Dual imaging of uranium ore by Laser Ablation Inductively Coupled Plasma Mass Spectrometry and Laser Induced Breakdown Spectroscopy
The great potential in combining two elemental imaging techniques - Laser Induced Breakdown Spectroscopy (LIBS) and Laser Ablation Inductively Coupled Plasma Mass Spectrometry (LA-ICP-MS) is demonstrated for uranium ore sample investigation. Dual imaging provides the advantages of both methods – hig...
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| Veröffentlicht in: | Spectrochimica acta. Part B: Atomic spectroscopy 2021-12, Vol.186, p.106312, Article 106312 |
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| container_title | Spectrochimica acta. Part B: Atomic spectroscopy |
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| creator | Holá, Markéta Novotný, Karel Dobeš, Jan Krempl, Ivo Wertich, Vojtěch Mozola, Juraj Kubeš, Martin Faltusová, Veronika Leichmann, Jaromír Kanický, Viktor |
| description | The great potential in combining two elemental imaging techniques - Laser Induced Breakdown Spectroscopy (LIBS) and Laser Ablation Inductively Coupled Plasma Mass Spectrometry (LA-ICP-MS) is demonstrated for uranium ore sample investigation. Dual imaging provides the advantages of both methods – high speed, large area imaging and additional evaluation of the whole spectrum for LIBS, and high resolution, low detection limits and isotopic imaging for LA-ICP-MS. Special software, ILAPS, was created for data processing to ensure the consistency of the resulting element images and the possibility of their combination. This new method for merging LIBS and LA-ICP-MS imaging data allows the display of detailed structures on the background of the overall sample image. Information contained in the detailed structures together with an overall view of the sample was displayed in one image to visualise the complete data from both methods. The effectiveness and usefulness of this new approach were demonstrated in identifying the structures responsible for elements migration in the uranium ore sample.
[Display omitted]
•Advanced combination of LIBS and LA-ICP-MS imaging of geological sample•Benefits of LIBS and ICP-MS imaging fully utilized without compromise•New approach for merging LIBS and LA-ICP-MS imaging data•Display of detailed structures on the background of the overall sample image |
| doi_str_mv | 10.1016/j.sab.2021.106312 |
| format | Article |
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[Display omitted]
•Advanced combination of LIBS and LA-ICP-MS imaging of geological sample•Benefits of LIBS and ICP-MS imaging fully utilized without compromise•New approach for merging LIBS and LA-ICP-MS imaging data•Display of detailed structures on the background of the overall sample image</description><identifier>ISSN: 0584-8547</identifier><identifier>EISSN: 1873-3565</identifier><identifier>DOI: 10.1016/j.sab.2021.106312</identifier><language>eng</language><publisher>Oxford: Elsevier B.V</publisher><subject>Ablation ; Analytical methods ; Data analysis ; Data processing ; Detection limits ; Elemental imaging ; Elemental mapping ; Emission spectroscopy ; Geological samples ; Imaging techniques ; Inductively coupled plasma mass spectrometry ; LA-ICP-MS ; Laser ablation ; Laser induced breakdown spectroscopy ; Lasers ; LIBS ; Mass spectrometry ; Mass spectroscopy ; Scientific imaging ; Spectroscopy ; Structures ; Uranium ; Uranium ore ; Uranium ores</subject><ispartof>Spectrochimica acta. Part B: Atomic spectroscopy, 2021-12, Vol.186, p.106312, Article 106312</ispartof><rights>2021 Elsevier B.V.</rights><rights>Copyright Elsevier BV Dec 2021</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c325t-a0de369eb33d3faf066ffb1f027e382d0b431648bba1c169119bd68f8367f9f43</citedby><cites>FETCH-LOGICAL-c325t-a0de369eb33d3faf066ffb1f027e382d0b431648bba1c169119bd68f8367f9f43</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S058485472100269X$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3536,27903,27904,65309</link.rule.ids></links><search><creatorcontrib>Holá, Markéta</creatorcontrib><creatorcontrib>Novotný, Karel</creatorcontrib><creatorcontrib>Dobeš, Jan</creatorcontrib><creatorcontrib>Krempl, Ivo</creatorcontrib><creatorcontrib>Wertich, Vojtěch</creatorcontrib><creatorcontrib>Mozola, Juraj</creatorcontrib><creatorcontrib>Kubeš, Martin</creatorcontrib><creatorcontrib>Faltusová, Veronika</creatorcontrib><creatorcontrib>Leichmann, Jaromír</creatorcontrib><creatorcontrib>Kanický, Viktor</creatorcontrib><title>Dual imaging of uranium ore by Laser Ablation Inductively Coupled Plasma Mass Spectrometry and Laser Induced Breakdown Spectroscopy</title><title>Spectrochimica acta. Part B: Atomic spectroscopy</title><description>The great potential in combining two elemental imaging techniques - Laser Induced Breakdown Spectroscopy (LIBS) and Laser Ablation Inductively Coupled Plasma Mass Spectrometry (LA-ICP-MS) is demonstrated for uranium ore sample investigation. Dual imaging provides the advantages of both methods – high speed, large area imaging and additional evaluation of the whole spectrum for LIBS, and high resolution, low detection limits and isotopic imaging for LA-ICP-MS. Special software, ILAPS, was created for data processing to ensure the consistency of the resulting element images and the possibility of their combination. This new method for merging LIBS and LA-ICP-MS imaging data allows the display of detailed structures on the background of the overall sample image. Information contained in the detailed structures together with an overall view of the sample was displayed in one image to visualise the complete data from both methods. The effectiveness and usefulness of this new approach were demonstrated in identifying the structures responsible for elements migration in the uranium ore sample.
