Nano-crystalline powders and microwave dielectric properties of Zr0.8Sn0.2TiO4 ceramics derived using deep eutectic solvents
Choline chloride-malonic acid deep eutectic solvent (Cm-DES) was employed to synthesize Zr 0.8 Sn 0.2 TiO 4 nano-powders using Zr(CH 3 COO) 4 , SnCl 2 ∙2H 2 O, and Ti(OCH 3 CH 3 ) 4 as raw materials. The Zr 0.8 Sn 0.2 TiO 4 nano-powder with the mean grain size of 10.7 nm was obtained at 450 °C, sign...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2021-09, Vol.32 (18), p.23317-23324 |
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| container_title | Journal of materials science. Materials in electronics |
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| creator | Wang, Qi-feng Gu, Yong-jun Li, Qian Huang, Jin-liang Chen, Min Gao, Shun Kim, Bok-hee |
| description | Choline chloride-malonic acid deep eutectic solvent (Cm-DES) was employed to synthesize Zr
0.8
Sn
0.2
TiO
4
nano-powders using Zr(CH
3
COO)
4
, SnCl
2
∙2H
2
O, and Ti(OCH
3
CH
3
)
4
as raw materials. The Zr
0.8
Sn
0.2
TiO
4
nano-powder with the mean grain size of 10.7 nm was obtained at 450 °C, significantly lower than that by conventional mixed oxide routes. Meantime, the densification of Zr
0.8
Sn
0.2
TiO
4
ceramics was improved using the as-synthesized powder. The Zr
0.8
Sn
0.2
TiO
4
ceramics with relative density of 96.8 % were obtained at 1350 °C and it exhibited good microwave dielectric properties (ε
r
= 37.8, Q
f
= 42,600 GHz, and τ
f
= − 4.1 ppm/°C). These results show that Cm-DES route is suitable for the synthesis of Zr
0.8
Sn
0.2
TiO
4
nano-powders, is beneficial to the low-temperature firing of Zr
0.8
Sn
0.2
TiO
4
ceramics, and helps reduce energy consumption and time costs. |
| doi_str_mv | 10.1007/s10854-021-06816-3 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2572076576</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2572076576</sourcerecordid><originalsourceid>FETCH-LOGICAL-c363t-86423e2325800f06fd3d09b67d75500f1ab0ec6957dfea44ab1b62aa96073ed73</originalsourceid><addsrcrecordid>eNp9kE9LAzEQxYMoWKtfwFPAc-ok2STboxT_QdGDFcRLSDezJbLursm2peCHN1rBm6dhhvd-M_MIOecw4QDmMnEoVcFAcAa65JrJAzLiykhWlOLlkIxgqgwrlBDH5CSlNwDQhSxH5PPBtR2r4i4NrmlCi7Tvth5joq719D1Usdu6DVIfsMFqiKGifex6jEPARLuavkaYlE8tTMQiPBa0wuiyK9HMCBv0dJ1Cu8od9hTXQ0ZkQuqaDbZDOiVHtWsSnv3WMXm-uV7M7tj88fZ-djVnldRyYKUuhEQhhSoBatC1lx6mS228USpPuFsCVjp_6Gt0ReGWfKmFc1MNRqI3ckwu9tx8-sca02DfunVs80orlBFgtDI6q8RelX9OKWJt-xjeXdxZDvY7ZbtP2eaU7U_KVmaT3JtSFrcrjH_of1xfgsOBAw</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2572076576</pqid></control><display><type>article</type><title>Nano-crystalline powders and microwave dielectric properties of Zr0.8Sn0.2TiO4 ceramics derived using deep eutectic solvents</title><source>SpringerLink Journals - AutoHoldings</source><creator>Wang, Qi-feng ; Gu, Yong-jun ; Li, Qian ; Huang, Jin-liang ; Chen, Min ; Gao, Shun ; Kim, Bok-hee</creator><creatorcontrib>Wang, Qi-feng ; Gu, Yong-jun ; Li, Qian ; Huang, Jin-liang ; Chen, Min ; Gao, Shun ; Kim, Bok-hee</creatorcontrib><description>Choline chloride-malonic acid deep eutectic solvent (Cm-DES) was employed to synthesize Zr
0.8
Sn
0.2
TiO
4
nano-powders using Zr(CH
3
COO)
4
, SnCl
2
∙2H
2
O, and Ti(OCH
3
CH
3
)
4
as raw materials. The Zr
0.8
Sn
0.2
TiO
4
nano-powder with the mean grain size of 10.7 nm was obtained at 450 °C, significantly lower than that by conventional mixed oxide routes. Meantime, the densification of Zr
0.8
Sn
0.2
TiO
4
ceramics was improved using the as-synthesized powder. The Zr
0.8
Sn
0.2
TiO
4
ceramics with relative density of 96.8 % were obtained at 1350 °C and it exhibited good microwave dielectric properties (ε
r
= 37.8, Q
f
= 42,600 GHz, and τ
f
= − 4.1 ppm/°C). These results show that Cm-DES route is suitable for the synthesis of Zr
0.8
Sn
0.2
TiO
4
nano-powders, is beneficial to the low-temperature firing of Zr
