Supported Nickel Zeolite Catalyst for Oxidative Conversion of Methane: Effect of Heteroatoms in the Zeolite Framework on Its Physicochemical and Catalytic Properties
Supported nickel CHA-type zeolites with different framework compositions including borosilicate, gallosilicate and aluminosilicate were synthesized. The effect of heteroatoms in the framework on the state of the Ni species introduced was investigated. The size and dispersibility of the Ni species di...
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| Veröffentlicht in: | Chemistry letters 2022-01, Vol.51 (1), p.46-49 |
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| container_title | Chemistry letters |
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| creator | Yasuda, Shuhei Kunitake, Yusuke Osuga, Ryota Nakamura, Kengo Matsumoto, Takeshi Sago, Keita Kondo, Junko N Yabushita, Mizuho Muramatsu, Atsushi Yokoi, Toshiyuki |
| description | Supported nickel CHA-type zeolites with different framework compositions including borosilicate, gallosilicate and aluminosilicate were synthesized. The effect of heteroatoms in the framework on the state of the Ni species introduced was investigated. The size and dispersibility of the Ni species differed greatly depending on the heteroatom in the zeolite framework, and the use of the aluminosilicate-type framework led to the formation of a highly dispersed and nano-sized Ni species. Thus, prepared Supported Ni CHA-type aluminosilicate exhibited the highest catalytic performance in oxidative conversion of CH4. |
| doi_str_mv | 10.1246/cl.210563 |
| format | Article |
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The effect of heteroatoms in the framework on the state of the Ni species introduced was investigated. The size and dispersibility of the Ni species differed greatly depending on the heteroatom in the zeolite framework, and the use of the aluminosilicate-type framework led to the formation of a highly dispersed and nano-sized Ni species. 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The effect of heteroatoms in the framework on the state of the Ni species introduced was investigated. The size and dispersibility of the Ni species differed greatly depending on the heteroatom in the zeolite framework, and the use of the aluminosilicate-type framework led to the formation of a highly dispersed and nano-sized Ni species. Thus, prepared Supported Ni CHA-type aluminosilicate exhibited the highest catalytic performance in oxidative conversion of CH4.</description><subject>Aluminosilicates</subject><subject>Aluminum silicates</subject><subject>Catalytic converters</subject><subject>Conversion</subject><subject>Dispersion</subject><subject>Methane</subject><subject>Nickel</subject><subject>Zeolites</subject><issn>0366-7022</issn><issn>1348-0715</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNplkc1OwzAQhC0EEqVw4A0sceKQYsexk3JDFaVI5UcCLlyixd6oLmkcbLfQB-I9SdUKDpxWGn0zo90l5JSzAU8zdaHrQcqZVGKP9LjIioTlXO6THhNKJTlL00NyFMKcMVYMRdoj30_LtnU-oqH3Vr9jTV_R1TYiHUGEeh0irZynD1_WQLSrTnbNCn2wrqGuoncYZ9DgJb2uKtRxI00woncQ3SJQ29A4w9_IsYcFfjr_Tjv3bQz0cbYOVjs9w4XVUFNozK43Wk0fvWvRR4vhmBxUUAc82c0-eRlfP48myfTh5nZ0NU20yFlMzJDnVSZVqt4EKzg32oDBVORZroQpmMiYGWb55i4SJQAwDlIMC21MplXBRZ-cbXNb7z6WGGI5d0vfdJVlqrjMpSyE6KjzLaW9C8FjVbbeLsCvS87KzRdKXZfbL3Ss2rG7HYPTFuN6Di00f-n_jT99Eo7x</recordid><startdate>20220101</startdate><enddate>20220101</enddate><creator>Yasuda, Shuhei</creator><creator>Kunitake, Yusuke</creator><creator>Osuga, Ryota</creator><creator>Nakamura, Kengo</creator><creator>Matsumoto, Takeshi</creator><creator>Sago, Keita</creator><creator>Kondo, Junko