CeO2/CdS heterojunction decorated cotton fabric as a recyclable photocatalyst for efficient light driven degradation of methylene blue
In this work, visible light response CeO 2 /CdS decorated cotton fabrics as durable and facile recyclable composite photocatalysts were fabricated for photo-degradation of methylene blue (MB). First of all, amino-functionalized CeO 2 /CdS heterojunctions were synthesized through a fast, efficient an...
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| Veröffentlicht in: | Cellulose (London) 2021-11, Vol.28 (17), p.11081-11096 |
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| creator | Zou, Rui Li, Linhua Yang, Lin Lan, Jianwu Liu, Hongyu Dou, Baojie Shang, Jiaojiao Lin, Shaojian |
| description | In this work, visible light response CeO
2
/CdS decorated cotton fabrics as durable and facile recyclable composite photocatalysts were fabricated for photo-degradation of methylene blue (MB). First of all, amino-functionalized CeO
2
/CdS heterojunctions were synthesized through a fast, efficient and low-cost co-precipitation method. Subsequently, the as-prepared CeO
2
/CdS heterojunctions were immobilized on aldehyde-functionalized cotton fabric surfaces as composite photocatalysts via "amine-aldehyde" chemical reaction. The surface microstructure and chemical composition of the CeO
2
/CdS decorated cotton fabric (CeO
2
/CdS-CF) were characterized by SEM, FTIR and XPS, respectively. The results showed that CeO
2
/CdS heterojunctions were successfully anchored and uniformly distributed on the surface of cotton fabric. Since the CeO
2
/CdS heterostructure with efficient photo-generated charge transfer and separation, the as-prepared CeO
2
/CdS-CF exhibited excellent photocatalytic activity, degrading MB under simulated sunlight irradiation with a degradation efficiency of 93.8% within 90 min. In addition, the degradation efficiency remained above 90.3% even after five successive degradation cycles, indicating the outstanding stability and recyclability of the obtained CeO
2
/CdS-CF. This work opened up a facile preparation way for the fabrication of durable and recyclable composite photocatalysts, and has a promising application in treating dye contaminated wastewater.
Graphic abstract |
| doi_str_mv | 10.1007/s10570-021-04203-z |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2587487223</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2587487223</sourcerecordid><originalsourceid>FETCH-LOGICAL-c319t-2c73b9c5ec388839b1584a7af67c6fbe79755f3f399cf846648dd6d31a954e1d3</originalsourceid><addsrcrecordid>eNp9kMtKAzEUhoMoWKsv4CrgemwuM5NkKcUbFLpQwV3IJCftlOmkJqlQH8DndtoK7lwdOOf_vwMfQteU3FJCxCRRUglSEEYLUjLCi68TNKKVYIWU7P0UjYiq1XDm6hxdpLQihCjB6Ah9T2HOJlP3gpeQIYbVtre5DT12YEM0GRy2Iedh4U0TW4tNwgZHsDvbmaYDvFmGHKzJptuljH2IGLxvbQt9xl27WGbsYvsJe-AiGmcO8ODxGvJy10EPuOm2cInOvOkSXP3OMXp7uH-dPhWz-ePz9G5WWE5VLpgVvFG2AsullFw1tJKlEcbXwta-AaFEVXnuuVLWy7KuS-lc7Tg1qiqBOj5GN0fuJoaPLaSsV2Eb--GlZpUUpRSM8SHFjikbQ0oRvN7Edm3iTlOi97710bcefOuDb_01lPixlIZwv4D4h_6n9QOY0IYo</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2587487223</pqid></control><display><type>article</type><title>CeO2/CdS heterojunction decorated cotton fabric as a recyclable photocatalyst for efficient light driven degradation of methylene blue</title><source>Springer Nature - Complete Springer Journals</source><creator>Zou, Rui ; Li, Linhua ; Yang, Lin ; Lan, Jianwu ; Liu, Hongyu ; Dou, Baojie ; Shang, Jiaojiao ; Lin, Shaojian</creator><creatorcontrib>Zou, Rui ; Li, Linhua ; Yang, Lin ; Lan, Jianwu ; Liu, Hongyu ; Dou, Baojie ; Shang, Jiaojiao ; Lin, Shaojian</creatorcontrib><description>In this work, visible light response CeO
2
/CdS decorated cotton fabrics as durable and facile recyclable composite photocatalysts were fabricated for photo-degradation of methylene blue (MB). First of all, amino-functionalized CeO
2
/CdS heterojunctions were synthesized through a fast, efficient and low-cost co-precipitation method. Subsequently, the as-prepared CeO
2
/CdS heterojunctions were immobilized on aldehyde-functionalized cotton fabric surfaces as composite photocatalysts via "amine-aldehyde" chemical reaction. The surface microstructure and chemical composition of the CeO
2
/CdS decorated cotton fabric (CeO
2
/CdS-CF) were characterized by SEM, FTIR and XPS, respectively. The results showed that CeO
