Egg White-Mediated Synthesis and Application of Ag/CeO2 Photocatalyst for Enhanced Photocatalytic Activity under Visible Light Irradiation
The Ag/CeO 2 composite photocatalysts have been successfully prepared using fresh egg white as a gelling agent at various calcination temperatures, respectively. It has been found that Ag doping reduces the band gap of the composite and improves its response to visible light. The photocatalytic perf...
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Veröffentlicht in: | Russian journal of inorganic chemistry 2021-12, Vol.66 (14), p.2036-2044 |
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container_title | Russian journal of inorganic chemistry |
container_volume | 66 |
creator | Zhang, Peng Liu, Bin Li, Yunfeng Chen, Ning Du, Yanping Chang, Wei Yang, Huixi Hong, Wanyu Li, Yidan Yang, Gaixia |
description | The Ag/CeO
2
composite photocatalysts have been successfully prepared using fresh egg white as a gelling agent at various calcination temperatures, respectively. It has been found that Ag doping reduces the band gap of the composite and improves its response to visible light. The photocatalytic performance of Ag/CeO
2
composite photocatalysts prepared at different calcination temperatures has been tested, and it has been found that the samples calcined at 600°C have excellent properties compared with pure CeO
2
. The degradation rate of the sample calcination at 600°C to methylene blue (MB) reached 94.9% under a 300 W Xenon lamp light irradiation for 60 min. In addition, the Ag/CeO
2
photocatalyst exhibits good photocatalytic stability and durability. Finally, the mechanism of photocatalytic degradation of MB is proposed in combination with the active substance capture test. The high photocatalytic activity of Ag/CeO
2
composite photocatalysts may be attributed to the doping of Ag, which inhibits the recombination of photogenerated electron-hole pairs. |
doi_str_mv | 10.1134/S0036023621140096 |
format | Article |
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2
composite photocatalysts have been successfully prepared using fresh egg white as a gelling agent at various calcination temperatures, respectively. It has been found that Ag doping reduces the band gap of the composite and improves its response to visible light. The photocatalytic performance of Ag/CeO
2
composite photocatalysts prepared at different calcination temperatures has been tested, and it has been found that the samples calcined at 600°C have excellent properties compared with pure CeO
2
. The degradation rate of the sample calcination at 600°C to methylene blue (MB) reached 94.9% under a 300 W Xenon lamp light irradiation for 60 min. In addition, the Ag/CeO
2
photocatalyst exhibits good photocatalytic stability and durability. Finally, the mechanism of photocatalytic degradation of MB is proposed in combination with the active substance capture test. The high photocatalytic activity of Ag/CeO
2
composite photocatalysts may be attributed to the doping of Ag, which inhibits the recombination of photogenerated electron-hole pairs.</description><identifier>ISSN: 0036-0236</identifier><identifier>EISSN: 1531-8613</identifier><identifier>DOI: 10.1134/S0036023621140096</identifier><language>eng</language><publisher>Moscow: Pleiades Publishing</publisher><subject>Albumen ; Catalytic activity ; Cerium oxides ; Chemistry ; Chemistry and Materials Science ; Doping ; Eggs ; Holes (electron deficiencies) ; Inorganic Chemistry ; Light irradiation ; Methylene blue ; Photocatalysis ; Photocatalysts ; Photodegradation ; Roasting ; Synthesis and Properties of Inorganic Compounds ; Xenon lamps</subject><ispartof>Russian journal of inorganic chemistry, 2021-12, Vol.66 (14), p.2036-2044</ispartof><rights>Pleiades Publishing, Ltd. 2021. ISSN 0036-0236, Russian Journal of Inorganic Chemistry, 2021, Vol. 66, No. 