Long-lived quantum coherent dynamics of a \(\Lambda\)-system driven by a thermal environment
We present a theoretical study of quantum coherent dynamics of a three-level \(\Lambda\) system driven by a thermal environment (such as blackbody radiation), which serves as an essential building block of photosynthetic light-harvesting models and quantum heat engines. By solving the nonsecular Blo...
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description | We present a theoretical study of quantum coherent dynamics of a three-level \(\Lambda\) system driven by a thermal environment (such as blackbody radiation), which serves as an essential building block of photosynthetic light-harvesting models and quantum heat engines. By solving the nonsecular Bloch-Redfield master equations, we obtain analytical results for the ground-state population and coherence dynamics and classify the dynamical regimes of the incoherently driven \(\Lambda\)-system as underdamped and overdamped depending on whether the ratio \(\Delta/[r f(p)]\) is greater or less than one, where \(\Delta\) is the ground-state energy splitting, \(r\) is the incoherent pumping rate, and \(f(p)\) is a function of the transition dipole alignment parameter \(p\). In the underdamped regime, we observe long-lived coherent dynamics that lasts for \(\tau_c\simeq 1/r\), even though the initial state of the \(\Lambda\)-system contains no coherences in the energy basis. In the overdamped regime for \(p = 1\), we observe the emergence of coherent quasi-steady states with the lifetime \(\tau_{c} = 1.34 (r/\Delta^{2})\), which have low von Neumann entropy compared to the conventional thermal states. We propose an experimental scenario for observing noise-induced coherent dynamics in metastable He\(^*\) atoms driven by x-polarized incoherent light. Our results suggest that thermal excitations can generate experimentally observable long-lived quantum coherent dynamics in the ground-state subspace of atomic and molecular \(\Lambda\) systems in the absence of coherent driving. |
doi_str_mv | 10.48550/arxiv.2108.07457 |
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By solving the nonsecular Bloch-Redfield master equations, we obtain analytical results for the ground-state population and coherence dynamics and classify the dynamical regimes of the incoherently driven \(\Lambda\)-system as underdamped and overdamped depending on whether the ratio \(\Delta/[r f(p)]\) is greater or less than one, where \(\Delta\) is the ground-state energy splitting, \(r\) is the incoherent pumping rate, and \(f(p)\) is a function of the transition dipole alignment parameter \(p\). In the underdamped regime, we observe long-lived coherent dynamics that lasts for \(\tau_c\simeq 1/r\), even though the initial state of the \(\Lambda\)-system contains no coherences in the energy basis. In the overdamped regime for \(p = 1\), we observe the emergence of coherent quasi-steady states with the lifetime \(\tau_{c} = 1.34 (r/\Delta^{2})\), which have low von Neumann entropy compared to the conventional thermal states. We propose an experimental scenario for observing noise-induced coherent dynamics in metastable He\(^*\) atoms driven by x-polarized incoherent light. Our results suggest that thermal excitations can generate experimentally observable long-lived quantum coherent dynamics in the ground-state subspace of atomic and molecular \(\Lambda\) systems in the absence of coherent driving.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.2108.07457</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Dipoles ; Dynamics ; Quantum phenomena ; Quasi-steady states ; Thermal environments</subject><ispartof>arXiv.org, 2022-10</ispartof><rights>2022. This work is published under http://arxiv.org/licenses/nonexclusive-distrib/1.0/ (the “License”). 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By solving the nonsecular Bloch-Redfield master equations, we obtain analytical results for the ground-state population and coherence dynamics and classify the dynamical regimes of the incoherently driven \(\Lambda\)-system as underdamped and overdamped depending on whether the ratio \(\Delta/[r f(p)]\) is greater or less than one, where \(\Delta\) is the ground-state energy splitting, \(r\) is the incoherent pumping rate, and \(f(p)\) is a function of the transition dipole alignment parameter \(p\). In the underdamped regime, we observe long-lived coherent dynamics that lasts for \(\tau_c\simeq 1/r\), even though the initial state of the \(\Lambda\)-system contains no coherences in the energy basis. In the overdamped regime for \(p = 1\), we observe the emergence of coherent quasi-steady states with the lifetime \(\tau_{c} = 1.34 (r/\Delta^{2})\), which have low von Neumann entropy compared to the conventional thermal states. We propose an experimental scenario for observing noise-induced coherent dynamics in metastable He\(^*\) atoms driven by x-polarized incoherent light. 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By solving the nonsecular Bloch-Redfield master equations, we obtain analytical results for the ground-state population and coherence dynamics and classify the dynamical regimes of the incoherently driven \(\Lambda\)-system as underdamped and overdamped depending on whether the ratio \(\Delta/[r f(p)]\) is greater or less than one, where \(\Delta\) is the ground-state energy splitting, \(r\) is the incoherent pumping rate, and \(f(p)\) is a function of the transition dipole alignment parameter \(p\). In the underdamped regime, we observe long-lived coherent dynamics that lasts for \(\tau_c\simeq 1/r\), even though the initial state of the \(\Lambda\)-system contains no coherences in the energy basis. In the overdamped regime for \(p = 1\), we observe the emergence of coherent quasi-steady states with the lifetime \(\tau_{c} = 1.34 (r/\Delta^{2})\), which have low von Neumann entropy compared to the conventional thermal states. We propose an experimental scenario for observing noise-induced coherent dynamics in metastable He\(^*\) atoms driven by x-polarized incoherent light. Our results suggest that thermal excitations can generate experimentally observable long-lived quantum coherent dynamics in the ground-state subspace of atomic and molecular \(\Lambda\) systems in the absence of coherent driving.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><doi>10.48550/arxiv.2108.07457</doi><oa>free_for_read</oa></addata></record> |
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subjects | Dipoles Dynamics Quantum phenomena Quasi-steady states Thermal environments |
title | Long-lived quantum coherent dynamics of a \(\Lambda\)-system driven by a thermal environment |
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