Nitrogenase-inspired bimetallic metal organic frameworks for visible-light-driven nitrogen fixation

[Display omitted] •Nitrogenase-inspired modular synthesis is designed to construct bimetallic UiO-66.•Zr-Hf clusters are constructed to coordinate the electron transfer and utilization.•U(0.5Hf)-2SH with TPA-2SH as the ligand can absorb and utilize the visible light.•A tandem ligand-to-metal-to-meta...

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Veröffentlicht in:	Applied catalysis. B, Environmental Environmental, 2021-09, Vol.292, p.120167, Article 120167
Hauptverfasser:	An, Ke, Ren, Hanjie, Yang, Dong, Zhao, Zhanfeng, Gao, Yuchen, Chen, Yao, Tan, Jiangdan, Wang, Wenjing, Jiang, Zhongyi
Format:	Artikel
Sprache:	eng
Schlagworte:	Absorption Bimetals Catalysts Electromagnetic absorption Electron transfer Electrons Functional groups Functional ligands Ligands Metal-organic frameworks Metals Nitrogen Nitrogen fixation Nitrogenase Nitrogenase-inspired Nitrogenation Nodes Optimization Photocatalysts Photocatalytic nitrogen fixation Zirconium Zr-Hf bimetallic clusters
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