Sub‐Second Time‐Resolved Surface‐Enhanced Raman Spectroscopy Reveals Dynamic CO Intermediates during Electrochemical CO2 Reduction on Copper

The electrocatalytic carbon dioxide (CO2) reduction reaction (CO2RR) into hydrocarbons is a promising approach for greenhouse gas mitigation, but many details of this dynamic reaction remain elusive. Here, time‐resolved surface‐enhanced Raman spectroscopy (TR‐SERS) is employed to successfully monito...

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Veröffentlicht in:	Angewandte Chemie 2021-07, Vol.133 (30), p.16712-16720
Hauptverfasser:	An, Hongyu, Wu, Longfei, Mandemaker, Laurens D. B., Yang, Shuang, Ruiter, Jim, Wijten, Jochem H. J., Janssens, Joris C. L., Hartman, Thomas, Stam, Ward, Weckhuysen, Bert M.
Format:	Artikel
Sprache:	eng
Schlagworte:	Alkalinity Carbon dioxide Chemical reduction Chemistry Copper electrocatalysis Electrochemistry Ethylene Greenhouse gases Intermediates in situ Mitigation Raman spectroscopy Roughening Spectroscopy Spectrum analysis Vibration
Online-Zugang:	Volltext
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