Adsorption of EDCs on Reclaimed Water-Irrigated Soils: A Comparative Analysis of a Branched Nonylphenol, Nonylphenol and Bisphenol A
Nonylphenol (NP) and bisphenol A (BPA) are two typical endocrine disrupter chemicals (EDCs) in reclaimed water. In this study, the adsorptions of NP, a branched NP (NP7) and BPA on reclaimed water-irrigated soils were studied by isothermal experiments, and the different environmental factors on thei...
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| Veröffentlicht in: | Water (Basel) 2021-09, Vol.13 (18), p.2532 |
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| creator | Wang, Shiyu Zhang, Junnan Zhou, Fada Liang, Cunzhen He, Liao Jiao, Wentao Wu, Wenyong |
| description | Nonylphenol (NP) and bisphenol A (BPA) are two typical endocrine disrupter chemicals (EDCs) in reclaimed water. In this study, the adsorptions of NP, a branched NP (NP7) and BPA on reclaimed water-irrigated soils were studied by isothermal experiments, and the different environmental factors on their adsorptions were investigated. The results showed that the adsorptions of NP and NP7 on soils conformed to the Linear model, and the adsorption of BPA conformed to the Freundlich model. The adsorptions of NP, NP7 and BPA on soils decreased with increasing temperatures and pHs. Adsorption equilibrium constant (Kd or Kf) were maximum at pH = 3, temperature 25 °C and As(III)-soil, respectively. The adsorption capacity of NP, NP7 and BPA to soils under different cation valence were as follows: neutrally > divalent cations > mono-cations. Kd of NP7 on soil was less than that of NP under different pH and temperatures, while under different cation concentrations it was the inverse. Fourier Transform Infrared Spectrometer (FTIR) analysis showed alkyl chains of NP and BPA seemed to form van der Waals interactions with the cavity of soil. Results of this study will provide further comprehensive fundamental data for human health risk assessment of NP and BPA in soil. |
| doi_str_mv | 10.3390/w13182532 |
| format | Article |
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In this study, the adsorptions of NP, a branched NP (NP7) and BPA on reclaimed water-irrigated soils were studied by isothermal experiments, and the different environmental factors on their adsorptions were investigated. The results showed that the adsorptions of NP and NP7 on soils conformed to the Linear model, and the adsorption of BPA conformed to the Freundlich model. The adsorptions of NP, NP7 and BPA on soils decreased with increasing temperatures and pHs. Adsorption equilibrium constant (Kd or Kf) were maximum at pH = 3, temperature 25 °C and As(III)-soil, respectively. The adsorption capacity of NP, NP7 and BPA to soils under different cation valence were as follows: neutrally > divalent cations > mono-cations. Kd of NP7 on soil was less than that of NP under different pH and temperatures, while under different cation concentrations it was the inverse. Fourier Transform Infrared Spectrometer (FTIR) analysis showed alkyl chains of NP and BPA seemed to form van der Waals interactions with the cavity of soil. Results of this study will provide further comprehensive fundamental data for human health risk assessment of NP and BPA in soil.</description><identifier>ISSN: 2073-4441</identifier><identifier>EISSN: 2073-4441</identifier><identifier>DOI: 10.3390/w13182532</identifier><language>eng</language><publisher>Basel: MDPI AG</publisher><subject>Adsorption ; Bisphenol A ; Carbon ; Cations ; Comparative analysis ; Divalent cations ; Endocrine disruptors ; Environmental factors ; Equilibrium ; Experiments ; Fourier analysis ; Fourier transforms ; FTIR spectrometers ; Groundwater ; Health risks ; Infrared analysis ; Infrared spectrometers ; Pollutants ; Reclaimed water ; Risk assessment ; Sewage irrigation ; Soil analysis ; Soil temperature ; Soil water ; Soils</subject><ispartof>Water (Basel), 2021-09, Vol.13 (18), p.2532</ispartof><rights>2021 