Enhanced dielectric performance of polydimethylsiloxane‐based ternary composites films via tailored hydrogen bonds between carbon nanotube and barium titanate as modified fillers
A series of BT–cCNT/PDMS and BT–aCNT/PDMS composites were developed by incorporating barium titanate (BT) nanoparticles together with carboxylic functionalized multiwalled carbon nanotubes (cCNT) and amino functionalization multiwalled carbon nanotubes (aCNT) in polydimethylsiloxane (PDMS). Benefitt...
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| Veröffentlicht in: | Journal of vinyl & additive technology 2022-02, Vol.28 (1), p.184-195 |
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| container_title | Journal of vinyl & additive technology |
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| creator | Tang, Yaokai Liu, Hongfu Wang, Xincheng Cheng, Shangru Gao, Qiangmin Liu, Jiwen Guan, Shanshan Zhao, Shugao |
| description | A series of BT–cCNT/PDMS and BT–aCNT/PDMS composites were developed by incorporating barium titanate (BT) nanoparticles together with carboxylic functionalized multiwalled carbon nanotubes (cCNT) and amino functionalization multiwalled carbon nanotubes (aCNT) in polydimethylsiloxane (PDMS). Benefitting from the abundant active groups, CNTs and BTs can be in situ “bridged” by hydrogen bond in all of the BT–cCNT/PDMS and BT–aCNT/PDMS composites. Here, we studied the effect of hydrogen bonds (type and amount) between BTs and CNTs at the interface and dielectric properties of the composites. The results indicated that the BT–cCNT/PDMS composite exhibited higher dielectric constant and comparable dielectric loss than the BT–aCNT/PDMS composite, especially when weightCNT |
| doi_str_mv | 10.1002/vnl.21879 |
| format | Article |
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Benefitting from the abundant active groups, CNTs and BTs can be in situ “bridged” by hydrogen bond in all of the BT–cCNT/PDMS and BT–aCNT/PDMS composites. Here, we studied the effect of hydrogen bonds (type and amount) between BTs and CNTs at the interface and dielectric properties of the composites. The results indicated that the BT–cCNT/PDMS composite exhibited higher dielectric constant and comparable dielectric loss than the BT–aCNT/PDMS composite, especially when weightCNT < 1 wt%. Also, the dielectric properties of BT–cCNT/PDMS composite show stronger temperature dependence than BT–aCNT/PDMS composite. Finally, the tailorable performance of the polymer‐based dielectric composites can be obtained by regulating the interface with the help of hydrogen bonds.</description><identifier>ISSN: 1083-5601</identifier><identifier>EISSN: 1548-0585</identifier><identifier>DOI: 10.1002/vnl.21879</identifier><language>eng</language><publisher>Hoboken, USA: John Wiley & Sons, Inc</publisher><subject>barium titanate ; Barium titanates ; Bonding ; Carbon ; carbon nanotube ; Dielectric loss ; dielectric performance ; Dielectric properties ; Dielectric strength ; hydrogen bonding ; Hydrogen bonds ; Multi wall carbon nanotubes ; Nanoparticles ; Polydimethylsiloxane ; Polymer matrix composites ; Temperature dependence</subject><ispartof>Journal of vinyl & additive technology, 2022-02, Vol.28 (1), p.184-195</ispartof><rights>2021 Society of Plastics Engineers.