[Display omitted]
•Advanced combination of LIBS and LA-ICP-MS imaging of geological sample•Benefits of LIBS and ICP-MS imaging fully utilized without compromise•New approach for merging LIBS and LA-ICP-MS imaging data•Display of detailed structures on the background of the overall sample image</description><subject>Ablation</subject><subject>Analytical methods</subject><subject>Data analysis</subject><subject>Data processing</subject><subject>Detection limits</subject><subject>Elemental imaging</subject><subject>Elemental mapping</subject><subject>Emission spectroscopy</subject><subject>Geological samples</subject><subject>Imaging techniques</subject><subject>Inductively coupled plasma mass spectrometry</subject><subject>LA-ICP-MS</subject><subject>Laser ablation</subject><subject>Laser induced breakdown spectroscopy</subject><subject>Lasers</subject><subject>LIBS</subject><subject>Mass spectrometry</subject><subject>Mass spectroscopy</subject><subject>Scientific imaging</subject><subject>Spectroscopy</subject><subject>Structures</subject><subject>Uranium</subject><subject>Uranium ore</subject><subject>Uranium ores</subject><issn>0584-8547</issn><issn>1873-3565</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNp9kLtOwzAUhi0EEqXwAGyWmFN8SdxETFBulYpAAmbLju3KIYmDnRRl5sVxaVmZjo70f-fyAXCO0QwjzC6rWRByRhDBsWcUkwMwwfmcJjRj2SGYoCxPkzxL58fgJIQKIUQykk3A9-0gamgbsbbtGjoDBy9aOzTQeQ3lCFciaA-vZS1661q4bNVQ9naj6xEu3NDVWsGXWoRGwCcRAnztdNl71-jej1C0as__YjF647X4UO6r_QuG0nXjKTgyog76bF-n4P3-7m3xmKyeH5aL61VSUpL1iUBKU1ZoSamiRhjEmDESG0TmmuZEIZlSzNJcSoFLzAqMC6lYbnLK5qYwKZ2Ci93czrvPQYeeV27wbVzJCcMFY0XOUEzhXaqM5wWvDe989ONHjhHfuuYVj6751jXfuY7M1Y7R8fyN1Z6H0uo2vmx9_JMrZ_-hfwBM9Yho</recordid><startdate>202112</startdate><enddate>202112</enddate><creator>Holá, Markéta</creator><creator>Novotný, Karel</creator><creator>Dobeš, Jan</creator><creator>Krempl, Ivo</creator><creator>Wertich, Vojtěch</creator><creator>Mozola, Juraj</creator><creator>Kubeš, Martin</creator><creator>Faltusová, Veronika</creator><creator>Leichmann, Jaromír</creator><creator>Kanický, Viktor</creator><general>Elsevier B.V</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7QH</scope><scope>7SR</scope><scope>7U5</scope><scope>7UA</scope><scope>8FD</scope><scope>C1K</scope><scope>F1W</scope><scope>H97</scope><scope>JG9</scope><scope>L.G</scope><scope>L7M</scope></search><sort><creationdate>202112</creationdate><title>Dual imaging of uranium ore by Laser Ablation Inductively Coupled Plasma Mass Spectrometry and Laser Induced Breakdown Spectroscopy</title><author>Holá, Markéta ; Novotný, Karel ; Dobeš, Jan ; Krempl, Ivo ; Wertich, Vojtěch ; Mozola, Juraj ; Kubeš, Martin ; Faltusová, Veronika ; Leichmann, Jaromír ; Kanický, Viktor</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c325t-a0de369eb33d3faf066ffb1f027e382d0b431648bba1c169119bd68f8367f9f43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Ablation</topic><topic>Analytical methods</topic><topic>Data analysis</topic><topic>Data processing</topic><topic>Detection limits</topic><topic>Elemental imaging</topic><topic>Elemental mapping</topic><topic>Emission spectroscopy</topic><topic>Geological samples</topic><topic>Imaging techniques</topic><topic>Inductively coupled plasma mass spectrometry</topic><topic>LA-ICP-MS</topic><topic>Laser ablation</topic><topic>Laser induced breakdown spectroscopy</topic><topic>Lasers</topic><topic>LIBS</topic><topic>Mass spectrometry</topic><topic>Mass spectroscopy</topic><topic>Scientific imaging</topic><topic>Spectroscopy</topic><topic>Structures</topic><topic>Uranium</topic><topic>Uranium ore</topic><topic>Uranium