Atom-Anchoring Strategy with Metal–Organic Frameworks for Highly Efficient Solid-State Electrochemiluminescence
A chemical fixation strategy originating from single-atom-anchoring with metal–organic frameworks as a carrying matrix was proposed for solid-state electrochemiluminescence (ECL). Herein, UiO-67(N) with the exposure of 2,2′-bipyridine (bpy) ligands could coordinate with Ru2+ to form a local structu...
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| Veröffentlicht in: | Analytical chemistry (Washington) 2021-07, Vol.93 (27), p.9628-9633 |
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| container_title | Analytical chemistry (Washington) |
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| creator | Zhu, Xinyang Xing, Huanhuan Xue, Yuan Li, Jing Wang, Erkang Dong, Shaojun |
| description | A chemical fixation strategy originating from single-atom-anchoring with metal–organic frameworks as a carrying matrix was proposed for solid-state electrochemiluminescence (ECL). Herein, UiO-67(N) with the exposure of 2,2′-bipyridine (bpy) ligands could coordinate with Ru2+ to form a local structure of [Ru(bpy)3]2+ (Ru-UiO). The influence of the steric effect induced with different Ru sources was discussed. The as-obtained Ru-UiO exhibits high ECL intensity and outstanding stability in the presence of a coreactant at low concentrations. The proposed synthesis strategy may hold great potential for the synthesis of solid-state ECL materials and their further utilization in ECL analysis. |
| doi_str_mv | 10.1021/acs.analchem.1c01838 |
| format | Article |
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Herein, UiO-67(N) with the exposure of 2,2′-bipyridine (bpy) ligands could coordinate with Ru2+ to form a local structure of [Ru(bpy)3]2+ (Ru-UiO). The influence of the steric effect induced with different Ru sources was discussed. The as-obtained Ru-UiO exhibits high ECL intensity and outstanding stability in the presence of a coreactant at low concentrations. The proposed synthesis strategy may hold great potential for the synthesis of solid-state ECL materials and their further utilization in ECL analysis.</description><identifier>ISSN: 0003-2700</identifier><identifier>EISSN: 1520-6882</identifier><identifier>DOI: 10.1021/acs.analchem.1c01838</identifier><identifier>PMID: 34213301</identifier><language>eng</language><publisher>WASHINGTON: American Chemical Society</publisher><subject>Analytical chemistry ; Chemistry ; Chemistry, Analytical ; Electrochemiluminescence ; Low concentrations ; Metal-organic frameworks ; Physical Sciences ; Science & Technology ; Solid state ; Synthesis</subject><ispartof>Analytical chemistry (Washington), 2021-07, Vol.93 (27), p.9628-9633</ispartof><rights>2021 American Chemical Society</rights><rights>Copyright American Chemical Society Jul 13, 2021</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>11</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000674254900040</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-a353t-fbdc1818b2869900150266c19866598cefb8441712f78d59fc106e1dc80678163</citedby><cites>FETCH-LOGICAL-a353t-fbdc1818b2869900150266c19866598cefb8441712f78d59fc106e1dc80678163</cites><orcidid>0000-0002-9828-7569 ; 0000-0001-9843-1834 ; 0000-0002-0263-6577</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.analchem.1c01838$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.analchem.1c01838$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>315,781,785,2766,27081,27929,27930,39263,56743,56793</link.rule.ids></links><search><creatorcontrib>Zhu, Xinyang</creatorcontrib><creatorcontrib>Xing, Huanhuan</creatorcontrib><creatorcontrib>Xue, Yuan</creatorcontrib><creatorcontrib>Li, Jing</creatorcontrib><creatorcontrib>Wang, Erkang</creatorcontrib><creatorcontrib>Dong, Shaojun</creatorcontrib><title>Atom-Anchoring Strategy with Metal–Organic Frameworks for Highly Efficient Solid-State Electrochemiluminescence</title><title>Analytical chemistry (Washington)</title><addtitle>ANAL CHEM</addtitle><addtitle>Anal. 