Oxidative synthesis of yellow photoluminescent carbon nanoribbons from carbon black
Micrometer long multilayer carbon nanoribbons with high oxygen content and nitrogen doping were obtained from the nitric acid treatment of Black Pearls 2000. The nanoribbons (NRs) exhibited yellow light emission under UV excitation. The oxidation of other grades of carbon black yielded irregular and...
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| Veröffentlicht in: | Carbon (New York) 2021-10, Vol.183, p.495-503 |
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| creator | Khodabakhshi, Saeed Fulvio, Pasquale F. Sousaraei, Ahmad Kiani, Sajad Niu, Yubiao Palmer, Richard E. Kuo, Winson C.H. Rudd, Jennifer Barron, Andrew R. Andreoli, Enrico |
| description | Micrometer long multilayer carbon nanoribbons with high oxygen content and nitrogen doping were obtained from the nitric acid treatment of Black Pearls 2000. The nanoribbons (NRs) exhibited yellow light emission under UV excitation. The oxidation of other grades of carbon black yielded irregular and small graphene oxide fragments or carbon quantum dots instead. Remarkably, the familiar and straightforward treatment of carbon materials with nitric acid reemerges as a powerful tool for the synthesis of technology-relevant carbon nanoribbons, and unlocking the potential of such straighforward oxidation chemistry applied to inexpensive and commercially available carbon black.
[Display omitted]
•Carbon nanoribbons are uniquely obtained from oxidation of carbon black (CB) BP2000.•Oxidation of Vulcan, Monarch and Acetylene Black grades yield graphene oxide sheets and carbon dots.•Nanostructure depends on CB surface area, amount of amorphous carbon and size of basic structural units.•Nanoribbons have yellow emission modulated by nitrogen doping and to oxygen defects. |
| doi_str_mv | 10.1016/j.carbon.2021.07.032 |
| format | Article |
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[Display omitted]
•Carbon nanoribbons are uniquely obtained from oxidation of carbon black (CB) BP2000.•Oxidation of Vulcan, Monarch and Acetylene Black grades yield graphene oxide sheets and carbon dots.•Nanostructure depends on CB surface area, amount of amorphous carbon and size of basic structural units.•Nanoribbons have yellow emission modulated by nitrogen doping and to oxygen defects.</description><identifier>ISSN: 0008-6223</identifier><identifier>EISSN: 1873-3891</identifier><identifier>DOI: 10.1016/j.carbon.2021.07.032</identifier><language>eng</language><publisher>New York: Elsevier Ltd</publisher><subject>Black pearls 2000 ; Carbon ; Carbon black ; Carbon nanoribbons ; Chemical synthesis ; Graphene ; Light emission ; Multilayers ; Nanoribbons ; Nanotubes ; Nitric acid ; Nitrogen doping ; Oxidation ; Oxygen content ; Photoluminescence ; Quantum dots</subject><ispartof>Carbon (New York), 2021-10, Vol.183, p.495-503</ispartof><rights>2021 Elsevier Ltd</rights><rights>Copyright Elsevier BV Oct 15, 2021</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c380t-654cddc7fd308fe84ed5190a74eb3ac6b76a23bc70b28b1884b441a90cd13fe53</citedby><cites>FETCH-LOGICAL-c380t-654cddc7fd308fe84ed5190a74eb3ac6b76a23bc70b28b1884b441a90cd13fe53</cites><orcidid>0000-0002-8096-6854 ; 0000-0002-5209-477X ; 0000-0002-1207-2314 ; 0000-0001-7580-727X ; 0000-0003-2821-7909</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.carbon.2021.07.032$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids></links><search><creatorcontrib>Khodabakhshi, Saeed</creatorcontrib><creatorcontrib>Fulvio, Pasquale F.</creatorcontrib><creatorcontrib>Sousaraei, Ahmad</creatorcontrib><creatorcontrib>Kiani, Sajad</creatorcontrib><creatorcontrib>Niu, Yubiao</creatorcontrib><creatorcontrib>Palmer, Richard E.</creatorcontrib><creatorcontrib>Kuo, Winson C.H.</creatorcontrib><creatorcontrib>Rudd, Jennifer</creatorcontrib><creatorcontrib>Barron, Andrew R.</creatorcontrib><creatorcontrib>Andreoli, Enrico</creatorcontrib><title>Oxidative synthesis of yellow photoluminescent carbon nanoribbons from carbon black</title><title>Carbon (New York)</title><description>Micrometer long multilayer carbon nanoribbons with high oxygen content and nitrogen doping were obtained from the nitric acid treatment of Black Pearls 2000. The nanoribbons (NRs) exhibited yellow light emission under UV excitation. The oxidation of other grades of carbon black yielded irregular and small graphene oxide fragments or carbon quantum dots instead. Remarkably, the familiar and straightforward treatment of carbon materials with nitric acid reemerges as a powerful tool for the synthesis of technology-relevant carbon nanoribbons, and unlocking the potential of such straighforward oxidation chemistry applied to inexpensive and commercially available carbon black.
