Isotopic 18O/16O substitution study on the direct partial oxidation of CH4 to dimethyl ether over a Pt/Y2O3 catalyst using NO/O2 as an oxidant

The direct partial oxidation of CH4 to dimethyl ether (DME) was achieved with a Pt/Y2O3 catalyst using a mixture of NO and O2. The actual gas composition contained a mixture of NO and NO2, with no decomposition or net consumption of these species. Use of 18O2 confirmed the transfer of labeled oxygen...

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Veröffentlicht in:	Catalysis science & technology 2021-01, Vol.11 (8), p.2708-2712
Hauptverfasser:	Ghampson, I Tyrone, Lundin, Sean-Thomas B, Shishido, Tetsuya, Oyama, S Ted
Format:	Artikel
Sprache:	eng
Schlagworte:	Catalysts Dimethyl ether Gas composition Methane Nitrogen dioxide Oxidation Oxidizing agents Yttrium oxide
Online-Zugang:	Volltext
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