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The proposed synthesis strategy may hold great potential for the synthesis of solid-state ECL materials and their further utilization in ECL analysis.</description><subject>Analytical chemistry</subject><subject>Chemistry</subject><subject>Chemistry, Analytical</subject><subject>Electrochemiluminescence</subject><subject>Low concentrations</subject><subject>Metal-organic frameworks</subject><subject>Physical Sciences</subject><subject>Science & Technology</subject><subject>Solid state</subject><subject>Synthesis</subject><issn>0003-2700</issn><issn>1520-6882</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>HGBXW</sourceid><recordid>eNqNkcFuEzEURS0EoqHwBywssUFCE96bGXs8yyhKKVJRF2nXI8exE5cZu7U9irLjH_qH_RI8SumCBWL1Nude3XcvIR8R5gglfpUqzqWTvdrrYY4KUFTiFZkhK6HgQpSvyQwAqqJsAM7IuxjvABAB-VtyVtUlVhXgjDwskh-KhVN7H6zb0XUKMundkR5s2tMfOsn-6dfjddhJZxW9CHLQBx9-Rmp8oJd2t--PdGWMVVa7RNe-t9tinbIFXfVapeCneLYfB-t0VNop_Z68MbKP-sPzPSe3F6ub5WVxdf3t-3JxVciKVakwm61CgWJTCt62OTqDknOFreCctUJpsxF1jQ2WphFb1hqFwDVulQDeCOTVOfl88r0P_mHUMXWDzQn6Xjrtx9iVrBY1spazjH76C73zY8jdThTjommEmAzrE6WCjzFo090HO8hw7BC6aZIuT9L9maR7niTLvpxkB73xJk5FKf0izRPxps5Z8otQQ6bF_9NLm5u23i396FKWwkk6xXh54J_ZfgP0IbKJ</recordid><startdate>20210713</startdate><enddate>20210713</enddate><creator>Zhu, Xinyang</creator><creator>Xing, Huanhuan</creator><creator>Xue, Yuan</creator><creator>Li, Jing</creator><creator>Wang, Erkang</creator><creator>Dong, Shaojun</creator><general>American Chemical Society</general><general>Amer Chemical Soc</general><scope>BLEPL</scope><scope>DTL</scope><scope>HGBXW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QO</scope><scope>7QQ</scope><scope>7SC</scope><scope>7SE</scope><scope>7SP</scope><scope>7SR</scope><scope>7TA</scope><scope>7TB</scope><scope>7TM</scope><scope>7U5</scope><scope>7U7</scope><scope>7U9</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>H94</scope><scope>JG9</scope><scope>JQ2</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>P64</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-9828-7569</orcidid><orcidid>https://orcid.org/0000-0001-9843-1834</orcidid><orcidid>https://orcid.org/0000-0002-0263-6577</orcidid></search><sort><creationdate>20210713</creationdate><title>Atom-Anchoring Strategy with Metal–Organic Frameworks for Highly Efficient Solid-State Electrochemiluminescence</title><author>Zhu, Xinyang ; 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Chem</addtitle><date>2021-07-13</date><risdate>2021</risdate><volume>93</volume><issue>27</issue><spage>9628</spage><epage>9633</epage><pages>9628-9633</pages><issn>0003-2700</issn><eissn>1520-6882</eissn><abstract>A chemical fixation strategy originating from single-atom-anchoring with metal–organic frameworks as a carrying matrix was proposed for solid-state electrochemiluminescence (ECL). Herein, UiO-67(N) with the exposure of 2,2′-bipyridine (bpy) ligands could coordinate with Ru2+ to form a local structure of [Ru(bpy)3]2+ (Ru-UiO). The influence of the steric effect induced with different Ru sources was discussed. The as-obtained Ru-UiO exhibits high ECL intensity and outstanding stability in the presence of a coreactant at low concentrations. 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| subjects | Analytical chemistry Chemistry Chemistry, Analytical Electrochemiluminescence Low concentrations Metal-organic frameworks Physical Sciences Science & Technology Solid state Synthesis |
| title | Atom-Anchoring Strategy with Metal–Organic Frameworks for Highly Efficient Solid-State Electrochemiluminescence |
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