[Display omitted]
•Carbon nanoribbons are uniquely obtained from oxidation of carbon black (CB) BP2000.•Oxidation of Vulcan, Monarch and Acetylene Black grades yield graphene oxide sheets and carbon dots.•Nanostructure depends on CB surface area, amount of amorphous carbon and size of basic structural units.•Nanoribbons have yellow emission modulated by nitrogen doping and to oxygen defects.</description><subject>Black pearls 2000</subject><subject>Carbon</subject><subject>Carbon black</subject><subject>Carbon nanoribbons</subject><subject>Chemical synthesis</subject><subject>Graphene</subject><subject>Light emission</subject><subject>Multilayers</subject><subject>Nanoribbons</subject><subject>Nanotubes</subject><subject>Nitric acid</subject><subject>Nitrogen doping</subject><subject>Oxidation</subject><subject>Oxygen content</subject><subject>Photoluminescence</subject><subject>Quantum dots</subject><issn>0008-6223</issn><issn>1873-3891</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNp9UMlOwzAQtRBIlMIfcIjEOcFbYveChCo2qVIPwNnyMlFd0rjYaaF_j6vAldMsesvMQ-ia4Ipg0tyuK6ujCX1FMSUVFhVm9ARNiBSsZHJGTtEEYyzLhlJ2ji5SWueRS8In6HX57Z0e_B6KdOiHFSSfitAWB-i68FVsV2EI3W7je0gW-qEYjYpe9yF6k9tUtDFs_vam0_bjEp21uktw9Vun6P3x4W3-XC6WTy_z-0VpmcRD2dTcOmdF6xiWLUgOriYzrAUHw7RtjGg0ZcYKbKg0REpuOCd6hq0jrIWaTdHNqLuN4XMHaVDrsIt9tlS0ljkZQrjIKD6ibAwpRWjVNvqNjgdFsDrGp9ZqvF4d41NYqBxfpt2NNMgf7D1ElayH3oLzEeygXPD_C_wAZ818Kw</recordid><startdate>20211015</startdate><enddate>20211015</enddate><creator>Khodabakhshi, Saeed</creator><creator>Fulvio, Pasquale F.</creator><creator>Sousaraei, Ahmad</creator><creator>Kiani, Sajad</creator><creator>Niu, Yubiao</creator><creator>Palmer, Richard E.</creator><creator>Kuo, Winson C.H.</creator><creator>Rudd, Jennifer</creator><creator>Barron, Andrew R.</creator><creator>Andreoli, Enrico</creator><general>Elsevier Ltd</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope><orcidid>https://orcid.org/0000-0002-8096-6854</orcidid><orcidid>https://orcid.org/0000-0002-5209-477X</orcidid><orcidid>https://orcid.org/0000-0002-1207-2314</orcidid><orcidid>https://orcid.org/0000-0001-7580-727X</orcidid><orcidid>https://orcid.org/0000-0003-2821-7909</orcidid></search><sort><creationdate>20211015</creationdate><title>Oxidative synthesis of yellow photoluminescent carbon nanoribbons from carbon black</title><author>Khodabakhshi, Saeed ; 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The nanoribbons (NRs) exhibited yellow light emission under UV excitation. The oxidation of other grades of carbon black yielded irregular and small graphene oxide fragments or carbon quantum dots instead. Remarkably, the familiar and straightforward treatment of carbon materials with nitric acid reemerges as a powerful tool for the synthesis of technology-relevant carbon nanoribbons, and unlocking the potential of such straighforward oxidation chemistry applied to inexpensive and commercially available carbon black.
[Display omitted]
•Carbon nanoribbons are uniquely obtained from oxidation of carbon black (CB) BP2000.•Oxidation of Vulcan, Monarch and Acetylene Black grades yield graphene oxide sheets and carbon dots.•Nanostructure depends on CB surface area, amount of amorphous carbon and size of basic structural units.•Nanoribbons have yellow emission modulated by nitrogen doping and to oxygen defects.</abstract><cop>New York</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.carbon.2021.07.032</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0002-8096-6854</orcidid><orcidid>https://orcid.org/0000-0002-5209-477X</orcidid><orcidid>https://orcid.org/0000-0002-1207-2314</orcidid><orcidid>https://orcid.org/0000-0001-7580-727X</orcidid><orcidid>https://orcid.org/0000-0003-2821-7909</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Black pearls 2000 Carbon Carbon black Carbon nanoribbons Chemical synthesis Graphene Light emission Multilayers Nanoribbons Nanotubes Nitric acid Nitrogen doping Oxidation Oxygen content Photoluminescence Quantum dots |
| title | Oxidative synthesis of yellow photoluminescent carbon nanoribbons from carbon black |
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