</rights><rights>2022 Society of Plastics Engineers</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c2979-37cd3189a7d74d2cdb81b127013681076182c0dda87b5d49970f3377c9651a463</citedby><cites>FETCH-LOGICAL-c2979-37cd3189a7d74d2cdb81b127013681076182c0dda87b5d49970f3377c9651a463</cites><orcidid>0000-0003-3499-8713 ; 0000-0003-2477-9920</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fvnl.21879$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fvnl.21879$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,780,784,1417,27924,27925,45574,45575</link.rule.ids></links><search><creatorcontrib>Tang, Yaokai</creatorcontrib><creatorcontrib>Liu, Hongfu</creatorcontrib><creatorcontrib>Wang, Xincheng</creatorcontrib><creatorcontrib>Cheng, Shangru</creatorcontrib><creatorcontrib>Gao, Qiangmin</creatorcontrib><creatorcontrib>Liu, Jiwen</creatorcontrib><creatorcontrib>Guan, Shanshan</creatorcontrib><creatorcontrib>Zhao, Shugao</creatorcontrib><title>Enhanced dielectric performance of polydimethylsiloxane‐based ternary composites films via tailored hydrogen bonds between carbon nanotube and barium titanate as modified fillers</title><title>Journal of vinyl & additive technology</title><description>A series of BT–cCNT/PDMS and BT–aCNT/PDMS composites were developed by incorporating barium titanate (BT) nanoparticles together with carboxylic functionalized multiwalled carbon nanotubes (cCNT) and amino functionalization multiwalled carbon nanotubes (aCNT) in polydimethylsiloxane (PDMS). Benefitting from the abundant active groups, CNTs and BTs can be in situ “bridged” by hydrogen bond in all of the BT–cCNT/PDMS and BT–aCNT/PDMS composites. Here, we studied the effect of hydrogen bonds (type and amount) between BTs and CNTs at the interface and dielectric properties of the composites. The results indicated that the BT–cCNT/PDMS composite exhibited higher dielectric constant and comparable dielectric loss than the BT–aCNT/PDMS composite, especially when weightCNT < 1 wt%. Also, the dielectric properties of BT–cCNT/PDMS composite show stronger temperature dependence than BT–aCNT/PDMS composite. Finally, the tailorable performance of the polymer‐based dielectric composites can be obtained by regulating the interface with the help of hydrogen bonds.</description><subject>barium titanate</subject><subject>Barium titanates</subject><subject>Bonding</subject><subject>Carbon</subject><subject>carbon nanotube</subject><subject>Dielectric loss</subject><subject>dielectric performance</subject><subject>Dielectric properties</subject><subject>Dielectric strength</subject><subject>hydrogen bonding</subject><subject>Hydrogen bonds</subject><subject>Multi wall carbon nanotubes</subject><subject>Nanoparticles</subject><subject>Polydimethylsiloxane</subject><subject>Polymer matrix composites</subject><subject>Temperature dependence</subject><issn>1083-5601</issn><issn>1548-0585</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNp1kc1OAyEUhSdGE2t14RuQuHIxCvMHszRN_Uka3ajbCQN3LA0DI9Dq7HwEH8Yn8kmk1q0JCdyT75zkcpLklOALgnF2uTH6IiOM1nvJhJQFS3HJyv34xixPywqTw-TI-xXGW72YJF9zs-RGgERSgQYRnBJoANdZ1291ZDs0WD1K1UNYjtorbd-5ge-Pz5b7aAvgDHcjErYfrFcBPOqU7j3aKI4Cj7iL1HKUzr6AQa010qMWwhvESXAXBWS4sWHdAuJGopY7te5RUIEbHqLmUW-l6lSMickanD9ODjquPZz83dPk6Xr-OLtNFw83d7OrRSqymtZpToXMCas5lbSQmZAtIy3JKCZ5xQimFWGZwFJyRttSFnVNcZfnlIq6KgkvqnyanO1yB2df1-BDs7LruK72TVZlZbE9NFLnO0o4672Drhmc6uOfNAQ321KaWErzW0pkL3fsm9Iw_g82z_eLneMHmy6T0w</recordid><startdate>202202</startdate><enddate>202202</enddate><creator>Tang, Yaokai</creator><creator>Liu, Hongfu</creator><creator>Wang, Xincheng</creator><creator>Cheng, Shangru</creator><creator>Gao, Qiangmin</creator><creator>Liu, Jiwen</creator><creator>Guan, Shanshan</creator><creator>Zhao, Shugao</creator><general>John Wiley & Sons, Inc</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>FR3</scope><scope>JG9</scope><scope>KR7</scope><scope>U9A</scope><orcidid>https://orcid.org/0000-0003-3499-8713</orcidid><orcidid>https://orcid.org/0000-0003-2477-9920</orcidid></search><sort><creationdate>202202</creationdate><title>Enhanced dielectric performance of polydimethylsiloxane‐based ternary composites films via tailored hydrogen bonds between carbon nanotube and barium titanate as modified fillers</title><author>Tang, Yaokai ; Liu, Hongfu ; Wang, Xincheng ; Cheng, Shangru ; Gao, Qiangmin ; Liu, Jiwen ; Guan, Shanshan ; Zhao, Shugao</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c2979-37cd3189a7d74d2cdb81b127013681076182c0dda87b5d49970f3377c9651a463</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>barium titanate</topic><topic>Barium titanates</topic><topic>Bonding</topic><topic>Carbon</topic><topic>carbon nanotube</topic><topic>Dielectric loss</topic><topic>dielectric performance</topic><topic>Dielectric properties</topic><topic>Dielectric strength</topic><topic>hydrogen bonding</topic><topic>Hydrogen bonds</topic><topic>Multi wall carbon nanotubes</topic><topic>Nanoparticles</topic><topic>Polydimethylsiloxane</topic><topic>Polymer matrix composites</topic><topic>Temperature dependence</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Tang, Yaokai</creatorcontrib><creatorcontrib>Liu, Hongfu</creatorcontrib><creatorcontrib>Wang, Xincheng</creatorcontrib><creatorcontrib>Cheng, Shangru</creatorcontrib><creatorcontrib>Gao, Qiangmin</creatorcontrib><creatorcontrib>Liu, Jiwen</creatorcontrib><creatorcontrib>Guan, Shanshan</creatorcontrib><creatorcontrib>Zhao, Shugao</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><collection>Civil Engineering Abstracts</collection><jtitle>Journal of vinyl & additive technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tang, Yaokai</au><au>Liu, Hongfu</au><au>Wang, Xincheng</au><au>Cheng, Shangru</au><au>Gao, Qiangmin</au><au>Liu, Jiwen</au><au>Guan, Shanshan</au><au>Zhao, Shugao</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced dielectric performance of polydimethylsiloxane‐based ternary composites films via tailored hydrogen bonds between carbon nanotube and barium titanate as modified fillers</atitle><jtitle>Journal of vinyl & additive technology</jtitle><date>2022-02</date><risdate>2022</risdate><volume>28</volume><issue>1</issue><spage>184</spage><epage>195</epage><pages>184-195</pages><issn>1083-5601</issn><eissn>1548-0585</eissn><abstract>A series of BT–cCNT/PDMS and BT–aCNT/PDMS composites were developed by incorporating barium titanate (BT) nanoparticles together with carboxylic functionalized multiwalled carbon nanotubes (cCNT) and amino functionalization multiwalled carbon nanotubes (aCNT) in polydimethylsiloxane (PDMS). Benefitting from the abundant active groups, CNTs and BTs can be in situ “bridged” by hydrogen bond in all of the BT–cCNT/PDMS and BT–aCNT/PDMS composites. Here, we studied the effect of hydrogen bonds (type and amount) between BTs and CNTs at the interface and dielectric properties of the composites. The results indicated that the BT–cCNT/PDMS composite exhibited higher dielectric constant and comparable dielectric loss than the BT–aCNT/PDMS composite, especially when weightCNT < 1 wt%. Also, the dielectric properties of BT–cCNT/PDMS composite show stronger temperature dependence than BT–aCNT/PDMS composite. Finally, the tailorable performance of the polymer‐based dielectric composites can be obtained by regulating the interface with the help of hydrogen bonds.</abstract><cop>Hoboken, USA</cop><pub>John Wiley & Sons, Inc</pub><doi>10.1002/vnl.21879</doi><tpages>12</tpages><orcidid>https://orcid.org/0000-0003-3499-8713</orcidid><orcidid>https://orcid.org/0000-0003-2477-9920</orcidid></addata></record> |
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| subjects | barium titanate Barium titanates Bonding Carbon carbon nanotube Dielectric loss dielectric performance Dielectric properties Dielectric strength hydrogen bonding Hydrogen bonds Multi wall carbon nanotubes Nanoparticles Polydimethylsiloxane Polymer matrix composites Temperature dependence |
| title | Enhanced dielectric performance of polydimethylsiloxane‐based ternary composites films via tailored hydrogen bonds between carbon nanotube and barium titanate as modified fillers |
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