14, pp. 2036–2044. © Pleiades Publishing, Ltd., 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c316t-4e63a6711646750a2777db9ed01085b0b32515fb4d25a78f211f123987d114803</citedby><cites>FETCH-LOGICAL-c316t-4e63a6711646750a2777db9ed01085b0b32515fb4d25a78f211f123987d114803</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1134/S0036023621140096$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1134/S0036023621140096$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Zhang, Peng</creatorcontrib><creatorcontrib>Liu, Bin</creatorcontrib><creatorcontrib>Li, Yunfeng</creatorcontrib><creatorcontrib>Chen, Ning</creatorcontrib><creatorcontrib>Du, Yanping</creatorcontrib><creatorcontrib>Chang, Wei</creatorcontrib><creatorcontrib>Yang, Huixi</creatorcontrib><creatorcontrib>Hong, Wanyu</creatorcontrib><creatorcontrib>Li, Yidan</creatorcontrib><creatorcontrib>Yang, Gaixia</creatorcontrib><title>Egg White-Mediated Synthesis and Application of Ag/CeO2 Photocatalyst for Enhanced Photocatalytic Activity under Visible Light Irradiation</title><title>Russian journal of inorganic chemistry</title><addtitle>Russ. J. Inorg. Chem</addtitle><description>The Ag/CeO
2
composite photocatalysts have been successfully prepared using fresh egg white as a gelling agent at various calcination temperatures, respectively. It has been found that Ag doping reduces the band gap of the composite and improves its response to visible light. The photocatalytic performance of Ag/CeO
2
composite photocatalysts prepared at different calcination temperatures has been tested, and it has been found that the samples calcined at 600°C have excellent properties compared with pure CeO
2
. The degradation rate of the sample calcination at 600°C to methylene blue (MB) reached 94.9% under a 300 W Xenon lamp light irradiation for 60 min. In addition, the Ag/CeO
2
photocatalyst exhibits good photocatalytic stability and durability. Finally, the mechanism of photocatalytic degradation of MB is proposed in combination with the active substance capture test. The high photocatalytic activity of Ag/CeO
2
composite photocatalysts may be attributed to the doping of Ag, which inhibits the recombination of photogenerated electron-hole pairs.</description><subject>Albumen</subject><subject>Catalytic activity</subject><subject>Cerium oxides</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Doping</subject><subject>Eggs</subject><subject>Holes (electron deficiencies)</subject><subject>Inorganic Chemistry</subject><subject>Light irradiation</subject><subject>Methylene blue</subject><subject>Photocatalysis</subject><subject>Photocatalysts</subject><subject>Photodegradation</subject><subject>Roasting</subject><subject>Synthesis and Properties of Inorganic Compounds</subject><subject>Xenon lamps</subject><issn>0036-0236</issn><issn>1531-8613</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNp1kN1KwzAUx4MoOKcP4F3A67qcJE27yzKmDiYK8-OypG3aZtR0JpnQV_CpTZmgIF4dOP8v-CF0CeQagPHZhhAmCGWCAnBC5uIITSBmEKUC2DGajHI06qfozLktIZyTJJ2gz2XT4NdWexXdq0pLryq8GYxvldMOS1PhbLfrdCm97g3ua5w1s4V6oPix7X0f3rIbnMd1b_HStNKUIf9L8rrEWen1h_YD3ptKWfyinS46hde6aT1eWSvH2dB-jk5q2Tl18X2n6Plm-bS4i9YPt6tFto5KBsJHXAkmRQIguEhiImmSJFUxVxUBksYFKRiNIa4LXtFYJmkdgNRA2TxNqoAmJWyKrg69O9u_75Xz-bbfWxMmcyogDdB4DMEFB1dpe-esqvOd1W_SDjmQfESe_0EeMvSQccFrGmV_mv8PfQFYAoI_</recordid><startdate>20211201</startdate><enddate>20211201</enddate><creator>Zhang, Peng</creator><creator>Liu, Bin</creator><creator>Li, Yunfeng</creator><creator>Chen, Ning</creator><creator>Du, Yanping</creator><creator>Chang, Wei</creator><creator>Yang, Huixi</creator><creator>Hong, Wanyu</creator><creator>Li, Yidan</creator><creator>Yang, Gaixia</creator><general>Pleiades Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20211201</creationdate><title>Egg White-Mediated Synthesis and Application of Ag/CeO2 Photocatalyst for Enhanced Photocatalytic