Studies on near infrared emission of Yb3+ ions in a SeO2 based glass system

SeO2 based glasses of the composition 39 PbO–(60-x) B2O3– xSeO2:1.0 Yb2O3 (with 10 ≤ x ≤ 50) was synthesized. Analysis of the results of structural studies of the samples revealed that the glass network consists of [SeO4]2− and [SeO3]2− units; the studies further indicated an increasing fraction of...

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Veröffentlicht in:Physica. B, Condensed matter Condensed matter, 2021-04, Vol.606, p.412827, Article 412827
Hauptverfasser: Naresh, Pathuri, Ravi Kumar, Valluri, Sesha Reddy, A. Siva, Kostrzewa, M., Venkatramaiah, N., Krishna Mohan, N., Ravi Kumar, V., Veeraiah, N.
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container_start_page 412827
container_title Physica. B, Condensed matter
container_volume 606
creator Naresh, Pathuri
Ravi Kumar, Valluri
Sesha Reddy, A. Siva
Kostrzewa, M.
Venkatramaiah, N.
Krishna Mohan, N.
Ravi Kumar, V.
Veeraiah, N.
description SeO2 based glasses of the composition 39 PbO–(60-x) B2O3– xSeO2:1.0 Yb2O3 (with 10 ≤ x ≤ 50) was synthesized. Analysis of the results of structural studies of the samples revealed that the glass network consists of [SeO4]2− and [SeO3]2− units; the studies further indicated an increasing fraction of [SeO3]2− units and decreasing concentration of [SeO4]2− groups with increase of SeO2 content. Optical Absorption (OA) and photoluminescence (PL) spectra have exhibited bands due to 2F7/2 → 2F5/2 and 2F5/2 → 2F7/2 transitions, respectively. Evaluated absorption and emission cross-sections and lifetime of the excited state of Yb3+ ions exhibited an increase with increase of SeO2 content. Results of PL studies indicated nearly fourfold increase of PL output with increase of SeO2 content up to 50%. Such increase is attributed to the increased concentration of isolated [SeO3]2- pyramidal groups. Overall, the rise of SeO2 content in Yb3+ doped PbO–B2O3–SeO2 glass system facilitated the increase of PL emission of Yb3+ ions largely.
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Siva</au><au>Kostrzewa, M.</au><au>Venkatramaiah, N.</au><au>Krishna Mohan, N.</au><au>Ravi Kumar, V.</au><au>Veeraiah, N.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Studies on near infrared emission of Yb3+ ions in a SeO2 based glass system</atitle><jtitle>Physica. B, Condensed matter</jtitle><date>2021-04-01</date><risdate>2021</risdate><volume>606</volume><spage>412827</spage><pages>412827-</pages><artnum>412827</artnum><issn>0921-4526</issn><eissn>1873-2135</eissn><abstract>SeO2 based glasses of the composition 39 PbO–(60-x) B2O3– xSeO2:1.0 Yb2O3 (with 10 ≤ x ≤ 50) was synthesized. Analysis of the results of structural studies of the samples revealed that the glass network consists of [SeO4]2− and [SeO3]2− units; the studies further indicated an increasing fraction of [SeO3]2− units and decreasing concentration of [SeO4]2− groups with increase of SeO2 content. 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subjects 1.0 μm emission
Absorption
Boron oxides
Chemical synthesis
Emission analysis
Emission and absorption cross-sections
Glass
Ions
Luminescence
Near infrared radiation
Photoluminescence
Selenium dioxide
SeO2 based glass system
Studies
Yb3+ ions
title Studies on near infrared emission of Yb3+ ions in a SeO2 based glass system
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