In-plane crystallographic orientations related spin-orbit torque in epitaxial Pt(111)/Co/Ta heterostructures

Current induced spin–orbit torque (SOT) in heavy metals with strong spin–orbit coupling strength has attracted considerable attention due to its potential applications in spintronic technology. Pt, as one of the mostly used heavy metals in SOT-based spintronic devices, shows large spin Hall angle (θSH) with its single phase and alloy counterparts. In this work, the in-plane crystallographic orientations related θSH of epitaxial Pt(111) layer is reported in MgO(111)/Pt(111)/Co/Ta heterostructures with strong perpendicular magnetic anisotropy. The θSH shows a quite large difference with values, respectively, around 0.083 and 0.057 when the current applied along the [ 1 1 ¯ 0 ] and [ 11 2 ¯ ] crystallographic directions of Pt(111) by the damping-like SOT efficiency using the harmonic Hall voltage measurement technique. The critical switching current densities also show large difference between these two orthogonal crystallographic orientations with the trend of that the larger SOT efficiency leads to the smaller critical switching current density. It independently confirms the generation of different damping-like SOT efficiency when current along [ 1 1 ¯ 0 ] and [ 11 2 ¯ ] directions of Pt(111). Moreover, a perpendicularly magnetized Pt/Co/Ta reference heterostructures with Pt having polycrystalline phase shows tiny variation of damping-like SOT efficiency in in-plane two orthogonal directions, which also indirectly indicates the crystallographic orientations related θSH in epitaxial Pt(111) layers. This study indicates that the θSH of epitaxial Pt is a crystallographic orientations related parameter.