Thermoenhanced osmotic power generator via lithium bromide and asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) nanofluidic membrane
Osmotic energy, existing between solutions with different concentrations, is a sustainable and ecofriendly resource for solving energy issues. However, current membrane-based osmotic energy conversion technologies focus on electricity generation from an “open” system by directly mixing salt (NaCl) s...
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| creator | Sun, Yue Wu, Yadong Hu, Yuhao Zhu, Congcong Guo, Hao Kong, Xiang-Yu Luo, Ercang Jiang, Lei Wen, Liping |
| description | Osmotic energy, existing between solutions with different concentrations, is a sustainable and ecofriendly resource for solving energy issues. However, current membrane-based osmotic energy conversion technologies focus on electricity generation from an “open” system by directly mixing salt (NaCl) solutions at room temperature. For the integrated utilization of thermal energy and higher power output performance, we demonstrate thermoenhanced osmotic energy conversion by employing highly soluble lithium bromide (LiBr) solutions, asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes, and LiMn
2
O
4
/carbon nanotube (LMO/CNT) electrodes. The thin top layer of this heat-resistant membrane contains hydrophilic groups (i.e., the sulfonated groups in SPEEK) that are beneficial for ion-selective transport. The thermal effect on each solution is investigated, and osmotic energy conversion can be improved by regulating the heat gradient. The power density is ~16.50 W/m
2
by coupling with a temperature gradient (30 °C). This work is a step forward for promoting the performance of osmotic energy conversion with thermal energy assistance and provides the basis for a closed-loop system with regenerated osmotic energy from other energy forms. Moreover, the external field-osmotic hybrid energy conversion system shows powerful potential in the energy harvesting field.
With the assistant of heat, the osmotic power generator with nanofluidic sulfonated poly(ether ether ketone)/poly(ether sulfone) membrane and high soluble lithium bromide shows excellent ion transport behavior and superior output power density for salinity gradient energy harvesting.
Research Summary
For integrated utilization of sustainable energy and pursuing the high performance of the osmotic energy harvesting, the authors propose a strategy to couple the low-grade thermal energy with the salinity gradient energy by employing a thermoenhanced osmotic power generator. In the system, the LiBr with high solubility and the asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes with high stability and ion selectivity are both chosen for the thermo-enhanced osmotic energy harvesting. The proposed generator achieved the output power density of ~16.50 W/m
2
, extremely high value at 50-fold artificial sea water/river water condition, by coupling with the configuration of 30 ºC temperature gradient. Thus, by using the proposed system, the thermal |
| doi_str_mv | 10.1038/s41427-021-00317-9 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2547178817</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2547178817</sourcerecordid><originalsourceid>FETCH-LOGICAL-c363t-8cd0f9a6665101ffbb8b3855e2603f116573d3e87e4257c00eea1466c913c98c3</originalsourceid><addsrcrecordid>eNp9kc1OxCAURhujiUZ9AVckbnRRhUKBLo3xLzFxo2tC6e1MxwIjUM28iM8rWqOu3FxuwnfOXXxFcUTwGcFUnkdGWCVKXJESY0pE2WwVe0RKVjJci-2fnTW7xWGMK4wx4ZzJmu0V749LCNaDW2pnoEM-Wp8Gg9b-DQJagIOgkw_oddBoHNJymCxqg7dDB0i7Dum4sRZSyEicxt47nbJl7cfNCaSsRvN8huQdnJ7_-ZjjcIqcdr4fp6HLDgu2DdrBQbHT6zHC4fe7XzxdXz1e3pb3Dzd3lxf3paGcplKaDveN5pzXBJO-b1vZUlnXUHFMe0J4LWhHQQpgVS0MxgCaMM5NQ6hppKH7xfHsXQf_MkFMauWn4PJJVdVMECElETlVzSkTfIwBerUOg9VhowhWnxWouQKVK1BfFagmQ3SGYg67BYRf9T_UB2NUjJI</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2547178817</pqid></control><display><type>article</type><title>Thermoenhanced osmotic power generator via lithium bromide and asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) nanofluidic membrane</title><source>DOAJ Directory of Open Access Journals</source><source>Springer Nature OA Free Journals</source><source>Nature Free</source><source>EZB-FREE-00999 freely available EZB journals</source><source>Free Full-Text Journals in Chemistry</source><creator>Sun, Yue ; Wu, Yadong ; Hu, Yuhao ; Zhu, Congcong ; Guo, Hao ; Kong, Xiang-Yu ; Luo, Ercang ; Jiang, Lei ; Wen, Liping</creator><creatorcontrib>Sun, Yue ; Wu, Yadong ; Hu, Yuhao ; Zhu, Congcong ; Guo, Hao ; Kong, Xiang-Yu ; Luo, Ercang ; Jiang, Lei ; Wen, Liping</creatorcontrib><description>Osmotic energy, existing between solutions with different concentrations, is a sustainable and ecofriendly resource for solving energy issues. However, current membrane-based osmotic energy conversion technologies focus on electricity generation from an “open” system by directly mixing salt (NaCl) solutions at room temperature. For the integrated utilization of thermal energy and higher power output performance, we demonstrate thermoenhanced osmotic energy conversion by employing highly soluble lithium bromide (LiBr) solutions, asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes, and LiMn
2
O
4
/carbon nanotube (LMO/CNT) electrodes. The thin top layer of this heat-resistant membrane contains hydrophilic groups (i.e., the sulfonated groups in SPEEK) that are beneficial for ion-selective transport. The thermal effect on each solution is investigated, and osmotic energy conversion can be improved by regulating the heat gradient. The power density is ~16.50 W/m
2
by coupling with a temperature gradient (30 °C). This work is a step forward for promoting the performance of osmotic energy conversion with thermal energy assistance and provides the basis for a closed-loop system with regenerated osmotic energy from other energy forms. Moreover, the external field-osmotic hybrid energy conversion system shows powerful potential in the energy harvesting field.
With the assistant of heat, the osmotic power generator with nanofluidic sulfonated poly(ether ether ketone)/poly(ether sulfone) membrane and high soluble lithium bromide shows excellent ion transport behavior and superior output power density for salinity gradient energy harvesting.
Research Summary
For integrated utilization of sustainable energy and pursuing the high performance of the osmotic energy harvesting, the authors propose a strategy to couple the low-grade thermal energy with the salinity gradient energy by employing a thermoenhanced osmotic power generator. In the system, the LiBr with high solubility and the asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes with high stability and ion selectivity are both chosen for the thermo-enhanced osmotic energy harvesting. The proposed generator achieved the output power density of ~16.50 W/m
2
, extremely high value at 50-fold artificial sea water/river water condition, by coupling with the configuration of 30 ºC temperature gradient. Thus, by using the proposed system, the thermal energy, especially low-grade ones, has been well harvested and greatly improve the osmotic energy conversion. Thus, the external field-osmotic hybrid energy conversion system could show its great potentials in different fields with proper coupling.</description><identifier>ISSN: 1884-4049</identifier><identifier>EISSN: 1884-4057</identifier><identifier>DOI: 10.1038/s41427-021-00317-9</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>140/131 ; 140/146 ; 639/301/299 ; 639/925 ; Asymmetry ; Biomaterials ; Carbon nanotubes ; Chemistry and Materials Science ; Energy conversion ; Energy harvesting ; Energy Systems ; Feedback control ; Fluidics ; Heat ; Hybrid systems ; Ion transport ; Lithium manganese oxides ; Materials Science ; Membranes ; Nanofluids ; Optical and Electronic Materials ; Power ; Room temperature ; Structural Materials ; Surface and Interface Science ; Temperature effects ; Thermal energy ; Thermal utilization ; Thin Films ; Transport phenomena</subject><ispartof>NPG Asia materials, 2021-07, Vol.13 (1), Article 50</ispartof><rights>The Author(s) 2021</rights><rights>The Author(s) 2021. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c363t-8cd0f9a6665101ffbb8b3855e2603f116573d3e87e4257c00eea1466c913c98c3</citedby><cites>FETCH-LOGICAL-c363t-8cd0f9a6665101ffbb8b3855e2603f116573d3e87e4257c00eea1466c913c98c3</cites><orcidid>0000-0002-4475-2162 ; 0000-0001-8546-8988</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1038/s41427-021-00317-9$$EPDF$$P50$$Gspringer$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://doi.org/10.1038/s41427-021-00317-9$$EHTML$$P50$$Gspringer$$Hfree_for_read</linktohtml><link.rule.ids>314,780,784,864,27922,27923,41118,42187,51574</link.rule.ids></links><search><creatorcontrib>Sun, Yue</creatorcontrib><creatorcontrib>Wu, Yadong</creatorcontrib><creatorcontrib>Hu, Yuhao</creatorcontrib><creatorcontrib>Zhu, Congcong</creatorcontrib><creatorcontrib>Guo, Hao</creatorcontrib><creatorcontrib>Kong, Xiang-Yu</creatorcontrib><creatorcontrib>Luo, Ercang</creatorcontrib><creatorcontrib>Jiang, Lei</creatorcontrib><creatorcontrib>Wen, Liping</creatorcontrib><title>Thermoenhanced