Effects of interactions between organic solid waste components on the formation of heavy components in oil during pyrolysis

This study focused on the interaction between organic solid waste (OSW) components on the formation and chemical composition of heavy components (>150 m/z) in OSW-oil. Rice husk (RH) and polypropylene (PP) as typical biomass and plastic fractions in OSW, were co-pyrolyzed at different blend ratio...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Fuel processing technology 2022-01, Vol.225, p.107041, Article 107041
Hauptverfasser: Engamba Esso, Samy Berthold, Xu, Longfei, Han, Hengda, Xiong, Zhe, Kamara, Melvina Fudia, Xu, Jun, Jiang, Long, Su, Sheng, Hu, Song, Wang, Yi, Xiang, Jun
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page
container_issue
container_start_page 107041
container_title Fuel processing technology
container_volume 225
creator Engamba Esso, Samy Berthold
Xu, Longfei
Han, Hengda
Xiong, Zhe
Kamara, Melvina Fudia
Xu, Jun
Jiang, Long
Su, Sheng
Hu, Song
Wang, Yi
Xiang, Jun
description This study focused on the interaction between organic solid waste (OSW) components on the formation and chemical composition of heavy components (>150 m/z) in OSW-oil. Rice husk (RH) and polypropylene (PP) as typical biomass and plastic fractions in OSW, were co-pyrolyzed at different blend ratios and different temperatures. The heavy components were characterized by FT-ICR MS, UV-F and GC MS. The results indicated that the yield of heavy components in PP-oil was higher than in RH-oil under the same temperature. Heavy hydrocarbons were found in PP-oil, while heavy phenols and heavy lipids existed in RH-oil. Significant interactions occurred at high temperatures (>600 °C). The interactions promoted the heavy components in all the blend-oils, corresponding to an increase of 20–35% compared to the calculated value of the content in PP-oil and RH-oil. At low PP ratio (25PP + 75RH), PP provided hydrogen to the reactive O-containing species in RH, leading to promoted heavy phenols and heavy lipids. At high PP ratio (50PP + 50RH and 75PP + 25RH), large aromatics (>3 rings) increased of 48–111% with respect to the calculated values. Plenty of PP‑hydrogen and a rich oxygen environment provided by RH radicals enhanced the formation of heavy aromatics and heavy PAH. •Interactions between OSW components affect the formation of heavy components in the oil.•Temperature and blending ratio change the interaction effects on the heavy component formation.•Hydrogen provided by PP enhanced the recombination of heavy O-containing species.•Rich oxygen environment provided by RH enhanced the formation of heavy PAH.
doi_str_mv 10.1016/j.fuproc.2021.107041
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2606929381</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S0378382021003209</els_id><sourcerecordid>2606929381</sourcerecordid><originalsourceid>FETCH-LOGICAL-c334t-bcacf9052826787bfcc702b27b336d4599c56d3b5cd8937a127acc9582609e413</originalsourceid><addsrcrecordid>eNp9kE1rGzEQhkVJIE7Sf5CDoOd19bG7ki6FEtK0YMilPQvt7MiWsSVXWieY_vlq2R56ymlgeN53mIeQB87WnPH-837tz6ecYC2Y4HWlWMs_kBXXSjaKa31FVkwq3Ugt2A25LWXPGOs6o1bkz5P3CFOhydMQJ8wOppBioQNOb4iRprx1MQAt6RBG-ubKhBTS8ZQixjkW6bRD6lM-ujk49-zQvV7-h0JdhwMdzznELT1dcjpcSij35Nq7Q8GP_-Yd-fXt6efj92bz8vzj8eumASnbqRnAgTesE1r0SqvBAygmBqEGKfux7YyBrh_l0MGojVSOC-UATFdxZrDl8o58Wnqro99nLJPdp3OO9aStSG-EkXqm2oWCnErJ6O0ph6PLF8uZnTXbvV0021mzXTTX2JclhvWD14DZFggYAceQq1g7pvB-wV-Gb4pI</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2606929381</pqid></control><display><type>article</type><title>Effects of interactions between organic solid waste components on the formation of heavy components in oil during pyrolysis</title><source>Access via ScienceDirect (Elsevier)</source><creator>Engamba Esso, Samy Berthold ; Xu, Longfei ; Han, Hengda ; Xiong, Zhe ; Kamara, Melvina Fudia ; Xu, Jun ; Jiang, Long ; Su, Sheng ; Hu, Song ; Wang, Yi ; Xiang, Jun</creator><creatorcontrib>Engamba Esso, Samy Berthold ; Xu, Longfei ; Han, Hengda ; Xiong, Zhe ; Kamara, Melvina Fudia ; Xu, Jun ; Jiang, Long ; Su, Sheng ; Hu, Song ; Wang, Yi ; Xiang, Jun</creatorcontrib><description>This study focused on the interaction between organic solid waste (OSW) components on the formation and chemical composition of heavy components (&gt;150 m/z) in OSW-oil. Rice husk (RH) and polypropylene (PP) as typical biomass and plastic fractions in OSW, were co-pyrolyzed at different blend ratios and different temperatures. The heavy components were characterized by FT-ICR MS, UV-F and GC MS. The results indicated that the yield of heavy components in PP-oil was higher than in RH-oil under the same temperature. Heavy hydrocarbons were found in PP-oil, while heavy phenols and heavy lipids existed in RH-oil. Significant interactions occurred at high temperatures (&gt;600 °C). The interactions promoted the heavy components in all the blend-oils, corresponding to an increase of 20–35% compared to the calculated value of the content in PP-oil and RH-oil. At low PP ratio (25PP + 75RH), PP provided hydrogen to the reactive O-containing species in RH, leading to promoted heavy phenols and heavy lipids. At high PP ratio (50PP + 50RH and 75PP + 25RH), large aromatics (&gt;3 rings) increased of 48–111% with respect to the calculated values. Plenty of PP‑hydrogen and a rich oxygen environment provided by RH radicals enhanced the formation of heavy aromatics and heavy PAH. •Interactions between OSW components affect the formation of heavy components in the oil.•Temperature and blending ratio change the interaction effects on the heavy component formation.•Hydrogen provided by PP enhanced the recombination of heavy O-containing species.•Rich oxygen environment provided by RH enhanced the formation of heavy PAH.</description><identifier>ISSN: 0378-3820</identifier><identifier>EISSN: 1873-7188</identifier><identifier>DOI: 10.1016/j.fuproc.2021.107041</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Chemical composition ; Co-pyrolysis ; Heavy components ; High temperature ; Interactions ; Lipids ; Mathematical analysis ; Organic solid waste (OSW) ; Phenols ; Polycyclic aromatic hydrocarbons ; Pyrolysis</subject><ispartof>Fuel processing technology, 2022-01, Vol.225, p.107041, Article 107041</ispartof><rights>2021 Elsevier B.V.</rights><rights>Copyright Elsevier Science Ltd. Jan 2022</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c334t-bcacf9052826787bfcc702b27b336d4599c56d3b5cd8937a127acc9582609e413</citedby><cites>FETCH-LOGICAL-c334t-bcacf9052826787bfcc702b27b336d4599c56d3b5cd8937a127acc9582609e413</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.fuproc.2021.107041$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids></links><search><creatorcontrib>Engamba Esso, Samy Berthold</creatorcontrib><creatorcontrib>Xu, Longfei</creatorcontrib><creatorcontrib>Han, Hengda</creatorcontrib><creatorcontrib>Xiong, Zhe</creatorcontrib><creatorcontrib>Kamara, Melvina Fudia</creatorcontrib><creatorcontrib>Xu, Jun</creatorcontrib><creatorcontrib>Jiang, Long</creatorcontrib><creatorcontrib>Su, Sheng</creatorcontrib><creatorcontrib>Hu, Song</creatorcontrib><creatorcontrib>Wang, Yi</creatorcontrib><creatorcontrib>Xiang, Jun</creatorcontrib><title>Effects of interactions between organic solid waste components on the formation of heavy components in oil during pyrolysis</title><title>Fuel processing technology</title><description>This study focused on the interaction between organic solid waste (OSW) components on the formation and chemical composition of heavy components (&gt;150 m/z) in OSW-oil. Rice husk (RH) and polypropylene (PP) as typical biomass and plastic fractions in OSW, were co-pyrolyzed at different blend ratios and different temperatures. The heavy components were characterized by FT-ICR MS, UV-F and GC MS. The results indicated that the yield of heavy components in PP-oil