ores</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Holá, Markéta</creatorcontrib><creatorcontrib>Novotný, Karel</creatorcontrib><creatorcontrib>Dobeš, Jan</creatorcontrib><creatorcontrib>Krempl, Ivo</creatorcontrib><creatorcontrib>Wertich, Vojtěch</creatorcontrib><creatorcontrib>Mozola, Juraj</creatorcontrib><creatorcontrib>Kubeš, Martin</creatorcontrib><creatorcontrib>Faltusová, Veronika</creatorcontrib><creatorcontrib>Leichmann, Jaromír</creatorcontrib><creatorcontrib>Kanický, Viktor</creatorcontrib><collection>CrossRef</collection><collection>Aqualine</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Water Resources Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><collection>Materials Research Database</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Spectrochimica acta. Part B: Atomic spectroscopy</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Holá, Markéta</au><au>Novotný, Karel</au><au>Dobeš, Jan</au><au>Krempl, Ivo</au><au>Wertich, Vojtěch</au><au>Mozola, Juraj</au><au>Kubeš, Martin</au><au>Faltusová, Veronika</au><au>Leichmann, Jaromír</au><au>Kanický, Viktor</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Dual imaging of uranium ore by Laser Ablation Inductively Coupled Plasma Mass Spectrometry and Laser Induced Breakdown Spectroscopy</atitle><jtitle>Spectrochimica acta. Part B: Atomic spectroscopy</jtitle><date>2021-12</date><risdate>2021</risdate><volume>186</volume><spage>106312</spage><pages>106312-</pages><artnum>106312</artnum><issn>0584-8547</issn><eissn>1873-3565</eissn><abstract>The great potential in combining two elemental imaging techniques - Laser Induced Breakdown Spectroscopy (LIBS) and Laser Ablation Inductively Coupled Plasma Mass Spectrometry (LA-ICP-MS) is demonstrated for uranium ore sample investigation. Dual imaging provides the advantages of both methods – high speed, large area imaging and additional evaluation of the whole spectrum for LIBS, and high resolution, low detection limits and isotopic imaging for LA-ICP-MS. Special software, ILAPS, was created for data processing to ensure the consistency of the resulting element images and the possibility of their combination. This new method for merging LIBS and LA-ICP-MS imaging data allows the display of detailed structures on the background of the overall sample image. Information contained in the detailed structures together with an overall view of the sample was displayed in one image to visualise the complete data from both methods. The effectiveness and usefulness of this new approach were demonstrated in identifying the structures responsible for elements migration in the uranium ore sample.
[Display omitted]
•Advanced combination of LIBS and LA-ICP-MS imaging of geological sample•Benefits of LIBS and ICP-MS imaging fully utilized without compromise•New approach for merging LIBS and LA-ICP-MS imaging data•Display of detailed structures on the background of the overall sample image</abstract><cop>Oxford</cop><pub>Elsevier B.V</pub><doi>10.1016/j.sab.2021.106312</doi></addata></record> |
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| source | Elsevier ScienceDirect Journals Complete |
| subjects | Ablation Analytical methods Data analysis Data processing Detection limits Elemental imaging Elemental mapping Emission spectroscopy Geological samples Imaging techniques Inductively coupled plasma mass spectrometry LA-ICP-MS Laser ablation Laser induced breakdown spectroscopy Lasers LIBS Mass spectrometry Mass spectroscopy Scientific imaging Spectroscopy Structures Uranium Uranium ore Uranium ores |
| title | Dual imaging of uranium ore by Laser Ablation Inductively Coupled Plasma Mass Spectrometry and Laser Induced Breakdown Spectroscopy |
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