT2RmHS0SyGzCbJGXKmGgrRaaOcVVLqFQpWJWF4LRVHPQLne6nJwompVSKbFEN_NuF9rPAWJvdu0Q_PTS8JRrziRjbKL4TOWhjTFAabpQ720YDaPmoNjMis2k2BwVGzqVxFyKE-wrCL_T_7S-AfCBgNQ</recordid><startdate>20220201</startdate><enddate>20220201</enddate><creator>Wu, Xiaoping</creator><creator>Shen, Zhong</creator><creator>Xiao, Wen</creator><creator>Yang, Jiaquan</creator><creator>Song, Changsheng</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0001-7163-5765</orcidid></search><sort><creationdate>20220201</creationdate><title>Tunable band gap and transition between antiferromagnetism and ferromagnetism by surface adsorption in single-layer FePS3</title><author>Wu, Xiaoping ; Shen, Zhong ; Xiao, Wen ; Yang, Jiaquan ; Song, Changsheng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-49ab0d5e9a51adcf751e8a8381b727c4ed7f71a8d310682e8bcb8f007709f4773</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Adatoms</topic><topic>Adsorption</topic><topic>Antiferromagnetism</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Energy gap</topic><topic>Ferromagnetism</topic><topic>First principles</topic><topic>Ground state</topic><topic>Magnetic properties</topic><topic>Magnets</topic><topic>Materials Science</topic><topic>Optical and Electronic Materials</topic><topic>Surface chemistry</topic><topic>Two dimensional materials</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wu, Xiaoping</creatorcontrib><creatorcontrib>Shen, Zhong</creatorcontrib><creatorcontrib>Xiao, Wen</creatorcontrib><creatorcontrib>Yang, Jiaquan</creatorcontrib><creatorcontrib>Song, Changsheng</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wu, Xiaoping</au><au>Shen, Zhong</au><au>Xiao, Wen</au><au>Yang, Jiaquan</au><au>Song, Changsheng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Tunable band gap and transition between antiferromagnetism and ferromagnetism by surface adsorption in single-layer FePS3</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2022-02-01</date><risdate>2022</risdate><volume>33</volume><issue>4</issue><spage>1871</spage><epage>1876</epage><pages>1871-1876</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>The electronic and magnetic characteristics of two-dimensional materials have been the focus of attention in order to a wider range of spintronic applications. By using first-principles calculations, H atomic adsorption converts single-layer FePS
3
from semiconductor to half-metal while Li makes it to metal. We also find that the magnetic ground state of intrinsic FePS
3
can be converted from antiferromagnetic to ferromagnetic by adsorbing H atoms, while alkali-metal atoms have no effect on it. Furthermore, the magnetic ground state is found sensitive to the numbers of H adatom on the surface of FePS
3
and demonstrates a vibration behavior. The present findings regarding a surface-adsorption-tuned bandgap and magnetism controlled by the adsorption concentration in a two-dimensional van der Waals magnets could lead to potential applications in next-generation magnetic memory storage, sensors and spintronic.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-021-07386-0</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0001-7163-5765</orcidid></addata></record> |
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| ispartof | Journal of materials science. Materials in electronics, 2022-02, Vol.33 (4), p.1871-1876 |
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| subjects | Adatoms Adsorption Antiferromagnetism Characterization and Evaluation of Materials Chemistry and Materials Science Energy gap Ferromagnetism First principles Ground state Magnetic properties Magnets Materials Science Optical and Electronic Materials Surface chemistry Two dimensional materials |
| title | Tunable band gap and transition between antiferromagnetism and ferromagnetism by surface adsorption in single-layer FePS3 |
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