Femtosecond laser micro-nano processing for boosting bubble releasing of gas evolution reactions
Coupling effect of chemical composition and physical structure is a key factor to construct superaerophobic electrodes. Almost all reports about superaerophobic electrodes were aimed at precisely controlling morphology of loaded materials (constructing specific structure) and ignored the due role of...
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| Veröffentlicht in: | Nano research 2022-02, Vol.15 (2), p.1672-1679 |
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| container_title | Nano research |
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| creator | Zhang, Shuai Xu, Lishuang Wu, Jie Yang, Ying Zhang, Chengxin Tao, Haiyan Lin, Jingquan Huang, Licheng Fang, Wencheng Shi, Keying Dong, Xiangting |
| description | Coupling effect of chemical composition and physical structure is a key factor to construct superaerophobic electrodes. Almost all reports about superaerophobic electrodes were aimed at precisely controlling morphology of loaded materials (constructing specific structure) and ignored the due role of substrate. Nevertheless, in this work, by using high precision and controllable femtosecond laser, hierarchical micro-nano structures with superaerophobic properties were constructed on the surface of silicon substrate (fs-Si), and such special super-wettability could be successfully inherited to subsequent self-supporting electrodes through chemical synthesis. Femtosecond laser processing endowed electrodes with high electrochemical surface area, strong physical structure, and remarkable superaerophobic efficacy. As an unconventional processing method, the reconstructed morphology of substrate surface bears the responsibility of superaerophobicity, thus liberating the structural constraints on loaded materials. Since this key of coupling effect is transferred from the loaded materials to substrate, we provided a new general scheme for synthesizing superaerophobic electrodes. The successful introduction of femtosecond laser will open a new idea to synthesize self-supporting electrodes for gas-involving reactions. |
| doi_str_mv | 10.1007/s12274-021-3811-3 |
| format | Article |
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Almost all reports about superaerophobic electrodes were aimed at precisely controlling morphology of loaded materials (constructing specific structure) and ignored the due role of substrate. Nevertheless, in this work, by using high precision and controllable femtosecond laser, hierarchical micro-nano structures with superaerophobic properties were constructed on the surface of silicon substrate (fs-Si), and such special super-wettability could be successfully inherited to subsequent self-supporting electrodes through chemical synthesis. Femtosecond laser processing endowed electrodes with high electrochemical surface area, strong physical structure, and remarkable superaerophobic efficacy. As an unconventional processing method, the reconstructed morphology of substrate surface bears the responsibility of superaerophobicity, thus liberating the structural constraints on loaded materials. Since this key of coupling effect is transferred from the loaded materials to substrate, we provided a new general scheme for synthesizing superaerophobic electrodes. The successful introduction of femtosecond laser will open a new idea to synthesize self-supporting electrodes for gas-involving reactions.</description><identifier>ISSN: 1998-0124</identifier><identifier>EISSN: 1998-0000</identifier><identifier>DOI: 10.1007/s12274-021-3811-3</identifier><language>eng</language><publisher>Beijing: Tsinghua University Press</publisher><subject>Atomic/Molecular Structure and Spectra ; Biomedicine ; Biotechnology ; Chemical composition ; Chemical reactions ; Chemical synthesis ; Chemistry and Materials Science ; Composition effects ; Condensed Matter Physics ; Controllability ; Coupling ; Electrochemistry ; Electrodes ; Gas evolution ; Laser processing ; Lasers ; Materials Science ; Morphology ; Nanotechnology ; Research Article ; Silicon substrates ; Structural hierarchy ; Substrates ; Wettability</subject><ispartof>Nano research, 2022-02, Vol.15 (2), p.1672-1679</ispartof><rights>Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c316t-ba376cf81ee586e2f8cfc2c895027f9bec1e775bbc479af284ab8d247e177233</citedby><cites>FETCH-LOGICAL-c316t-ba376cf81ee586e2f8cfc2c895027f9bec1e775bbc479af284ab8d247e177233</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s12274-021-3811-3$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s12274-021-3811-3$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Zhang, Shuai</creatorcontrib><creatorcontrib>Xu, Lishuang</creatorcontrib><creatorcontrib>Wu, Jie</creatorcontrib><creatorcontrib>Yang, Ying</creatorcontrib><creatorcontrib>Zhang, Chengxin</creatorcontrib><creatorcontrib>Tao, Haiyan</creatorcontrib><creatorcontrib>Lin, Jingquan</creatorcontrib><creatorcontrib>Huang, Licheng</creatorcontrib><creatorcontrib>Fang, Wencheng</creatorcontrib><creatorcontrib>Shi, Keying</creatorcontrib><creatorcontrib>Dong, Xiangting</creatorcontrib><title>Femtosecond laser micro-nano processing for boosting bubble releasing of gas evolution reactions</title><title>Nano research</title><addtitle>Nano