Activity under Visible Light Irradiation</title><author>Zhang, Peng ; Liu, Bin ; Li, Yunfeng ; Chen, Ning ; Du, Yanping ; Chang, Wei ; Yang, Huixi ; Hong, Wanyu ; Li, Yidan ; Yang, Gaixia</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c316t-4e63a6711646750a2777db9ed01085b0b32515fb4d25a78f211f123987d114803</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Albumen</topic><topic>Catalytic activity</topic><topic>Cerium oxides</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Doping</topic><topic>Eggs</topic><topic>Holes (electron deficiencies)</topic><topic>Inorganic Chemistry</topic><topic>Light irradiation</topic><topic>Methylene blue</topic><topic>Photocatalysis</topic><topic>Photocatalysts</topic><topic>Photodegradation</topic><topic>Roasting</topic><topic>Synthesis and Properties of Inorganic Compounds</topic><topic>Xenon lamps</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Peng</creatorcontrib><creatorcontrib>Liu, Bin</creatorcontrib><creatorcontrib>Li, Yunfeng</creatorcontrib><creatorcontrib>Chen, Ning</creatorcontrib><creatorcontrib>Du, Yanping</creatorcontrib><creatorcontrib>Chang, Wei</creatorcontrib><creatorcontrib>Yang, Huixi</creatorcontrib><creatorcontrib>Hong, Wanyu</creatorcontrib><creatorcontrib>Li, Yidan</creatorcontrib><creatorcontrib>Yang, Gaixia</creatorcontrib><collection>CrossRef</collection><jtitle>Russian journal of inorganic chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Peng</au><au>Liu, Bin</au><au>Li, Yunfeng</au><au>Chen, Ning</au><au>Du, Yanping</au><au>Chang, Wei</au><au>Yang, Huixi</au><au>Hong, Wanyu</au><au>Li, Yidan</au><au>Yang, Gaixia</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Egg White-Mediated Synthesis and Application of Ag/CeO2 Photocatalyst for Enhanced Photocatalytic Activity under Visible Light Irradiation</atitle><jtitle>Russian journal of inorganic chemistry</jtitle><stitle>Russ. J. Inorg. Chem</stitle><date>2021-12-01</date><risdate>2021</risdate><volume>66</volume><issue>14</issue><spage>2036</spage><epage>2044</epage><pages>2036-2044</pages><issn>0036-0236</issn><eissn>1531-8613</eissn><abstract>The Ag/CeO
2
composite photocatalysts have been successfully prepared using fresh egg white as a gelling agent at various calcination temperatures, respectively. It has been found that Ag doping reduces the band gap of the composite and improves its response to visible light. The photocatalytic performance of Ag/CeO
2
composite photocatalysts prepared at different calcination temperatures has been tested, and it has been found that the samples calcined at 600°C have excellent properties compared with pure CeO
2
. The degradation rate of the sample calcination at 600°C to methylene blue (MB) reached 94.9% under a 300 W Xenon lamp light irradiation for 60 min. In addition, the Ag/CeO
2
photocatalyst exhibits good photocatalytic stability and durability. Finally, the mechanism of photocatalytic degradation of MB is proposed in combination with the active substance capture test. The high photocatalytic activity of Ag/CeO
2
composite photocatalysts may be attributed to the doping of Ag, which inhibits the recombination of photogenerated electron-hole pairs.</abstract><cop>Moscow</cop><pub>Pleiades Publishing</pub><doi>10.1134/S0036023621140096</doi><tpages>9</tpages></addata></record> |
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subjects | Albumen Catalytic activity Cerium oxides Chemistry Chemistry and Materials Science Doping Eggs Holes (electron deficiencies) Inorganic Chemistry Light irradiation Methylene blue Photocatalysis Photocatalysts Photodegradation Roasting Synthesis and Properties of Inorganic Compounds Xenon lamps |
title | Egg White-Mediated Synthesis and Application of Ag/CeO2 Photocatalyst for Enhanced Photocatalytic Activity under Visible Light Irradiation |
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