2
/CdS heterojunctions were successfully anchored and uniformly distributed on the surface of cotton fabric. Since the CeO
2
/CdS heterostructure with efficient photo-generated charge transfer and separation, the as-prepared CeO
2
/CdS-CF exhibited excellent photocatalytic activity, degrading MB under simulated sunlight irradiation with a degradation efficiency of 93.8% within 90 min. In addition, the degradation efficiency remained above 90.3% even after five successive degradation cycles, indicating the outstanding stability and recyclability of the obtained CeO
2
/CdS-CF. This work opened up a facile preparation way for the fabrication of durable and recyclable composite photocatalysts, and has a promising application in treating dye contaminated wastewater.
Graphic abstract</description><identifier>ISSN: 0969-0239</identifier><identifier>EISSN: 1572-882X</identifier><identifier>DOI: 10.1007/s10570-021-04203-z</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Aldehydes ; Bioorganic Chemistry ; Catalytic activity ; Ceramics ; Cerium oxides ; Charge transfer ; Chemical composition ; Chemical reactions ; Chemistry ; Chemistry and Materials Science ; Composites ; Cotton ; Cotton fabrics ; Decoration ; Glass ; Heterojunctions ; Heterostructures ; Methylene blue ; Natural Materials ; Organic Chemistry ; Original Research ; Photocatalysis ; Photocatalysts ; Photodegradation ; Physical Chemistry ; Polymer Sciences ; Recyclability ; Sustainable Development ; Wastewater treatment ; X ray photoelectron spectroscopy</subject><ispartof>Cellulose (London), 2021-11, Vol.28 (17), p.11081-11096</ispartof><rights>The Author(s), under exclusive licence to Springer Nature B.V. 2021</rights><rights>The Author(s), under exclusive licence to Springer Nature B.V. 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-2c73b9c5ec388839b1584a7af67c6fbe79755f3f399cf846648dd6d31a954e1d3</citedby><cites>FETCH-LOGICAL-c319t-2c73b9c5ec388839b1584a7af67c6fbe79755f3f399cf846648dd6d31a954e1d3</cites><orcidid>0000-0003-0874-6301</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10570-021-04203-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10570-021-04203-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51297</link.rule.ids></links><search><creatorcontrib>Zou, Rui</creatorcontrib><creatorcontrib>Li, Linhua</creatorcontrib><creatorcontrib>Yang, Lin</creatorcontrib><creatorcontrib>Lan, Jianwu</creatorcontrib><creatorcontrib>Liu, Hongyu</creatorcontrib><creatorcontrib>Dou, Baojie</creatorcontrib><creatorcontrib>Shang, Jiaojiao</creatorcontrib><creatorcontrib>Lin, Shaojian</creatorcontrib><title>CeO2/CdS heterojunction decorated cotton fabric as a recyclable photocatalyst for efficient light driven degradation of methylene blue</title><title>Cellulose (London)</title><addtitle>Cellulose</addtitle><description>In this work, visible light response CeO
2
/CdS decorated cotton fabrics as durable and facile recyclable composite photocatalysts were fabricated for photo-degradation of methylene blue (MB). First of all, amino-functionalized CeO
2
/CdS heterojunctions were synthesized through a fast, efficient and low-cost co-precipitation method. Subsequently, the as-prepared CeO
2
/CdS heterojunctions were immobilized on aldehyde-functionalized cotton fabric surfaces as composite photocatalysts via "amine-aldehyde" chemical reaction. The surface microstructure and chemical composition of the CeO
2
/CdS decorated cotton fabric (CeO
2
/CdS-CF) were characterized by SEM, FTIR and XPS, respectively. The results showed that CeO
2
/CdS heterojunctions were successfully anchored and uniformly distributed on the surface of cotton fabric. Since the CeO
2
/CdS heterostructure with efficient photo-generated charge transfer and separation, the as-prepared CeO
2
/CdS-CF exhibited excellent photocatalytic activity, degrading MB under simulated sunlight irradiation with a degradation efficiency of 93.8% within 90 min. In addition, the degradation efficiency remained above 90.3% even after five successive degradation cycles, indicating the outstanding stability and recyclability of the obtained CeO
2
/CdS-CF. This work opened up a facile preparation way for the fabrication of durable and recyclable composite photocatalysts, and has a promising application in treating dye contaminated wastewater.
