Au-Pd modified SnS2 nanosheets for conductometric detection of xylene gas

Two-dimensional metal sulfide semiconductor materials have received a lot of attention recently due to their large surface-to-volume ratio, outstanding chemical properties, and suitable band gap, and possess the potential in the application of gas sensors. In this work, SnS2 nanosheets were synthesi...

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Veröffentlicht in:Sensors and actuators. B, Chemical Chemical, 2022-01, Vol.351, p.130907, Article 130907
Hauptverfasser: Lu, Yang, Zhang, Jiafeng, Wang, Wei, Fan, Yizhuo, Liu, Caixia, Zhou, Jingran, Liu, Dali, Ruan, Shengping
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container_start_page 130907
container_title Sensors and actuators. B, Chemical
container_volume 351
creator Lu, Yang
Zhang, Jiafeng
Wang, Wei
Fan, Yizhuo
Liu, Caixia
Zhou, Jingran
Liu, Dali
Ruan, Shengping
description Two-dimensional metal sulfide semiconductor materials have received a lot of attention recently due to their large surface-to-volume ratio, outstanding chemical properties, and suitable band gap, and possess the potential in the application of gas sensors. In this work, SnS2 nanosheets were synthesized by a simple hydrothermal method and successfully modified with Au, Pd, and Au-Pd nanoparticles on their surfaces using reducing agents for xylene detection. The experimental results show that the gas-sensitive performance of the sensor can be significantly improved by modifying Au-Pd nanoparticles on the surface of SnS2 nanosheets, which can be attributed to the synergistic effect of the bimetal and the catalytic properties of bimetallic systems. The response of the prepared sensor is more than ten times higher than that of the pure material. In addition, the optimal operating temperature of the sensor modified by Au-Pd nanoparticles was also decreased compared to that of the sensor prepared by SnS2. The outstanding performance makes Au-Pd nanoparticles-modified SnS2 gas sensor a great potential candidate for xylene detection. •A facile method was used to obtain bimetallic-modified SnS2 semiconductor structures.•The AuPd-SnS2 gas sensor exhibited excellent xylene-sensitive properties.•The AuPd-SnS2 gas sensor showed significant selectivity for xylene and lower operating temperatures.•The discussion of the effect of the synergistic effect of Au-Pd nanoparticals on the sensing performance of xylene.
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In this work, SnS2 nanosheets were synthesized by a simple hydrothermal method and successfully modified with Au, Pd, and Au-Pd nanoparticles on their surfaces using reducing agents for xylene detection. The experimental results show that the gas-sensitive performance of the sensor can be significantly improved by modifying Au-Pd nanoparticles on the surface of SnS2 nanosheets, which can be attributed to the synergistic effect of the bimetal and the catalytic properties of bimetallic systems. The response of the prepared sensor is more than ten times higher than that of the pure material. In addition, the optimal operating temperature of the sensor modified by Au-Pd nanoparticles was also decreased compared to that of the sensor prepared by SnS2. The outstanding performance makes Au-Pd nanoparticles-modified SnS2 gas sensor a great potential candidate for xylene detection. •A facile method was used to obtain bimetallic-modified SnS2 semiconductor structures.•The AuPd-SnS2 gas sensor exhibited excellent xylene-sensitive properties.•The AuPd-SnS2 gas sensor showed significant selectivity for xylene and lower operating temperatures.•The discussion of the effect of the synergistic effect of Au-Pd nanoparticals on the sensing performance of xylene.</description><identifier>ISSN: 0925-4005</identifier><identifier>EISSN: 1873-3077</identifier><identifier>DOI: 10.1016/j.snb.2021.130907</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Bimetallic decoration ; Bimetals ; Chemical properties ; Gas sensors ; Gold ; Nanoparticles ; Nanosheets ; Operating temperature ; Palladium ; Reducing agents ; Semiconductor materials ; Sensors ; Synergistic effect ; Tin disulfide ; Two-dimensional materials ; Xylene ; Xylene gas sensor</subject><ispartof>Sensors and actuators. 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B, Chemical</title><description>Two-dimensional metal sulfide semiconductor materials have received a lot of attention recently due to their large surface-to-volume ratio, outstanding chemical properties, and suitable band gap, and possess the potential in the application of gas sensors. In this work, SnS2 nanosheets were synthesized by a simple hydrothermal method and successfully modified with Au, Pd, and Au-Pd nanoparticles on their surfaces using reducing agents for xylene detection. The experimental results show that the gas-sensitive performance of the sensor can be significantly improved by modifying Au-Pd nanoparticles on the surface of SnS2 nanosheets, which can be attributed to the synergistic effect of the bimetal and the catalytic properties of bimetallic systems. The response of the prepared sensor is more than ten times higher than that of the pure material. 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subjects Bimetallic decoration
Bimetals
Chemical properties
Gas sensors
Gold
Nanoparticles
Nanosheets
Operating temperature
Palladium
Reducing agents
Semiconductor materials
Sensors
Synergistic effect
Tin disulfide
Two-dimensional materials
Xylene
Xylene gas sensor
title Au-Pd modified SnS2 nanosheets for conductometric detection of xylene gas
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