Determining the origin and fate of nitrate in the Nanyang Basin, Central China, using environmental isotopes and the Bayesian mixing model
Identifying sources of nitrate contamination has been a long-term challenge in areas with different land uses. We investigated the biogeochemical processes and quantified the contribution of potential nitrate sources in the Nanyang Basin, the source area of the South to North Water Diversion Project...
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| Veröffentlicht in: | Environmental science and pollution research international 2021-09, Vol.28 (35), p.48343-48361 |
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| creator | Cao, Shengwei Fei, Yuhong Tian, Xia Cui, Xiangxiang Zhang, Xueqing Yuan, Ruoxi Li, Yasong |
| description | Identifying sources of nitrate contamination has been a long-term challenge in areas with different land uses. We investigated the biogeochemical processes and quantified the contribution of potential nitrate sources in the Nanyang Basin, the source area of the South to North Water Diversion Project in China. Hydrogeochemical characteristics, the dual-isotope method (δ
15
N-NO
3
−
and δ
18
O-NO
3
−
), and the Bayesian mixing model (SIAR) were combined. The results for 160 samples indicated that mean nitrate concentrations of residential area (162.83 mg L
−1
) and farmland (75.71 mg L
−1
) were higher compared with those of surface water (16.15 mg L
−1
) and forest (36.25 mg L
−1
). Hydrochemical facies and molar ratios of major ions indicated that the natural environment was greatly impacted by anthropogenic activities. Nitrification, ammonium volatilization, and mixing effects were the dominant processes in nitrogen transformation. The contributions of different sources to nitrate contamination were 45.41%, 35.81%, 17.87%, and 0.91% for sewage and manure, soil organic nitrogen, synthetic fertilizer, and atmospheric deposition, respectively. Undeveloped infrastructure and sewage disposal in rural areas were the main causes of nitrate contamination. Our results provide a theoretical basis for the development of measures to guarantee long-term water supply of the South to North Water Diversion Project. |
| doi_str_mv | 10.1007/s11356-021-14083-2 |
| format | Article |
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15
N-NO
3
−
and δ
18
O-NO
3
−
), and the Bayesian mixing model (SIAR) were combined. The results for 160 samples indicated that mean nitrate concentrations of residential area (162.83 mg L
−1
) and farmland (75.71 mg L
−1
) were higher compared with those of surface water (16.15 mg L
−1
) and forest (36.25 mg L
−1
). Hydrochemical facies and molar ratios of major ions indicated that the natural environment was greatly impacted by anthropogenic activities. Nitrification, ammonium volatilization, and mixing effects were the dominant processes in nitrogen transformation. The contributions of different sources to nitrate contamination were 45.41%, 35.81%, 17.87%, and 0.91% for sewage and manure, soil organic nitrogen, synthetic fertilizer, and atmospheric deposition, respectively. Undeveloped infrastructure and sewage disposal in rural areas were the main causes of nitrate contamination. Our results provide a theoretical basis for the development of measures to guarantee long-term water supply of the South to North Water Diversion Project.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-14083-2</identifier><identifier>PMID: 33907952</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Agricultural land ; Agrochemicals ; Ammonium ; Anthropogenic factors ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Bayesian analysis ; Contamination ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Hydrogeochemistry ; Isotopes ; Land use ; Natural environment ; Nitrates ; Nitrification ; Nitrogen ; Organic nitrogen ; Organic soils ; Research Article ; Residential areas ; Rural areas ; Sewage ; Sewage disposal ; Soil contamination ; Surface water ; Volatilization ; Waste Water Technology ; Water diversion ; Water Management ; Water Pollution Control ; Water supply</subject><ispartof>Environmental science and pollution research international, 2021-09, Vol.28 (35), p.48343-48361</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c375t-46718e51e66664635d38b2537ff83ad89507e547d9ef5de260f446d464f4d0143</citedby><cites>FETCH-LOGICAL-c375t-46718e51e66664635d38b2537ff83ad89507e547d9ef5de260f446d464f4d0143</cites><orcidid>0000-0003-0764-4629</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-021-14083-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-021-14083-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/33907952$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Cao, Shengwei</creatorcontrib><creatorcontrib>Fei, Yuhong</creatorcontrib><creatorcontrib>Tian, Xia</creatorcontrib><creatorcontrib>Cui, Xiangxiang</creatorcontrib><creatorcontrib>Zhang, Xueqing</creatorcontrib><creatorcontrib>Yuan, Ruoxi</creatorcontrib><creatorcontrib>Li, Yasong</creatorcontrib><title>Determining the origin and fate of nitrate in the Nanyang Basin, Central China, using environmental isotopes and the Bayesian mixing model</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Identifying sources of nitrate contamination has been a long-term challenge in areas with different land uses. We investigated the biogeochemical processes and quantified the contribution of potential nitrate sources in the Nanyang Basin, the source area of the South to North Water Diversion Project in China. Hydrogeochemical characteristics, the dual-isotope method (δ
