Photocatalysis-activated SR-AOP over PDINH/MIL-88A(Fe) composites for boosted chloroquine phosphate degradation: Performance, mechanism, pathway and DFT calculations

[Display omitted] •PDINH/MIL-88A(Fe) composites were prepared via a facile ball-milled method.•Chloroquine phosphate (CQ) degradation over SR-AOP was achieved for the first time.•DFT calculations helped to explain the reactive sites of CQ and degradation pathways.•The toxicities of degradation produ...

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Veröffentlicht in:	Applied catalysis. B, Environmental Environmental, 2021-09, Vol.293, p.120229, Article 120229
Hauptverfasser:	Yi, Xiao-Hong, Ji, Haodong, Wang, Chong-Chen, Li, Yang, Li, Yu-Hang, Zhao, Chen, Wang, Ao, Fu, Huifen, Wang, Peng, Zhao, Xu, Liu, Wen
Format:	Artikel
Sprache:	eng
Schlagworte:	Ball milling Chloroquine Chloroquine phosphate Composite materials Degradation pathways DFT calculation Diimide Electron paramagnetic resonance Electron spin Electron spin resonance Electron transfer Environmental degradation Free radicals Intermediates Light effects Light emitting diodes Mathematical analysis Metal-organic framework Performance degradation Photocatalysis Pollutants Singlet oxygen Spin resonance Sulfate radical-advanced oxidation process Synergistic effect Toxicity
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