0.8
Sn
0.2
TiO
4
ceramics, and helps reduce energy consumption and time costs.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-021-06816-3</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Ceramic powders ; Ceramics ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Choline ; Densification ; Dielectric properties ; Energy consumption ; Energy costs ; Grain size ; Low temperature ; Materials Science ; Optical and Electronic Materials ; Raw materials ; Solvents ; Synthesis ; Zirconium</subject><ispartof>Journal of materials science. Materials in electronics, 2021-09, Vol.32 (18), p.23317-23324</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c363t-86423e2325800f06fd3d09b67d75500f1ab0ec6957dfea44ab1b62aa96073ed73</citedby><cites>FETCH-LOGICAL-c363t-86423e2325800f06fd3d09b67d75500f1ab0ec6957dfea44ab1b62aa96073ed73</cites><orcidid>0000-0002-4193-4737</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-021-06816-3$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-021-06816-3$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,778,782,27907,27908,41471,42540,51302</link.rule.ids></links><search><creatorcontrib>Wang, Qi-feng</creatorcontrib><creatorcontrib>Gu, Yong-jun</creatorcontrib><creatorcontrib>Li, Qian</creatorcontrib><creatorcontrib>Huang, Jin-liang</creatorcontrib><creatorcontrib>Chen, Min</creatorcontrib><creatorcontrib>Gao, Shun</creatorcontrib><creatorcontrib>Kim, Bok-hee</creatorcontrib><title>Nano-crystalline powders and microwave dielectric properties of Zr0.8Sn0.2TiO4 ceramics derived using deep eutectic solvents</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>Choline chloride-malonic acid deep eutectic solvent (Cm-DES) was employed to synthesize Zr
0.8
Sn
0.2
TiO
4
nano-powders using Zr(CH
3
COO)
4
, SnCl
2
∙2H
2
O, and Ti(OCH
3
CH
3
)
4
as raw materials. The Zr
0.8
Sn
0.2
TiO
4
nano-powder with the mean grain size of 10.7 nm was obtained at 450 °C, significantly lower than that by conventional mixed oxide routes. Meantime, the densification of Zr
0.8
Sn
0.2
TiO
4
ceramics was improved using the as-synthesized powder. The Zr
0.8
Sn
0.2
TiO
4
ceramics with relative density of 96.8 % were obtained at 1350 °C and it exhibited good microwave dielectric properties (ε
r
= 37.8, Q
f
= 42,600 GHz, and τ
f
= − 4.1 ppm/°C). These results show that Cm-DES route is suitable for the synthesis of Zr
0.8
Sn
0.2
TiO
4
nano-powders, is beneficial to the low-temperature firing of Zr
0.8
Sn
0.2
TiO
4
ceramics, and helps reduce energy consumption and time costs.</description><subject>Ceramic powders</subject><subject>Ceramics</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Choline</subject><subject>Densification</subject><subject>Dielectric properties</subject><subject>Energy consumption</subject><subject>Energy costs</subject><subject>Grain size</subject><subject>Low temperature</subject><subject>Materials Science</subject><subject>Optical and Electronic Materials</subject><subject>Raw materials</subject><subject>Solvents</subject><subject>Synthesis</subject><subject>Zirconium</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kE9LAzEQxYMoWKtfwFPAc-ok2STboxT_QdGDFcRLSDezJbLursm2peCHN1rBm6dhhvd-M_MIOecw4QDmMnEoVcFAcAa65JrJAzLiykhWlOLlkIxgqgwrlBDH5CSlNwDQhSxH5PPBtR2r4i4NrmlCi7Tvth5joq719D1Usdu6DVIfsMFqiKGifex6jEPARLuavkaYlE8tTMQiPBa0wuiyK9HMCBv0dJ1Cu8od9hTXQ0ZkQuqaDbZDOiVHtWsSnv3WMXm-uV7M7tj88fZ-djVnldRyYKUuhEQhhSoBatC1lx6mS228USpPuFsCVjp_6Gt0ReGWfKmFc1MNRqI3ckwu9tx8-sca02DfunVs80orlBFgtDI6q8RelX9OKWJt-xjeXdxZDvY7ZbtP2eaU7U_KVmaT3JtSFrcrjH_of1xfgsOBAw</recordid><startdate>20210901</startdate><enddate>20210901</enddate><creator>Wang, Qi-feng</creator><creator>Gu, Yong-jun</creator><creator>Li, Qian</creator><creator>Huang, Jin-liang</creator><creator>Chen, Min</creator><creator>Gao, Shun</creator><creator>Kim, Bok-hee</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0002-4193-4737</orcidid></search><sort><creationdate>20210901</creationdate><title>Nano-crystalline