osmotic power generator via lithium bromide and asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) nanofluidic membrane</title><title>NPG Asia materials</title><addtitle>NPG Asia Mater</addtitle><description>Osmotic energy, existing between solutions with different concentrations, is a sustainable and ecofriendly resource for solving energy issues. However, current membrane-based osmotic energy conversion technologies focus on electricity generation from an “open” system by directly mixing salt (NaCl) solutions at room temperature. For the integrated utilization of thermal energy and higher power output performance, we demonstrate thermoenhanced osmotic energy conversion by employing highly soluble lithium bromide (LiBr) solutions, asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes, and LiMn
2
O
4
/carbon nanotube (LMO/CNT) electrodes. The thin top layer of this heat-resistant membrane contains hydrophilic groups (i.e., the sulfonated groups in SPEEK) that are beneficial for ion-selective transport. The thermal effect on each solution is investigated, and osmotic energy conversion can be improved by regulating the heat gradient. The power density is ~16.50 W/m
2
by coupling with a temperature gradient (30 °C). This work is a step forward for promoting the performance of osmotic energy conversion with thermal energy assistance and provides the basis for a closed-loop system with regenerated osmotic energy from other energy forms. Moreover, the external field-osmotic hybrid energy conversion system shows powerful potential in the energy harvesting field.
With the assistant of heat, the osmotic power generator with nanofluidic sulfonated poly(ether ether ketone)/poly(ether sulfone) membrane and high soluble lithium bromide shows excellent ion transport behavior and superior output power density for salinity gradient energy harvesting.
Research Summary
For integrated utilization of sustainable energy and pursuing the high performance of the osmotic energy harvesting, the authors propose a strategy to couple the low-grade thermal energy with the salinity gradient energy by employing a thermoenhanced osmotic power generator. In the system, the LiBr with high solubility and the asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes with high stability and ion selectivity are both chosen for the thermo-enhanced osmotic energy harvesting. The proposed generator achieved the output power density of ~16.50 W/m
2
, extremely high value at 50-fold artificial sea water/river water condition, by coupling with the configuration of 30 ºC temperature gradient. Thus, by using the proposed system, the thermal energy, especially low-grade ones, has been well harvested and greatly improve the osmotic energy conversion. Thus, the external field-osmotic hybrid energy conversion system could show its great potentials in different fields with proper coupling.</description><subject>140/131</subject><subject>140/146</subject><subject>639/301/299</subject><subject>639/925</subject><subject>Asymmetry</subject><subject>Biomaterials</subject><subject>Carbon nanotubes</subject><subject>Chemistry and Materials Science</subject><subject>Energy conversion</subject><subject>Energy harvesting</subject><subject>Energy Systems</subject><subject>Feedback control</subject><subject>Fluidics</subject><subject>Heat</subject><subject>Hybrid systems</subject><subject>Ion transport</subject><subject>Lithium manganese oxides</subject><subject>Materials Science</subject><subject>Membranes</subject><subject>Nanofluids</subject><subject>Optical and Electronic Materials</subject><subject>Power</subject><subject>Room temperature</subject><subject>Structural Materials</subject><subject>Surface and Interface Science</subject><subject>Temperature effects</subject><subject>Thermal energy</subject><subject>Thermal utilization</subject><subject>Thin Films</subject><subject>Transport