Plasmon–Exciton Interactions: Spontaneous Emission and Strong Coupling

The extraordinary optical properties of surface plasmons in metal nanostructures provide the possibilities to enhance and accelerate the spontaneous emission, and manipulate the decay and emission processes of quantum emitters. The extremely small mode volume of plasmonic nanocavities also benefits...

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Veröffentlicht in:Advanced functional materials 2021-12, Vol.31 (51), p.n/a
Hauptverfasser: Wei, Hong, Yan, Xiaohong, Niu, Yijie, Li, Qiang, Jia, Zhili, Xu, Hongxing
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container_issue 51
container_start_page
container_title Advanced functional materials
container_volume 31
creator Wei, Hong
Yan, Xiaohong
Niu, Yijie
Li, Qiang
Jia, Zhili
Xu, Hongxing
description The extraordinary optical properties of surface plasmons in metal nanostructures provide the possibilities to enhance and accelerate the spontaneous emission, and manipulate the decay and emission processes of quantum emitters. The extremely small mode volume of plasmonic nanocavities also benefits the realization of plasmon–exciton strong coupling. Here, the progress on the study of plasmon modified spontaneous emission and plasmon–exciton strong coupling are reviewed. The fundamentals of surface plasmons and quantum emitters, and the methods for assembling coupling systems of plasmonic nanostructures and quantum emitters are first introduced. Then the major aspects of plasmon modified spontaneous emission, including emission intensity, lifetime, spectral profile, direction, polarization, and energy transfer are reviewed. The coupling of quantum emitters and plasmonic waveguides is then discussed. Next, the developments of strong coupling between plasmonic structures and various quantum emitters are reviewed. Finally a few applications are highlighted followed by conclusions and outlook. This review summarizes the progress on both the weak and strong coupling between surface plasmons and excitons. Typical methods for assembling coupling systems of plasmonic nanostructures and quantum emitters are introduced. The major aspects of plasmon modified spontaneous emission and the developments of strong coupling between plasmonic structures and various quantum emitters are reviewed.
doi_str_mv 10.1002/adfm.202100889
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The extremely small mode volume of plasmonic nanocavities also benefits the realization of plasmon–exciton strong coupling. Here, the progress on the study of plasmon modified spontaneous emission and plasmon–exciton strong coupling are reviewed. The fundamentals of surface plasmons and quantum emitters, and the methods for assembling coupling systems of plasmonic nanostructures and quantum emitters are first introduced. Then the major aspects of plasmon modified spontaneous emission, including emission intensity, lifetime, spectral profile, direction, polarization, and energy transfer are reviewed. The coupling of quantum emitters and plasmonic waveguides is then discussed. Next, the developments of strong coupling between plasmonic structures and various quantum emitters are reviewed. Finally a few applications are highlighted followed by conclusions and outlook. This review summarizes the progress on both the weak and strong coupling between surface plasmons and excitons. 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subjects Coupling
Emission analysis
Emitters
Energy transfer
Excitons
Materials science
nanocavities
Nanostructure
optical antennas
Optical properties
Plasmonics
Plasmons
quantum emitters
Rabi splitting
single‐photon sources
Spontaneous emission
surface plasmons
surface‐enhanced fluorescence
Waveguides
title Plasmon–Exciton Interactions: Spontaneous Emission and Strong Coupling
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