powders and microwave dielectric properties of Zr0.8Sn0.2TiO4 ceramics derived using deep eutectic solvents</title><author>Wang, Qi-feng ; Gu, Yong-jun ; Li, Qian ; Huang, Jin-liang ; Chen, Min ; Gao, Shun ; Kim, Bok-hee</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c363t-86423e2325800f06fd3d09b67d75500f1ab0ec6957dfea44ab1b62aa96073ed73</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Ceramic powders</topic><topic>Ceramics</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Choline</topic><topic>Densification</topic><topic>Dielectric properties</topic><topic>Energy consumption</topic><topic>Energy costs</topic><topic>Grain size</topic><topic>Low temperature</topic><topic>Materials Science</topic><topic>Optical and Electronic Materials</topic><topic>Raw materials</topic><topic>Solvents</topic><topic>Synthesis</topic><topic>Zirconium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Qi-feng</creatorcontrib><creatorcontrib>Gu, Yong-jun</creatorcontrib><creatorcontrib>Li, Qian</creatorcontrib><creatorcontrib>Huang, Jin-liang</creatorcontrib><creatorcontrib>Chen, Min</creatorcontrib><creatorcontrib>Gao, Shun</creatorcontrib><creatorcontrib>Kim, Bok-hee</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Qi-feng</au><au>Gu, Yong-jun</au><au>Li, Qian</au><au>Huang, Jin-liang</au><au>Chen, Min</au><au>Gao, Shun</au><au>Kim, Bok-hee</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Nano-crystalline powders and microwave dielectric properties of Zr0.8Sn0.2TiO4 ceramics derived using deep eutectic solvents</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2021-09-01</date><risdate>2021</risdate><volume>32</volume><issue>18</issue><spage>23317</spage><epage>23324</epage><pages>23317-23324</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>Choline chloride-malonic acid deep eutectic solvent (Cm-DES) was employed to synthesize Zr
0.8
Sn
0.2
TiO
4
nano-powders using Zr(CH
3
COO)
4
, SnCl
2
∙2H
2
O, and Ti(OCH
3
CH
3
)
4
as raw materials. The Zr
0.8
Sn
0.2
TiO
4
nano-powder with the mean grain size of 10.7 nm was obtained at 450 °C, significantly lower than that by conventional mixed oxide routes. Meantime, the densification of Zr
0.8
Sn
0.2
TiO
4
ceramics was improved using the as-synthesized powder. The Zr
0.8
Sn
0.2
TiO
4
ceramics with relative density of 96.8 % were obtained at 1350 °C and it exhibited good microwave dielectric properties (ε
r
= 37.8, Q
f
= 42,600 GHz, and τ
f
= − 4.1 ppm/°C). These results show that Cm-DES route is suitable for the synthesis of Zr
0.8
Sn
0.2
TiO
4
nano-powders, is beneficial to the low-temperature firing of Zr
0.8
Sn
0.2
TiO
4
ceramics, and helps reduce energy consumption and time costs.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-021-06816-3</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-4193-4737</orcidid><oa>free_for_read</oa></addata></record> |
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| ispartof | Journal of materials science. Materials in electronics, 2021-09, Vol.32 (18), p.23317-23324 |
| issn | 0957-4522 1573-482X |
| language | eng |
| recordid | cdi_proquest_journals_2572076576 |
| source | SpringerLink Journals - AutoHoldings |
| subjects | Ceramic powders Ceramics Characterization and Evaluation of Materials Chemistry and Materials Science Choline Densification Dielectric properties Energy consumption Energy costs Grain size Low temperature Materials Science Optical and Electronic Materials Raw materials Solvents Synthesis Zirconium |
| title | Nano-crystalline powders and microwave dielectric properties of Zr0.8Sn0.2TiO4 ceramics derived using deep eutectic solvents |
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