Res</addtitle><description>Coupling effect of chemical composition and physical structure is a key factor to construct superaerophobic electrodes. Almost all reports about superaerophobic electrodes were aimed at precisely controlling morphology of loaded materials (constructing specific structure) and ignored the due role of substrate. Nevertheless, in this work, by using high precision and controllable femtosecond laser, hierarchical micro-nano structures with superaerophobic properties were constructed on the surface of silicon substrate (fs-Si), and such special super-wettability could be successfully inherited to subsequent self-supporting electrodes through chemical synthesis. Femtosecond laser processing endowed electrodes with high electrochemical surface area, strong physical structure, and remarkable superaerophobic efficacy. As an unconventional processing method, the reconstructed morphology of substrate surface bears the responsibility of superaerophobicity, thus liberating the structural constraints on loaded materials. Since this key of coupling effect is transferred from the loaded materials to substrate, we provided a new general scheme for synthesizing superaerophobic electrodes. The successful introduction of femtosecond laser will open a new idea to synthesize self-supporting electrodes for gas-involving reactions.</description><subject>Atomic/Molecular Structure and Spectra</subject><subject>Biomedicine</subject><subject>Biotechnology</subject><subject>Chemical composition</subject><subject>Chemical reactions</subject><subject>Chemical synthesis</subject><subject>Chemistry and Materials Science</subject><subject>Composition effects</subject><subject>Condensed Matter Physics</subject><subject>Controllability</subject><subject>Coupling</subject><subject>Electrochemistry</subject><subject>Electrodes</subject><subject>Gas evolution</subject><subject>Laser processing</subject><subject>Lasers</subject><subject>Materials Science</subject><subject>Morphology</subject><subject>Nanotechnology</subject><subject>Research Article</subject><subject>Silicon substrates</subject><subject>Structural 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evolution</topic><topic>Laser processing</topic><topic>Lasers</topic><topic>Materials Science</topic><topic>Morphology</topic><topic>Nanotechnology</topic><topic>Research Article</topic><topic>Silicon substrates</topic><topic>Structural hierarchy</topic><topic>Substrates</topic><topic>Wettability</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Shuai</creatorcontrib><creatorcontrib>Xu, Lishuang</creatorcontrib><creatorcontrib>Wu, Jie</creatorcontrib><creatorcontrib>Yang, Ying</creatorcontrib><creatorcontrib>Zhang, Chengxin</creatorcontrib><creatorcontrib>Tao, Haiyan</creatorcontrib><creatorcontrib>Lin, Jingquan</creatorcontrib><creatorcontrib>Huang, Licheng</creatorcontrib><creatorcontrib>Fang, Wencheng</creatorcontrib><creatorcontrib>Shi, Keying</creatorcontrib><creatorcontrib>Dong, Xiangting</creatorcontrib><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aluminium Industry 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Almost all reports about superaerophobic electrodes were aimed at precisely controlling morphology of loaded materials (constructing specific structure) and ignored the due role of substrate. Nevertheless, in this work, by using high precision and controllable femtosecond laser, hierarchical micro-nano structures with superaerophobic properties were constructed on the surface of silicon substrate (fs-Si), and such special super-wettability could be successfully inherited to subsequent self-supporting electrodes through chemical synthesis. Femtosecond laser processing endowed electrodes with high electrochemical surface area, strong physical structure, and remarkable superaerophobic efficacy. As an unconventional processing method, the reconstructed morphology of substrate surface bears the responsibility of superaerophobicity, thus liberating the structural constraints on loaded materials. Since this key of coupling effect is transferred from the loaded materials to substrate, we provided a new general scheme for synthesizing superaerophobic electrodes. The successful introduction of femtosecond laser will open a new idea to synthesize self-supporting electrodes for gas-involving reactions.</abstract><cop>Beijing</cop><pub>Tsinghua University Press</pub><doi>10.1007/s12274-021-3811-3</doi><tpages>8</tpages></addata></record> |
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| identifier | ISSN: 1998-0124 |
| ispartof | Nano research, 2022-02, Vol.15 (2), p.1672-1679 |
| issn | 1998-0124 1998-0000 |
| language | eng |
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| subjects | Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Chemical composition Chemical reactions Chemical synthesis Chemistry and Materials Science Composition effects Condensed Matter Physics Controllability Coupling Electrochemistry Electrodes Gas evolution Laser processing Lasers Materials Science Morphology Nanotechnology Research Article Silicon substrates Structural hierarchy Substrates Wettability |
| title | Femtosecond laser micro-nano processing for boosting bubble releasing of gas evolution reactions |
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