was higher than in RH-oil under the same temperature. Heavy hydrocarbons were found in PP-oil, while heavy phenols and heavy lipids existed in RH-oil. Significant interactions occurred at high temperatures (&gt;600 °C). The interactions promoted the heavy components in all the blend-oils, corresponding to an increase of 20–35% compared to the calculated value of the content in PP-oil and RH-oil. At low PP ratio (25PP + 75RH), PP provided hydrogen to the reactive O-containing species in RH, leading to promoted heavy phenols and heavy lipids. At high PP ratio (50PP + 50RH and 75PP + 25RH), large aromatics (&gt;3 rings) increased of 48–111% with respect to the calculated values. Plenty of PP‑hydrogen and a rich oxygen environment provided by RH radicals enhanced the formation of heavy aromatics and heavy PAH. •Interactions between OSW components affect the formation of heavy components in the oil.•Temperature and blending ratio change the interaction effects on the heavy component formation.•Hydrogen provided by PP enhanced the recombination of heavy O-containing species.•Rich oxygen environment provided by RH enhanced the formation of heavy PAH.</description><subject>Chemical composition</subject><subject>Co-pyrolysis</subject><subject>Heavy components</subject><subject>High temperature</subject><subject>Interactions</subject><subject>Lipids</subject><subject>Mathematical analysis</subject><subject>Organic solid waste (OSW)</subject><subject>Phenols</subject><subject>Polycyclic aromatic hydrocarbons</subject><subject>Pyrolysis</subject><issn>0378-3820</issn><issn>1873-7188</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNp9kE1rGzEQhkVJIE7Sf5CDoOd19bG7ki6FEtK0YMilPQvt7MiWsSVXWieY_vlq2R56ymlgeN53mIeQB87WnPH-837tz6ecYC2Y4HWlWMs_kBXXSjaKa31FVkwq3Ugt2A25LWXPGOs6o1bkz5P3CFOhydMQJ8wOppBioQNOb4iRprx1MQAt6RBG-ubKhBTS8ZQixjkW6bRD6lM-ujk49-zQvV7-h0JdhwMdzznELT1dcjpcSij35Nq7Q8GP_-Yd-fXt6efj92bz8vzj8eumASnbqRnAgTesE1r0SqvBAygmBqEGKfux7YyBrh_l0MGojVSOC-UATFdxZrDl8o58Wnqro99nLJPdp3OO9aStSG-EkXqm2oWCnErJ6O0ph6PLF8uZnTXbvV0021mzXTTX2JclhvWD14DZFggYAceQq1g7pvB-wV-Gb4pI</recordid><startdate>202201</startdate><enddate>202201</enddate><creator>Engamba Esso, Samy Berthold</creator><creator>Xu, Longfei</creator><creator>Han, Hengda</creator><creator>Xiong, Zhe</creator><creator>Kamara, Melvina Fudia</creator><creator>Xu, Jun</creator><creator>Jiang, Long</creator><creator>Su, Sheng</creator><creator>Hu, Song</creator><creator>Wang, Yi</creator><creator>Xiang, Jun</creator><general>Elsevier B.V</general><general>Elsevier Science Ltd</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7TB</scope><scope>8FD</scope><scope>FR3</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>202201</creationdate><title>Effects of interactions between organic solid waste components on the formation of heavy components in oil during pyrolysis</title><author>Engamba Esso, Samy Berthold ; Xu, Longfei ; Han, Hengda ; Xiong, Zhe ; Kamara, Melvina Fudia ; Xu, Jun ; Jiang, Long ; Su, Sheng ; Hu, Song ; Wang, Yi ; Xiang, Jun</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c334t-bcacf9052826787bfcc702b27b336d4599c56d3b5cd8937a127acc9582609e413</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Chemical composition</topic><topic>Co-pyrolysis</topic><topic>Heavy components</topic><topic>High temperature</topic><topic>Interactions</topic><topic>Lipids</topic><topic>Mathematical analysis</topic><topic>Organic solid waste (OSW)</topic><topic>Phenols</topic><topic>Polycyclic aromatic hydrocarbons</topic><topic>Pyrolysis</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Engamba Esso, Samy Berthold</creatorcontrib><creatorcontrib>Xu, Longfei</creatorcontrib><creatorcontrib>Han, Hengda</creatorcontrib><creatorcontrib>Xiong, Zhe</creatorcontrib><creatorcontrib>Kamara, Melvina