Nuclear forensics methodology identifies legacy plutonium from the Manhattan Project

The X-10 nuclear reactor was built at the Clinton Engineering Works in Oak Ridge, Tennessee, USA, as the world’s first Pu production reactor. Operation commenced in November 1943, producing Pu on the gram-scale for the first time. A 61.1 mg sample of 239 Pu has been identified at Los Alamos National...

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Veröffentlicht in:Journal of radioanalytical and nuclear chemistry 2021-10, Vol.330 (1), p.57-65
Hauptverfasser: Glennon, Kevin J., Bond, Evelyn M., Bredeweg, Todd A., Chirayath, Sunil S., O’Neal, Patrick J., Folden, Charles M.
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container_issue 1
container_start_page 57
container_title Journal of radioanalytical and nuclear chemistry
container_volume 330
creator Glennon, Kevin J.
Bond, Evelyn M.
Bredeweg, Todd A.
Chirayath, Sunil S.
O’Neal, Patrick J.
Folden, Charles M.
description The X-10 nuclear reactor was built at the Clinton Engineering Works in Oak Ridge, Tennessee, USA, as the world’s first Pu production reactor. Operation commenced in November 1943, producing Pu on the gram-scale for the first time. A 61.1 mg sample of 239 Pu has been identified at Los Alamos National Laboratory containing multiple forensic signatures consistent with production from the X-10 reactor in early 1944, when the first samples of reactor-produced Pu were shipped from X-10 to Los Alamos. Our nuclear forensics investigation included Pu isotopic analysis, chronometry, X-10 reactor physics simulations, and trace metal analyses. This historic sample has been determined to be among the oldest reactor-produced Pu reported in the literature and is among the first 1.4 kg of Pu ever produced.
doi_str_mv 10.1007/s10967-021-07924-4
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subjects Analysis
Chemistry
Chemistry and Materials Science
Diagnostic Radiology
Forensic sciences
Hadrons
Heavy Ions
Inorganic Chemistry
Measuring instruments
Methods
Nuclear Chemistry
Nuclear facilities
Nuclear Physics
Nuclear reactors
Physical Chemistry
Plutonium
Reactor physics
Research facilities
Trace metals
title Nuclear forensics methodology identifies legacy plutonium from the Manhattan Project
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