Experimental and theoretical study of a new CDI device for the treatment of desulfurization wastewater
According to the characteristics of desulfurization wastewater, A new capacitive deionization (CDI) device was designed to study the desalination characteristics of desulfurization wastewater in this paper. The experiments investigated the desalination efficiency under different conditions which fin...
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| Veröffentlicht in: | Environmental science and pollution research international 2022, Vol.29 (1), p.518-530 |
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| creator | Liu, Chang Ma, Lan Xu, Yongyi Wang, Feng Tan, Yu Huang, Luyue Ma, Shuangchen |
| description | According to the characteristics of desulfurization wastewater, A new capacitive deionization (CDI) device was designed to study the desalination characteristics of desulfurization wastewater in this paper. The experiments investigated the desalination efficiency under different conditions which find that the best desalination efficiency is achieved at a voltage of 1.2V, pH=11 and 50°C. Besides, ion adsorption is more favorable under acidic and alkaline conditions. The anion and cation removal performance experiments showed that the order of cation removal is Mg
2+
>Na
+
>Ca
2+
>K
+
and the order of anion removal is Cl
-
>CO
3
2-
>NO
3
-
>SO
4
2-
>HCO
3
-
. The mechanism of CDI was studied and analyzed by the isothermal adsorption model and COMSOL simulation software. It was found that the Freundlich model and Redlich-Peterson model have a good fit with the experimental results. The experiments show that the CDI device has excellent stability. CDI device was used to treat actual desulfurization wastewater. Furthermore, the study provides theoretical support for the industrial application of CDI for desulfurization wastewater treatment in the future.
Graphical abstract |
| doi_str_mv | 10.1007/s11356-021-15651-2 |
| format | Article |
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2+
>Na
+
>Ca
2+
>K
+
and the order of anion removal is Cl
-
>CO
3
2-
>NO
3
-
>SO
4
2-
>HCO
3
-
. The mechanism of CDI was studied and analyzed by the isothermal adsorption model and COMSOL simulation software. It was found that the Freundlich model and Redlich-Peterson model have a good fit with the experimental results. The experiments show that the CDI device has excellent stability. CDI device was used to treat actual desulfurization wastewater. Furthermore, the study provides theoretical support for the industrial application of CDI for desulfurization wastewater treatment in the future.
Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-15651-2</identifier><identifier>PMID: 34331231</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Anions ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Calcium ions ; Cations ; Chlorides ; Deionization ; Desalination ; Desulfurization ; Desulfurizing ; Earth and Environmental Science ; Ecotoxicology ; Electrodes ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Experiments ; Industrial applications ; Ion adsorption ; Magnesium ; Models, Theoretical ; Research Article ; Waste Water ; Waste Water Technology ; Wastewater treatment ; Water Management ; Water Pollution Control ; Water Purification</subject><ispartof>Environmental science and pollution research international, 2022, Vol.29 (1), p.518-530</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>2021. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c419t-86a4a218c72987533e2da3d2fab51b5eb82c6b886c9a4e2e5e67ddd3b479cb073</citedby><cites>FETCH-LOGICAL-c419t-86a4a218c72987533e2da3d2fab51b5eb82c6b886c9a4e2e5e67ddd3b479cb073</cites><orcidid>0000-0002-9640-2957</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-021-15651-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-021-15651-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,782,786,27931,27932,41495,42564,51326</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/34331231$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Chang</creatorcontrib><creatorcontrib>Ma, Lan</creatorcontrib><creatorcontrib>Xu, Yongyi</creatorcontrib><creatorcontrib>Wang, Feng</creatorcontrib><creatorcontrib>Tan, Yu</creatorcontrib><creatorcontrib>Huang, Luyue</creatorcontrib><creatorcontrib>Ma, Shuangchen</creatorcontrib><title>Experimental and theoretical study of a new CDI device for the treatment of desulfurization wastewater</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>According to the characteristics of desulfurization wastewater, A new capacitive deionization (CDI) device was designed to study the desalination characteristics of desulfurization wastewater in this paper. The experiments investigated the desalination efficiency under different conditions which find that the best desalination efficiency is achieved at a voltage of 1.2V, pH=11 and 50°C. Besides, ion adsorption is more favorable under acidic and alkaline conditions. The anion and cation removal performance experiments showed that the order of cation removal is Mg
2+
>Na
+
>Ca
2+
>K
+
and the order of anion removal is Cl
-
>CO
3
2-
>NO
3
-
>SO
4
2-
>HCO
3
-
. The mechanism of CDI was studied and analyzed by the isothermal adsorption model and COMSOL simulation software. It was found that the Freundlich model and Redlich-Peterson model have a good fit with the experimental results. The experiments show that the CDI device has excellent stability. CDI device was used to treat actual desulfurization wastewater. Furthermore, the study provides theoretical support for the industrial application of CDI for desulfurization wastewater treatment in the future.