phenomena</subject><issn>1884-4049</issn><issn>1884-4057</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>C6C</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kc1OxCAURhujiUZ9AVckbnRRhUKBLo3xLzFxo2tC6e1MxwIjUM28iM8rWqOu3FxuwnfOXXxFcUTwGcFUnkdGWCVKXJESY0pE2WwVe0RKVjJci-2fnTW7xWGMK4wx4ZzJmu0V749LCNaDW2pnoEM-Wp8Gg9b-DQJagIOgkw_oddBoHNJymCxqg7dDB0i7Dum4sRZSyEicxt47nbJl7cfNCaSsRvN8huQdnJ7_-ZjjcIqcdr4fp6HLDgu2DdrBQbHT6zHC4fe7XzxdXz1e3pb3Dzd3lxf3paGcplKaDveN5pzXBJO-b1vZUlnXUHFMe0J4LWhHQQpgVS0MxgCaMM5NQ6hppKH7xfHsXQf_MkFMauWn4PJJVdVMECElETlVzSkTfIwBerUOg9VhowhWnxWouQKVK1BfFagmQ3SGYg67BYRf9T_UB2NUjJI</recordid><startdate>20210702</startdate><enddate>20210702</enddate><creator>Sun, Yue</creator><creator>Wu, Yadong</creator><creator>Hu, Yuhao</creator><creator>Zhu, Congcong</creator><creator>Guo, Hao</creator><creator>Kong, Xiang-Yu</creator><creator>Luo, Ercang</creator><creator>Jiang, Lei</creator><creator>Wen, Liping</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><scope>C6C</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><orcidid>https://orcid.org/0000-0002-4475-2162</orcidid><orcidid>https://orcid.org/0000-0001-8546-8988</orcidid></search><sort><creationdate>20210702</creationdate><title>Thermoenhanced osmotic power generator via lithium bromide and asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) nanofluidic membrane</title><author>Sun, Yue ; 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However, current membrane-based osmotic energy conversion technologies focus on electricity generation from an “open” system by directly mixing salt (NaCl) solutions at room temperature. For the integrated utilization of thermal energy and higher power output performance, we demonstrate thermoenhanced osmotic energy conversion by employing highly soluble lithium bromide (LiBr) solutions, asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes, and LiMn
2
O
4
/carbon nanotube (LMO/CNT) electrodes. The thin top layer of this heat-resistant membrane contains hydrophilic groups (i.e., the sulfonated groups in SPEEK) that are beneficial for ion-selective transport. The thermal effect on each solution is investigated, and osmotic energy conversion can be improved by regulating the heat gradient. The power density is ~16.50 W/m
2
by coupling with a temperature gradient (30 °C). This work is a step forward for promoting the performance of osmotic energy conversion with thermal energy assistance and provides the basis for a closed-loop system with regenerated osmotic energy from other energy forms. Moreover, the external field-osmotic hybrid energy conversion system shows powerful potential in the energy harvesting field.
With the assistant of heat, the osmotic power generator with nanofluidic sulfonated poly(ether ether ketone)/poly(ether sulfone) membrane and high soluble lithium bromide shows excellent ion transport behavior and superior output power density for salinity gradient energy harvesting.
Research Summary
For integrated utilization of sustainable energy and pursuing the high performance of the osmotic energy harvesting, the authors propose a strategy to couple the low-grade thermal energy with the salinity gradient energy by employing a thermoenhanced osmotic power generator. In the system, the LiBr with high solubility and the asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) (SPEEK/PES) membranes with high stability and ion selectivity are both chosen for the thermo-enhanced osmotic energy harvesting. The proposed generator achieved the output power density of ~16.50 W/m
2
, extremely high value at 50-fold artificial sea water/river water condition, by coupling with the configuration of 30 ºC temperature gradient. Thus, by using the proposed system, the thermal energy, especially low-grade ones, has been well harvested and greatly improve the osmotic energy conversion. Thus, the external field-osmotic hybrid energy conversion system could show its great potentials in different fields with proper coupling.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><doi>10.1038/s41427-021-00317-9</doi><orcidid>https://orcid.org/0000-0002-4475-2162</orcidid><orcidid>https://orcid.org/0000-0001-8546-8988</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | 140/131 140/146 639/301/299 639/925 Asymmetry Biomaterials Carbon nanotubes Chemistry and Materials Science Energy conversion Energy harvesting Energy Systems Feedback control Fluidics Heat Hybrid systems Ion transport Lithium manganese oxides Materials Science Membranes Nanofluids Optical and Electronic Materials Power Room temperature Structural Materials Surface and Interface Science Temperature effects Thermal energy Thermal utilization Thin Films Transport phenomena |
| title | Thermoenhanced osmotic power generator via lithium bromide and asymmetric sulfonated poly(ether ether ketone)/poly(ether sulfone) nanofluidic membrane |
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