N</creator><creator>Yabushita, Mizuho</creator><creator>Muramatsu, Atsushi</creator><creator>Yokoi, Toshiyuki</creator><general>The Chemical Society of Japan</general><general>Chemical Society of Japan</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope></search><sort><creationdate>20220101</creationdate><title>Supported Nickel Zeolite Catalyst for Oxidative Conversion of Methane: Effect of Heteroatoms in the Zeolite Framework on Its Physicochemical and Catalytic Properties</title><author>Yasuda, Shuhei ; Kunitake, Yusuke ; Osuga, Ryota ; Nakamura, Kengo ; Matsumoto, Takeshi ; Sago, Keita ; Kondo, Junko N ; Yabushita, Mizuho ; Muramatsu, Atsushi ; Yokoi, Toshiyuki</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c370t-d917f45626b30811dcdade2374763d80340d94713485e5aaa01a5398cdd4c6813</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Aluminosilicates</topic><topic>Aluminum silicates</topic><topic>Catalytic converters</topic><topic>Conversion</topic><topic>Dispersion</topic><topic>Methane</topic><topic>Nickel</topic><topic>Zeolites</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yasuda, Shuhei</creatorcontrib><creatorcontrib>Kunitake, Yusuke</creatorcontrib><creatorcontrib>Osuga, Ryota</creatorcontrib><creatorcontrib>Nakamura, Kengo</creatorcontrib><creatorcontrib>Matsumoto, Takeshi</creatorcontrib><creatorcontrib>Sago, Keita</creatorcontrib><creatorcontrib>Kondo, Junko N</creatorcontrib><creatorcontrib>Yabushita, Mizuho</creatorcontrib><creatorcontrib>Muramatsu, Atsushi</creatorcontrib><creatorcontrib>Yokoi, Toshiyuki</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Chemistry letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yasuda, Shuhei</au><au>Kunitake, Yusuke</au><au>Osuga, Ryota</au><au>Nakamura, Kengo</au><au>Matsumoto, Takeshi</au><au>Sago, Keita</au><au>Kondo, Junko N</au><au>Yabushita, Mizuho</au><au>Muramatsu, Atsushi</au><au>Yokoi, Toshiyuki</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Supported Nickel Zeolite Catalyst for Oxidative Conversion of Methane: Effect of Heteroatoms in the Zeolite Framework on Its Physicochemical and Catalytic Properties</atitle><jtitle>Chemistry letters</jtitle><date>2022-01-01</date><risdate>2022</risdate><volume>51</volume><issue>1</issue><spage>46</spage><epage>49</epage><pages>46-49</pages><issn>0366-7022</issn><eissn>1348-0715</eissn><abstract>Supported nickel CHA-type zeolites with different framework compositions including borosilicate, gallosilicate and aluminosilicate were synthesized. The effect of heteroatoms in the framework on the state of the Ni species introduced was investigated. The size and dispersibility of the Ni species differed greatly depending on the heteroatom in the zeolite framework, and the use of the aluminosilicate-type framework led to the formation of a highly dispersed and nano-sized Ni species. Thus, prepared Supported Ni CHA-type aluminosilicate exhibited the highest catalytic performance in oxidative conversion of CH4.</abstract><cop>Tokyo</cop><pub>The Chemical Society of Japan</pub><doi>10.1246/cl.210563</doi><tpages>4</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0366-7022 |
| ispartof | Chemistry letters, 2022-01, Vol.51 (1), p.46-49 |
| issn | 0366-7022 1348-0715 |
| language | eng |
| recordid | cdi_proquest_journals_2615755833 |
| source | Oxford University Press Journals All Titles (1996-Current) |
| subjects | Aluminosilicates Aluminum silicates Catalytic converters Conversion Dispersion Methane Nickel Zeolites |
| title | Supported Nickel Zeolite Catalyst for Oxidative Conversion of Methane: Effect of Heteroatoms in the Zeolite Framework on Its Physicochemical and Catalytic Properties |
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