15
N-NO
3
−
and δ
18
O-NO
3
−
), and the Bayesian mixing model (SIAR) were combined. The results for 160 samples indicated that mean nitrate concentrations of residential area (162.83 mg L
−1
) and farmland (75.71 mg L
−1
) were higher compared with those of surface water (16.15 mg L
−1
) and forest (36.25 mg L
−1
). Hydrochemical facies and molar ratios of major ions indicated that the natural environment was greatly impacted by anthropogenic activities. Nitrification, ammonium volatilization, and mixing effects were the dominant processes in nitrogen transformation. The contributions of different sources to nitrate contamination were 45.41%, 35.81%, 17.87%, and 0.91% for sewage and manure, soil organic nitrogen, synthetic fertilizer, and atmospheric deposition, respectively. Undeveloped infrastructure and sewage disposal in rural areas were the main causes of nitrate contamination. Our results provide a theoretical basis for the development of measures to guarantee long-term water supply of the South to North Water Diversion Project.</description><subject>Agricultural land</subject><subject>Agrochemicals</subject><subject>Ammonium</subject><subject>Anthropogenic factors</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Bayesian analysis</subject><subject>Contamination</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Hydrogeochemistry</subject><subject>Isotopes</subject><subject>Land use</subject><subject>Natural environment</subject><subject>Nitrates</subject><subject>Nitrification</subject><subject>Nitrogen</subject><subject>Organic nitrogen</subject><subject>Organic soils</subject><subject>Research Article</subject><subject>Residential areas</subject><subject>Rural areas</subject><subject>Sewage</subject><subject>Sewage disposal</subject><subject>Soil contamination</subject><subject>Surface water</subject><subject>Volatilization</subject><subject>Waste Water Technology</subject><subject>Water diversion</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>Water 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pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2021-09-01</date><risdate>2021</risdate><volume>28</volume><issue>35</issue><spage>48343</spage><epage>48361</epage><pages>48343-48361</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Identifying sources of nitrate contamination has been a long-term challenge in areas with different land uses. We investigated the biogeochemical processes and quantified the contribution of potential nitrate sources in the Nanyang Basin, the source area of the South to North Water Diversion Project in China. Hydrogeochemical characteristics, the dual-isotope method (δ
15
N-NO
3
−
and δ
18
O-NO
3
−
), and the Bayesian mixing model (SIAR) were combined. The results for 160 samples indicated that mean nitrate concentrations of residential area (162.83 mg L
−1
) and farmland (75.71 mg L
−1
) were higher compared with those of surface water (16.15 mg L
−1
) and forest (36.25 mg L
−1
). Hydrochemical facies and molar ratios of major ions indicated that the natural environment was greatly impacted by anthropogenic activities. Nitrification, ammonium volatilization, and mixing effects were the dominant processes in nitrogen transformation. The contributions of different sources to nitrate contamination were 45.41%, 35.81%, 17.87%, and 0.91% for sewage and manure, soil organic nitrogen, synthetic fertilizer, and atmospheric deposition, respectively. Undeveloped infrastructure and sewage disposal in rural areas were the main causes of nitrate contamination. Our results provide a theoretical basis for the development of measures to guarantee long-term water supply of the South to North Water Diversion Project.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>33907952</pmid><doi>10.1007/s11356-021-14083-2</doi><tpages>19</tpages><orcidid>https://orcid.org/0000-0003-0764-4629</orcidid></addata></record> |
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| ispartof | Environmental science and pollution research international, 2021-09, Vol.28 (35), p.48343-48361 |
| issn | 0944-1344 1614-7499 |
| language | eng |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Agricultural land Agrochemicals Ammonium Anthropogenic factors Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Bayesian analysis Contamination Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Hydrogeochemistry Isotopes Land use Natural environment Nitrates Nitrification Nitrogen Organic nitrogen Organic soils Research Article Residential areas Rural areas Sewage Sewage disposal Soil contamination Surface water Volatilization Waste Water Technology Water diversion Water Management Water Pollution Control Water supply |
| title | Determining the origin and fate of nitrate in the Nanyang Basin, Central China, using environmental isotopes and the Bayesian mixing model |
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