Composite of aromatic polythiourea/BaTiO3 nanowires with high energy density and high discharge efficiency for energy storage applications
Ceramic/polymer nanocomposites have shown great potential in high energy storage density capacitors for pulsed power applications. However, due to the difference in surface energy between inorganic fillers and polymers, the discharge energy density and efficiency of nanocomposites are limited. In th...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2021-07, Vol.32 (14), p.19309-19326 |
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| container_title | Journal of materials science. Materials in electronics |
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| creator | Li, Xiali Shi, Liuwei Chen, Lei Yang, Wenyao Zha, Xiaoting Wang, Chengpeng Xi, Runhui Xu, Jianhua Yang, Yajie |
| description | Ceramic/polymer nanocomposites have shown great potential in high energy storage density capacitors for pulsed power applications. However, due to the difference in surface energy between inorganic fillers and polymers, the discharge energy density and efficiency of nanocomposites are limited. In this article, the BaTiO
3
(BT) nanowires (NWs) modified with dopamine (Dopa) was introduced into aromatic polythiourea (ArPTU) polymer matrix as composite for high-performance dielectrics. This is a new path about the introduction of a high dielectric constant ceramic into high dipole moment linear polymers (HDMLP), which produces the polymer composite with high energy storage density and high discharge efficiency. The composite ArPTU/BT NWs shows an energy density of 7.5 J cm
−3
and high efficiency more than 90% is obtained under an electric field of 250 MV m
−1
. It also has been found that the modification of BT NWs with the Dopa reduces the dielectric loss of composite effectively due to the good synergistic effective between ArPTU and BT NWs, and high stability of composite for energy storage is also achieved. This work provides an effective solution for achieving high energy storage density and high discharge efficiency in polymer dielectrics for practical capacitor applications. |
| doi_str_mv | 10.1007/s10854-021-06450-z |
| format | Article |
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3
(BT) nanowires (NWs) modified with dopamine (Dopa) was introduced into aromatic polythiourea (ArPTU) polymer matrix as composite for high-performance dielectrics. This is a new path about the introduction of a high dielectric constant ceramic into high dipole moment linear polymers (HDMLP), which produces the polymer composite with high energy storage density and high discharge efficiency. The composite ArPTU/BT NWs shows an energy density of 7.5 J cm
−3
and high efficiency more than 90% is obtained under an electric field of 250 MV m
−1
. It also has been found that the modification of BT NWs with the Dopa reduces the dielectric loss of composite effectively due to the good synergistic effective between ArPTU and BT NWs, and high stability of composite for energy storage is also achieved. This work provides an effective solution for achieving high energy storage density and high discharge efficiency in polymer dielectrics for practical capacitor applications.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-021-06450-z</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Barium titanates ; Capacitors ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Dielectric loss ; Dipole moments ; Discharge ; Dopamine ; Efficiency ; Electric fields ; Energy storage ; Flux density ; Materials Science ; Nanocomposites ; Nanowires ; Optical and Electronic Materials ; Polymer matrix composites ; Polymers ; Surface energy</subject><ispartof>Journal of materials science. Materials in electronics, 2021-07, Vol.32 (14), p.19309-19326</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c363t-c786b5e2daccf367d5660ae4a2d349633c261305f55bdb13dd11405e8f5604403</citedby><cites>FETCH-LOGICAL-c363t-c786b5e2daccf367d5660ae4a2d349633c261305f55bdb13dd11405e8f5604403</cites><orcidid>0000-0002-5292-0349</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-021-06450-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-021-06450-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Li, Xiali</creatorcontrib><creatorcontrib>Shi, Liuwei</creatorcontrib><creatorcontrib>Chen, Lei</creatorcontrib><creatorcontrib>Yang, Wenyao</creatorcontrib><creatorcontrib>Zha, Xiaoting</creatorcontrib><creatorcontrib>Wang, Chengpeng</creatorcontrib><creatorcontrib>Xi, Runhui</creatorcontrib><creatorcontrib>Xu, Jianhua</creatorcontrib><creatorcontrib>Yang, Yajie</creatorcontrib><title>Composite of aromatic polythiourea/BaTiO3 nanowires with high energy density and high discharge efficiency for energy storage applications</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>Ceramic/polymer nanocomposites have shown great potential in high energy storage density capacitors for pulsed power applications. However, due to the difference in surface energy between inorganic fillers and polymers, the discharge energy density and efficiency of nanocomposites are limited. In this article, the BaTiO
3
(BT) nanowires (NWs) modified with dopamine (Dopa) was introduced into aromatic polythiourea (ArPTU) polymer matrix as composite for high-performance dielectrics. This is a new path about the introduction of a high dielectric constant ceramic into high dipole moment linear polymers (HDMLP), which produces the polymer composite with high energy storage density and high discharge efficiency. The composite ArPTU/BT NWs shows an energy density of 7.5 J cm
−3
and high efficiency more than 90% is obtained under an electric field of 250 MV m
−1
