Nickel–Promoted Molybdenum or Tungsten Carbides as Catalysts in Dry Reforming of Methane: Effects of Variation in CH4/CO2 Molar Ratio
Ni–Mo 2 C and Ni–WC were evaluated in dry reforming of methane employing different CH 4 /CO 2 ratios. Ni–Mo 2 C remained active under an excess of CH 4 , but deactivation occurred under an excess of CO 2 . Ni–WC was resistant to excess of CO 2 but showed carbon deposition under excess of CH 4 . Grap...
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| Veröffentlicht in: | Catalysis letters 2021-06, Vol.151 (6), p.1578-1591 |
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| container_end_page | 1591 |
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| container_issue | 6 |
| container_start_page | 1578 |
| container_title | Catalysis letters |
| container_volume | 151 |
| creator | Barbosa, Renato Dias Baldanza, Maria Auxiliadora Scaramelo de Resende, Neuman Solange Passos, Fabio Barboza da Silva, Victor Luis dos Santos Teixeira |
| description | Ni–Mo
2
C and Ni–WC were evaluated in dry reforming of methane employing different CH
4
/CO
2
ratios. Ni–Mo
2
C remained active under an excess of CH
4
, but deactivation occurred under an excess of CO
2
. Ni–WC was resistant to excess of CO
2
but showed carbon deposition under excess of CH
4
.
Graphic Abstract |
| doi_str_mv | 10.1007/s10562-020-03420-8 |
| format | Article |
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2
C and Ni–WC were evaluated in dry reforming of methane employing different CH
4
/CO
2
ratios. Ni–Mo
2
C remained active under an excess of CH
4
, but deactivation occurred under an excess of CO
2
. Ni–WC was resistant to excess of CO
2
but showed carbon deposition under excess of CH
4
.
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2
C and Ni–WC were evaluated in dry reforming of methane employing different CH
4
/CO
2
ratios. Ni–Mo
2
C remained active under an excess of CH
4
, but deactivation occurred under an excess of CO
2
. Ni–WC was resistant to excess of CO
2
but showed carbon deposition under excess of CH
4
.
Graphic Abstract</description><subject>Carbon dioxide</subject><subject>Catalysis</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Methane</subject><subject>Molybdenum carbide</subject><subject>Nickel</subject><subject>Organometallic Chemistry</subject><subject>Physical Chemistry</subject><subject>Reforming</subject><subject>Tungsten carbide</subject><issn>1011-372X</issn><issn>1572-879X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kE1OwzAQhSMEEqVwAVaWWIeO7fyyQ6FQpJaiqqDuLCexS0prFztZZMeOA3BDToJDkNixmRnNvDdP-jzvHMMlBohHFkMYER8I-EADV5MDb4DDmPhJnK4O3QwY-zQmq2PvxNoNAKQxTgfex0NVvIrt1_vno9E7XYsSzfS2zUuhmh3SBi0btba1UCjjJq9KYRG3bq75trW1RZVCN6ZFCyG12VVqjbREM1G_cCWu0FhKUTiR2z1zU_G60qpzZJNglM1Jl8QNWnT7U-9I8q0VZ7996D3djpfZxJ_O7-6z66lf0DCqfRFESQFpLqMwDyOeSFxCSfMk4Q5AERUljSNwFDDlMZFBwCUQ7E6QR2keUk6H3kX_d2_0WyNszTa6McpFMhJSmiYxoeBUpFcVRltrhGR7U-24aRkG1gFnPXDmotgPcJY4E-1N1onVWpi_1_-4vgFyyIO1</recordid><startdate>20210601</startdate><enddate>20210601</enddate><creator>Barbosa, Renato Dias</creator><creator>Baldanza, Maria Auxiliadora Scaramelo</creator><creator>de Resende, Neuman Solange</creator><creator>Passos, Fabio Barboza</creator><creator>da Silva, Victor Luis dos Santos Teixeira</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope></search><sort><creationdate>20210601</creationdate><title>Nickel–Promoted Molybdenum or Tungsten Carbides as Catalysts in Dry Reforming of Methane: Effects of Variation in CH4/CO2 Molar Ratio</title><author>Barbosa, Renato Dias ; Baldanza, Maria Auxiliadora Scaramelo ; de Resende, Neuman Solange ; Passos, Fabio Barboza ; da Silva, Victor Luis dos Santos Teixeira</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c356t-e468c09bf65b56a8f1d0d3b88a105c6cd376002013a72f44af0211050b69b53a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Carbon dioxide</topic><topic>Catalysis</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Methane</topic><topic>Molybdenum carbide</topic><topic>Nickel</topic><topic>Organometallic Chemistry</topic><topic>Physical Chemistry</topic><topic>Reforming</topic><topic>Tungsten carbide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Barbosa, Renato Dias</creatorcontrib><creatorcontrib>Baldanza, Maria Auxiliadora Scaramelo</creatorcontrib><creatorcontrib>de Resende, Neuman Solange</creatorcontrib><creatorcontrib>Passos, Fabio Barboza</creatorcontrib><creatorcontrib>da Silva, Victor Luis dos Santos Teixeira</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><jtitle>Catalysis letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Barbosa, Renato Dias</au><au>Baldanza, Maria Auxiliadora Scaramelo</au><au>de Resende, Neuman Solange</au><au>Passos, Fabio Barboza</au><au>da Silva, Victor Luis dos Santos Teixeira</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Nickel–Promoted Molybdenum or Tungsten Carbides as Catalysts in Dry Reforming of Methane: Effects of Variation in CH4/CO2 Molar Ratio</atitle><jtitle>Catalysis letters</jtitle><stitle>Catal Lett</stitle><date>2021-06-01</date><risdate>2021</risdate><volume>151</volume><issue>6</issue><spage>1578</spage><epage>1591</epage><pages>1578-1591</pages><issn>1011-372X</issn><eissn>1572-879X</eissn><abstract>Ni–Mo
2
C and Ni–WC were evaluated in dry reforming of methane employing different CH
4
/CO
2
ratios. Ni–Mo
2
C remained active under an excess of CH
4
, but deactivation occurred under an excess of CO
2
. Ni–WC was resistant to excess of CO
2
but showed carbon deposition under excess of CH
4
.
Graphic Abstract</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10562-020-03420-8</doi><tpages>14</tpages></addata></record> |
| fulltext | fulltext |
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| ispartof | Catalysis letters, 2021-06, Vol.151 (6), p.1578-1591 |
| issn | 1011-372X 1572-879X |
| language | eng |
| recordid | cdi_proquest_journals_2533987230 |
| source | SpringerLink Journals |
| subjects | Carbon dioxide Catalysis Chemistry Chemistry and Materials Science Industrial Chemistry/Chemical Engineering Methane Molybdenum carbide Nickel Organometallic Chemistry Physical Chemistry Reforming Tungsten carbide |
| title | Nickel–Promoted Molybdenum or Tungsten Carbides as Catalysts in Dry Reforming of Methane: Effects of Variation in CH4/CO2 Molar Ratio |
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