Graphic abstract</description><subject>Aldehydes</subject><subject>Bioorganic Chemistry</subject><subject>Catalytic activity</subject><subject>Ceramics</subject><subject>Cerium oxides</subject><subject>Charge transfer</subject><subject>Chemical composition</subject><subject>Chemical reactions</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Composites</subject><subject>Cotton</subject><subject>Cotton fabrics</subject><subject>Decoration</subject><subject>Glass</subject><subject>Heterojunctions</subject><subject>Heterostructures</subject><subject>Methylene blue</subject><subject>Natural Materials</subject><subject>Organic Chemistry</subject><subject>Original Research</subject><subject>Photocatalysis</subject><subject>Photocatalysts</subject><subject>Photodegradation</subject><subject>Physical Chemistry</subject><subject>Polymer Sciences</subject><subject>Recyclability</subject><subject>Sustainable Development</subject><subject>Wastewater treatment</subject><subject>X ray photoelectron spectroscopy</subject><issn>0969-0239</issn><issn>1572-882X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kMtKAzEUhoMoWKsv4CrgemwuM5NkKcUbFLpQwV3IJCftlOmkJqlQH8DndtoK7lwdOOf_vwMfQteU3FJCxCRRUglSEEYLUjLCi68TNKKVYIWU7P0UjYiq1XDm6hxdpLQihCjB6Ah9T2HOJlP3gpeQIYbVtre5DT12YEM0GRy2Iedh4U0TW4tNwgZHsDvbmaYDvFmGHKzJptuljH2IGLxvbQt9xl27WGbsYvsJe-AiGmcO8ODxGvJy10EPuOm2cInOvOkSXP3OMXp7uH-dPhWz-ePz9G5WWE5VLpgVvFG2AsullFw1tJKlEcbXwta-AaFEVXnuuVLWy7KuS-lc7Tg1qiqBOj5GN0fuJoaPLaSsV2Eb--GlZpUUpRSM8SHFjikbQ0oRvN7Edm3iTlOi97710bcefOuDb_01lPixlIZwv4D4h_6n9QOY0IYo</recordid><startdate>20211101</startdate><enddate>20211101</enddate><creator>Zou, Rui</creator><creator>Li, Linhua</creator><creator>Yang, Lin</creator><creator>Lan, Jianwu</creator><creator>Liu, Hongyu</creator><creator>Dou, Baojie</creator><creator>Shang, Jiaojiao</creator><creator>Lin, Shaojian</creator><general>Springer Netherlands</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><orcidid>https://orcid.org/0000-0003-0874-6301</orcidid></search><sort><creationdate>20211101</creationdate><title>CeO2/CdS heterojunction decorated cotton fabric as a recyclable photocatalyst for efficient light driven degradation of methylene blue</title><author>Zou, Rui ; Li, Linhua ; Yang, Lin ; Lan, Jianwu ; Liu, Hongyu ; Dou, Baojie ; Shang, Jiaojiao ; Lin, Shaojian</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-2c73b9c5ec388839b1584a7af67c6fbe79755f3f399cf846648dd6d31a954e1d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Aldehydes</topic><topic>Bioorganic Chemistry</topic><topic>Catalytic activity</topic><topic>Ceramics</topic><topic>Cerium oxides</topic><topic>Charge transfer</topic><topic>Chemical composition</topic><topic>Chemical reactions</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Composites</topic><topic>Cotton</topic><topic>Cotton fabrics</topic><topic>Decoration</topic><topic>Glass</topic><topic>Heterojunctions</topic><topic>Heterostructures</topic><topic>Methylene blue</topic><topic>Natural Materials</topic><topic>Organic Chemistry</topic><topic>Original Research</topic><topic>Photocatalysis</topic><topic>Photocatalysts</topic><topic>Photodegradation</topic><topic>Physical Chemistry</topic><topic>Polymer Sciences</topic><topic>Recyclability</topic><topic>Sustainable Development</topic><topic>Wastewater treatment</topic><topic>X ray photoelectron