Graphical abstract</description><subject>Adsorption</subject><subject>Anions</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Calcium ions</subject><subject>Cations</subject><subject>Chlorides</subject><subject>Deionization</subject><subject>Desalination</subject><subject>Desulfurization</subject><subject>Desulfurizing</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Electrodes</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Experiments</subject><subject>Industrial applications</subject><subject>Ion adsorption</subject><subject>Magnesium</subject><subject>Models, Theoretical</subject><subject>Research Article</subject><subject>Waste Water</subject><subject>Waste Water Technology</subject><subject>Wastewater 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and theoretical study of a new CDI device for the treatment of desulfurization wastewater</title><author>Liu, Chang ; Ma, Lan ; Xu, Yongyi ; Wang, Feng ; Tan, Yu ; Huang, Luyue ; Ma, Shuangchen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c419t-86a4a218c72987533e2da3d2fab51b5eb82c6b886c9a4e2e5e67ddd3b479cb073</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Adsorption</topic><topic>Anions</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Calcium ions</topic><topic>Cations</topic><topic>Chlorides</topic><topic>Deionization</topic><topic>Desalination</topic><topic>Desulfurization</topic><topic>Desulfurizing</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Electrodes</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental 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Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2022</date><risdate>2022</risdate><volume>29</volume><issue>1</issue><spage>518</spage><epage>530</epage><pages>518-530</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>According to the characteristics of desulfurization wastewater, A new capacitive deionization (CDI) device was designed to study the desalination characteristics of desulfurization wastewater in this paper. The experiments investigated the desalination efficiency under different conditions which find that the best desalination efficiency is achieved at a voltage of 1.2V, pH=11 and 50°C. Besides, ion adsorption is more favorable under acidic and alkaline conditions. The anion and cation removal performance experiments showed that the order of cation removal is Mg
2+
>Na
+
>Ca
2+
>K
+
and the order of anion removal is Cl
-
>CO
3
2-
>NO
3
-
>SO
4
2-
>HCO
3
-
. The mechanism of CDI was studied and analyzed by the isothermal adsorption model and COMSOL simulation software. It was found that the Freundlich model and Redlich-Peterson model have a good fit with the experimental results. The experiments show that the CDI device has excellent stability. CDI device was used to treat actual desulfurization wastewater. Furthermore, the study provides theoretical support for the industrial application of CDI for desulfurization wastewater treatment in the future.
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| source | MEDLINE; SpringerNature Journals |
| subjects | Adsorption Anions Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Calcium ions Cations Chlorides Deionization Desalination Desulfurization Desulfurizing Earth and Environmental Science Ecotoxicology Electrodes Environment Environmental Chemistry Environmental Health Environmental science Experiments Industrial applications Ion adsorption Magnesium Models, Theoretical Research Article Waste Water Waste Water Technology Wastewater treatment Water Management Water Pollution Control Water Purification |
| title | Experimental and theoretical study of a new CDI device for the treatment of desulfurization wastewater |
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