Fudia</creatorcontrib><creatorcontrib>Xu, Jun</creatorcontrib><creatorcontrib>Jiang, Long</creatorcontrib><creatorcontrib>Su, Sheng</creatorcontrib><creatorcontrib>Hu, Song</creatorcontrib><creatorcontrib>Wang, Yi</creatorcontrib><creatorcontrib>Xiang, Jun</creatorcontrib><collection>CrossRef</collection><collection>Mechanical &amp; Transportation Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Fuel processing technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Engamba Esso, Samy Berthold</au><au>Xu, Longfei</au><au>Han, Hengda</au><au>Xiong, Zhe</au><au>Kamara, Melvina Fudia</au><au>Xu, Jun</au><au>Jiang, Long</au><au>Su, Sheng</au><au>Hu, Song</au><au>Wang, Yi</au><au>Xiang, Jun</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of interactions between organic solid waste components on the formation of heavy components in oil during pyrolysis</atitle><jtitle>Fuel processing technology</jtitle><date>2022-01</date><risdate>2022</risdate><volume>225</volume><spage>107041</spage><pages>107041-</pages><artnum>107041</artnum><issn>0378-3820</issn><eissn>1873-7188</eissn><abstract>This study focused on the interaction between organic solid waste (OSW) components on the formation and chemical composition of heavy components (&gt;150 m/z) in OSW-oil. Rice husk (RH) and polypropylene (PP) as typical biomass and plastic fractions in OSW, were co-pyrolyzed at different blend ratios and different temperatures. The heavy components were characterized by FT-ICR MS, UV-F and GC MS. The results indicated that the yield of heavy components in PP-oil was higher than in RH-oil under the same temperature. Heavy hydrocarbons were found in PP-oil, while heavy phenols and heavy lipids existed in RH-oil. Significant interactions occurred at high temperatures (&gt;600 °C). The interactions promoted the heavy components in all the blend-oils, corresponding to an increase of 20–35% compared to the calculated value of the content in PP-oil and RH-oil. At low PP ratio (25PP + 75RH), PP provided hydrogen to the reactive O-containing species in RH, leading to promoted heavy phenols and heavy lipids. At high PP ratio (50PP + 50RH and 75PP + 25RH), large aromatics (&gt;3 rings) increased of 48–111% with respect to the calculated values. Plenty of PP‑hydrogen and a rich oxygen environment provided by RH radicals enhanced the formation of heavy aromatics and heavy PAH. •Interactions between OSW components affect the formation of heavy components in the oil.•Temperature and blending ratio change the interaction effects on the heavy component formation.•Hydrogen provided by PP enhanced the recombination of heavy O-containing species.•Rich oxygen environment provided by RH enhanced the formation of heavy PAH.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.fuproc.2021.107041</doi></addata></record>
fulltext fulltext
identifier ISSN: 0378-3820
ispartof Fuel processing technology, 2022-01, Vol.225, p.107041, Article 107041
issn 0378-3820
1873-7188
language eng
recordid cdi_proquest_journals_2606929381
source Access via ScienceDirect (Elsevier)
subjects Chemical composition
Co-pyrolysis
Heavy components
High temperature
Interactions
Lipids
Mathematical analysis
Organic solid waste (OSW)
Phenols
Polycyclic aromatic hydrocarbons
Pyrolysis
title Effects of interactions between organic solid waste components on the formation of heavy components in oil during pyrolysis
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-25T03%3A13%3A55IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Effects%20of%20interactions%20between%20organic%20solid%20waste%20components%20on%20the%20formation%20of%20heavy%20components%20in%20oil%20during%20pyrolysis&rft.jtitle=Fuel%20processing%20technology&rft.au=Engamba%20Esso,%20Samy%20Berthold&rft.date=2022-01&rft.volume=225&rft.spage=107041&rft.pages=107041-&rft.artnum=107041&rft.issn=0378-3820&rft.eissn=1873-7188&rft_id=info:doi/10.1016/j.fuproc.2021.107041&rft_dat=%3Cproquest_cross%3E2606929381%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2606929381&rft_id=info:pmid/&rft_els_id=S0378382021003209&rfr_iscdi=true