spectroscopy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zou, Rui</creatorcontrib><creatorcontrib>Li, Linhua</creatorcontrib><creatorcontrib>Yang, Lin</creatorcontrib><creatorcontrib>Lan, Jianwu</creatorcontrib><creatorcontrib>Liu, Hongyu</creatorcontrib><creatorcontrib>Dou, Baojie</creatorcontrib><creatorcontrib>Shang, Jiaojiao</creatorcontrib><creatorcontrib>Lin, Shaojian</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><jtitle>Cellulose (London)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zou, Rui</au><au>Li, Linhua</au><au>Yang, Lin</au><au>Lan, Jianwu</au><au>Liu, Hongyu</au><au>Dou, Baojie</au><au>Shang, Jiaojiao</au><au>Lin, Shaojian</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>CeO2/CdS heterojunction decorated cotton fabric as a recyclable photocatalyst for efficient light driven degradation of methylene blue</atitle><jtitle>Cellulose (London)</jtitle><stitle>Cellulose</stitle><date>2021-11-01</date><risdate>2021</risdate><volume>28</volume><issue>17</issue><spage>11081</spage><epage>11096</epage><pages>11081-11096</pages><issn>0969-0239</issn><eissn>1572-882X</eissn><abstract>In this work, visible light response CeO
2
/CdS decorated cotton fabrics as durable and facile recyclable composite photocatalysts were fabricated for photo-degradation of methylene blue (MB). First of all, amino-functionalized CeO
2
/CdS heterojunctions were synthesized through a fast, efficient and low-cost co-precipitation method. Subsequently, the as-prepared CeO
2
/CdS heterojunctions were immobilized on aldehyde-functionalized cotton fabric surfaces as composite photocatalysts via "amine-aldehyde" chemical reaction. The surface microstructure and chemical composition of the CeO
2
/CdS decorated cotton fabric (CeO
2
/CdS-CF) were characterized by SEM, FTIR and XPS, respectively. The results showed that CeO
2
/CdS heterojunctions were successfully anchored and uniformly distributed on the surface of cotton fabric. Since the CeO
2
/CdS heterostructure with efficient photo-generated charge transfer and separation, the as-prepared CeO
2
/CdS-CF exhibited excellent photocatalytic activity, degrading MB under simulated sunlight irradiation with a degradation efficiency of 93.8% within 90 min. In addition, the degradation efficiency remained above 90.3% even after five successive degradation cycles, indicating the outstanding stability and recyclability of the obtained CeO
2
/CdS-CF. This work opened up a facile preparation way for the fabrication of durable and recyclable composite photocatalysts, and has a promising application in treating dye contaminated wastewater.
Graphic abstract</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><doi>10.1007/s10570-021-04203-z</doi><tpages>16</tpages><orcidid>https://orcid.org/0000-0003-0874-6301</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0969-0239 |
| ispartof | Cellulose (London), 2021-11, Vol.28 (17), p.11081-11096 |
| issn | 0969-0239 1572-882X |
| language | eng |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Aldehydes Bioorganic Chemistry Catalytic activity Ceramics Cerium oxides Charge transfer Chemical composition Chemical reactions Chemistry Chemistry and Materials Science Composites Cotton Cotton fabrics Decoration Glass Heterojunctions Heterostructures Methylene blue Natural Materials Organic Chemistry Original Research Photocatalysis Photocatalysts Photodegradation Physical Chemistry Polymer Sciences Recyclability Sustainable Development Wastewater treatment X ray photoelectron spectroscopy |
| title | CeO2/CdS heterojunction decorated cotton fabric as a recyclable photocatalyst for efficient light driven degradation of methylene blue |
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