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c292t-e7fabe772d42b7f75488f79fad32671e960280cdbc2d9f6c5a4fd3c545ab07663</citedby><cites>FETCH-LOGICAL-c292t-e7fabe772d42b7f75488f79fad32671e960280cdbc2d9f6c5a4fd3c545ab07663</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,781,785,27926,27927</link.rule.ids></links><search><creatorcontrib>Wang, Shiyu</creatorcontrib><creatorcontrib>Zhang, Junnan</creatorcontrib><creatorcontrib>Zhou, Fada</creatorcontrib><creatorcontrib>Liang, Cunzhen</creatorcontrib><creatorcontrib>He, Liao</creatorcontrib><creatorcontrib>Jiao, Wentao</creatorcontrib><creatorcontrib>Wu, Wenyong</creatorcontrib><title>Adsorption of EDCs on Reclaimed Water-Irrigated Soils: A Comparative Analysis of a Branched Nonylphenol, Nonylphenol and Bisphenol A</title><title>Water (Basel)</title><description>Nonylphenol (NP) and bisphenol A (BPA) are two typical endocrine disrupter chemicals (EDCs) in reclaimed water. In this study, the adsorptions of NP, a branched NP (NP7) and BPA on reclaimed water-irrigated soils were studied by isothermal experiments, and the different environmental factors on their adsorptions were investigated. The results showed that the adsorptions of NP and NP7 on soils conformed to the Linear model, and the adsorption of BPA conformed to the Freundlich model. The adsorptions of NP, NP7 and BPA on soils decreased with increasing temperatures and pHs. Adsorption equilibrium constant (Kd or Kf) were maximum at pH = 3, temperature 25 °C and As(III)-soil, respectively. The adsorption capacity of NP, NP7 and BPA to soils under different cation valence were as follows: neutrally > divalent cations > mono-cations. Kd of NP7 on soil was less than that of NP under different pH and temperatures, while under different cation concentrations it was the inverse. Fourier Transform Infrared Spectrometer (FTIR) analysis showed alkyl chains of NP and BPA seemed to form van der Waals interactions with the cavity of soil. Results of this study will provide further comprehensive fundamental data for human health risk assessment of NP and BPA in soil.</description><subject>Adsorption</subject><subject>Bisphenol A</subject><subject>Carbon</subject><subject>Cations</subject><subject>Comparative analysis</subject><subject>Divalent cations</subject><subject>Endocrine disruptors</subject><subject>Environmental factors</subject><subject>Equilibrium</subject><subject>Experiments</subject><subject>Fourier analysis</subject><subject>Fourier transforms</subject><subject>FTIR spectrometers</subject><subject>Groundwater</subject><subject>Health risks</subject><subject>Infrared analysis</subject><subject>Infrared spectrometers</subject><subject>Pollutants</subject><subject>Reclaimed water</subject><subject>Risk assessment</subject><subject>Sewage irrigation</subject><subject>Soil analysis</subject><subject>Soil temperature</subject><subject>Soil water</subject><subject>Soils</subject><issn>2073-4441</issn><issn>2073-4441</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpNkEtLw0AUhQdRsNQu_AcDrgSjk3lkEndprFooCj5wGSbzsFPSTJxJlez94aa0SO_mnAOHw-UD4DxG14Rk6OYnJnGKGcFHYIQRJxGlND4-8KdgEsIKDUezNGVoBH5zFZxvO-sa6Ayc3RUBDvZFy1rYtVbwQ3TaR3Pv7efgFHx1tg63MIeFW7fCi85-a5g3ou6DDdsJAadeNHI5dJ9c09ftUjeuvjoMUDQKTm3Yp_wMnBhRBz3Z6xi838_eisdo8fwwL_JFJHGGu0hzIyrNOVYUV9xwRtPU8MwIRXDCY50lCKdIqkpilZlEMkGNIpJRJirEk4SMwcVut_Xua6NDV67cxg-_hxIznjDC0oHUGFzuWtK7ELw2ZevtWvi-jFG55Vz-cyZ_9Bhv0g</recordid><startdate>20210901</startdate><enddate>20210901</enddate><creator>Wang, Shiyu</creator><creator>Zhang, Junnan</creator><creator>Zhou, Fada</creator><creator>Liang, Cunzhen</creator><creator>He, Liao</creator><creator>Jiao, Wentao</creator><creator>Wu, Wenyong</creator><general>MDPI AG</general><scope>AAYXX</scope><scope>CITATION</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope></search><sort><creationdate>20210901</creationdate><title>Adsorption of EDCs on Reclaimed Water-Irrigated Soils: A Comparative Analysis of a Branched Nonylphenol, Nonylphenol and Bisphenol A</title><author>Wang, Shiyu ; Zhang, Junnan ; Zhou, Fada ; Liang, Cunzhen ; He, Liao ; Jiao, Wentao ; Wu, Wenyong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c292t-e7fabe772d42b7f75488f79fad32671e960280cdbc2d9f6c5a4fd3c545ab07663</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Adsorption</topic><topic>Bisphenol A</topic><topic>Carbon</topic><topic>Cations</topic><topic>Comparative analysis</topic><topic>Divalent cations</topic><topic>Endocrine disruptors</topic><topic>Environmental factors</topic><topic>Equilibrium</topic><topic>Experiments</topic><topic>Fourier analysis</topic><topic>Fourier transforms</topic><topic>FTIR spectrometers</topic><topic>Groundwater</topic><topic>Health risks</topic><topic>Infrared analysis</topic><topic>Infrared spectrometers</topic><topic>Pollutants</topic><topic>Reclaimed water</topic><topic>Risk assessment</topic><topic>Sewage irrigation</topic><topic>Soil analysis</topic><topic>Soil temperature</topic><topic>Soil water</topic><topic>Soils</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Shiyu</creatorcontrib><creatorcontrib>Zhang, Junnan</creatorcontrib><creatorcontrib>Zhou, Fada</creatorcontrib><creatorcontrib>Liang, Cunzhen</creatorcontrib><creatorcontrib>He, Liao</creatorcontrib><creatorcontrib>Jiao, Wentao</creatorcontrib><creatorcontrib>Wu, Wenyong</creatorcontrib><collection>CrossRef</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>Access via ProQuest (Open Access)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><jtitle>Water (Basel)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Shiyu</au><au>Zhang, Junnan</au><au>Zhou, Fada</au><au>Liang, Cunzhen</au><au>He, Liao</au><au>Jiao, Wentao</au><au>Wu, Wenyong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Adsorption of EDCs on Reclaimed Water-Irrigated Soils: A Comparative Analysis of a Branched Nonylphenol, Nonylphenol and Bisphenol A</atitle><jtitle>Water (Basel)</jtitle><date>2021-09-01</date><risdate>2021</risdate><volume>13</volume><issue>18</issue><spage>2532</spage><pages>2532-</pages><issn>2073-4441</issn><eissn>2073-4441</eissn><abstract>Nonylphenol (NP) and bisphenol A (BPA) are two typical endocrine disrupter chemicals (EDCs) in reclaimed water. In this study, the adsorptions of NP, a branched NP (NP7) and BPA on reclaimed water-irrigated soils were studied by isothermal experiments, and the different environmental factors on their adsorptions were investigated. The results showed that the adsorptions of NP and NP7 on soils conformed to the Linear model, and the adsorption of BPA conformed to the Freundlich model. The adsorptions of NP, NP7 and BPA on soils decreased with increasing temperatures and pHs. Adsorption equilibrium constant (Kd or Kf) were maximum at pH = 3, temperature 25 °C and As(III)-soil, respectively. The adsorption capacity of NP, NP7 and BPA to soils under different cation valence were as follows: neutrally > divalent cations > mono-cations. Kd of NP7 on soil was less than that of NP under different pH and temperatures, while under different cation concentrations it was the inverse. Fourier Transform Infrared Spectrometer (FTIR) analysis showed alkyl chains of NP and BPA seemed to form van der Waals interactions with the cavity of soil. Results of this study will provide further comprehensive fundamental data for human health risk assessment of NP and BPA in soil.</abstract><cop>Basel</cop><pub>MDPI AG</pub><doi>10.3390/w13182532</doi><oa>free_for_read</oa></addata></record> |
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| subjects | Adsorption Bisphenol A Carbon Cations Comparative analysis Divalent cations Endocrine disruptors Environmental factors Equilibrium Experiments Fourier analysis Fourier transforms FTIR spectrometers Groundwater Health risks Infrared analysis Infrared spectrometers Pollutants Reclaimed water Risk assessment Sewage irrigation Soil analysis Soil temperature Soil water Soils |
| title | Adsorption of EDCs on Reclaimed Water-Irrigated Soils: A Comparative Analysis of a Branched Nonylphenol, Nonylphenol and Bisphenol A |
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