. It also has been found that the modification of BT NWs with the Dopa reduces the dielectric loss of composite effectively due to the good synergistic effective between ArPTU and BT NWs, and high stability of composite for energy storage is also achieved. This work provides an effective solution for achieving high energy storage density and high discharge efficiency in polymer dielectrics for practical capacitor applications.</description><subject>Barium titanates</subject><subject>Capacitors</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Dielectric loss</subject><subject>Dipole moments</subject><subject>Discharge</subject><subject>Dopamine</subject><subject>Efficiency</subject><subject>Electric fields</subject><subject>Energy storage</subject><subject>Flux density</subject><subject>Materials Science</subject><subject>Nanocomposites</subject><subject>Nanowires</subject><subject>Optical and Electronic Materials</subject><subject>Polymer matrix composites</subject><subject>Polymers</subject><subject>Surface energy</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kMtqGzEUhkVpIG6SF8hKkPU0R9cZLxuTNgGDNyl0J2RdPAq2NJEmmPEj9KmrZlqyy-rAOf-F8yF0TeArAWhvC4FO8AYoaUByAc3pE1oQ0bKGd_TXZ7SApWgbLig9R19KeQaoMtYt0O9VOgyphNHh5LHO6aDHYPCQ9tPYh_Sanb69009hw3DUMR1DdgUfw9jjPux67KLLuwlbF2vEhHW0896GYnqddw4774MJLpoJ-5T_G8qYsq5XPQz7YGpliuUSnXm9L-7q37xAP7_fP60emvXmx-Pq27oxTLKxMW0nt8JRq43xTLZWSAnacU0t40vJmKGSMBBeiK3dEmYtIRyE67yQwDmwC3Qz5w45vby6Mqrn-meslYoKUeGBZMuqorPK5FRKdl4NORx0nhQB9Ze5mpmryly9MVenamKzqVRx3Ln8Hv2B6w-cN4fJ</recordid><startdate>20210701</startdate><enddate>20210701</enddate><creator>Li, Xiali</creator><creator>Shi, Liuwei</creator><creator>Chen, Lei</creator><creator>Yang, Wenyao</creator><creator>Zha, Xiaoting</creator><creator>Wang, Chengpeng</creator><creator>Xi, Runhui</creator><creator>Xu, Jianhua</creator><creator>Yang, Yajie</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0002-5292-0349</orcidid></search><sort><creationdate>20210701</creationdate><title>Composite of aromatic polythiourea/BaTiO3 nanowires with high energy density and high discharge efficiency for energy storage applications</title><author>Li, Xiali ; Shi, Liuwei ; Chen, Lei ; Yang, Wenyao ; Zha, Xiaoting ; Wang, Chengpeng ; Xi, Runhui ; Xu, Jianhua ; Yang, Yajie</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c363t-c786b5e2daccf367d5660ae4a2d349633c261305f55bdb13dd11405e8f5604403</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Barium titanates</topic><topic>Capacitors</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Dielectric loss</topic><topic>Dipole moments</topic><topic>Discharge</topic><topic>Dopamine</topic><topic>Efficiency</topic><topic>Electric fields</topic><topic>Energy storage</topic><topic>Flux density</topic><topic>Materials Science</topic><topic>Nanocomposites</topic><topic>Nanowires</topic><topic>Optical and Electronic Materials</topic><topic>Polymer matrix composites</topic><topic>Polymers</topic><topic>Surface energy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Xiali</creatorcontrib><creatorcontrib>Shi, Liuwei</creatorcontrib><creatorcontrib>Chen, Lei</creatorcontrib><creatorcontrib>Yang, Wenyao</creatorcontrib><creatorcontrib>Zha, Xiaoting</creatorcontrib><creatorcontrib>Wang, Chengpeng</creatorcontrib><creatorcontrib>Xi, Runhui</creatorcontrib><creatorcontrib>Xu, Jianhua</creatorcontrib><creatorcontrib>Yang, Yajie</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Xiali</au><au>Shi, Liuwei</au><au>Chen, Lei</au><au>Yang, Wenyao</au><au>Zha, Xiaoting</au><au>Wang, Chengpeng</au><au>Xi, Runhui</au><au>Xu, Jianhua</au><au>Yang, Yajie</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Composite of aromatic polythiourea/BaTiO3 nanowires with high energy density and high discharge efficiency for energy storage applications</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2021-07-01</date><risdate>2021</risdate><volume>32</volume><issue>14</issue><spage>19309</spage><epage>19326</epage><pages>19309-19326</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>Ceramic/polymer nanocomposites have shown great potential in high energy storage density capacitors for pulsed power applications. However, due to the difference in surface energy between inorganic fillers and polymers, the discharge energy density and efficiency of nanocomposites are limited. In this article, the BaTiO
3
(BT) nanowires (NWs) modified with dopamine (Dopa) was introduced into aromatic polythiourea (ArPTU) polymer matrix as composite for high-performance dielectrics. This is a new path about the introduction of a high dielectric constant ceramic into high dipole moment linear polymers (HDMLP), which produces the polymer composite with high energy storage density and high discharge efficiency. The composite ArPTU/BT NWs shows an energy density of 7.5 J cm
−3
and high efficiency more than 90% is obtained under an electric field of 250 MV m
−1
. It also has been found that the modification of BT NWs with the Dopa reduces the dielectric loss of composite effectively due to the good synergistic effective between ArPTU and BT NWs, and high stability of composite for energy storage is also achieved. This work provides an effective solution for achieving high energy storage density and high discharge efficiency in polymer dielectrics for practical capacitor applications.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-021-06450-z</doi><tpages>18</tpages><orcidid>https://orcid.org/0000-0002-5292-0349</orcidid><oa>free_for_read</oa></addata></record> |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Barium titanates Capacitors Characterization and Evaluation of Materials Chemistry and Materials Science Dielectric loss Dipole moments Discharge Dopamine Efficiency Electric fields Energy storage Flux density Materials Science Nanocomposites Nanowires Optical and Electronic Materials Polymer matrix composites Polymers Surface energy |
| title | Composite of aromatic polythiourea/BaTiO3 nanowires with high energy density and high discharge efficiency for energy storage applications |
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