Metal organic frameworks derived single atom catalysts for electrocatalytic energy conversion
The development of efficient and cost-effective catalysts to catalyze a wide variety of electrochemical reactions is key to realize the large-scale application of renewable and clean energy technologies. Owing to the maximum atom-utilization efficiency and unique electronic and geometric structures,...
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| Veröffentlicht in: | Nano research 2019-09, Vol.12 (9), p.2067-2080 |
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| container_title | Nano research |
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| creator | Sun, Tingting Xu, Lianbin Wang, Dingsheng Li, Yadong |
| description | The development of efficient and cost-effective catalysts to catalyze a wide variety of electrochemical reactions is key to realize the large-scale application of renewable and clean energy technologies. Owing to the maximum atom-utilization efficiency and unique electronic and geometric structures, single atom catalysts (SACs) have exhibited superior performance in various catalytic systems. Recently, assembled from the functionalized organic linkers and metal nodes, metal-organic frameworks (MOFs) with ultrafine porosity have received tremendous attention as precursors or self-sacrificing templates for preparing porous SACs. Here, the recent advances toward the synthesis strategies for using MOF precursors/templates to construct SACs are systematically summarized with special emphasis on the types of central metal sites. The electrochemical applications of these recently emerged MOF-derived SACs for various energy-conversion processes, such as oxygen reduction/evolution reaction (ORR/OER), hydrogen evolution reaction (HER), and CO
2
reduction reaction (CO
2
RR), are also discussed and reviewed. Finally, the current challenges and prospects regarding the development of MOF-derived SACs are proposed. |
| doi_str_mv | 10.1007/s12274-019-2345-4 |
| format | Article |
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2
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2
reduction reaction (CO
2
RR), are also discussed and reviewed. 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2
reduction reaction (CO
2
RR), are also discussed and reviewed. Finally, the current challenges and prospects regarding the development of MOF-derived SACs are proposed.</abstract><cop>Beijing</cop><pub>Tsinghua University Press</pub><doi>10.1007/s12274-019-2345-4</doi><tpages>14</tpages><oa>free_for_read</oa></addata></record> |
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| identifier | ISSN: 1998-0124 |
| ispartof | Nano research, 2019-09, Vol.12 (9), p.2067-2080 |
| issn | 1998-0124 1998-0000 |
| language | eng |
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| subjects | Atomic/Molecular Structure and Spectra Atoms & subatomic particles Biomedicine Biotechnology Carbon Carbon dioxide Catalysis Catalysts Chemical reduction Chemistry and Materials Science Clean energy Clean technology Condensed Matter Physics Conversion Efficiency Electrochemistry Energy Energy conversion Energy conversion efficiency Energy technology Hydrogen evolution reactions Materials Science Metal-organic frameworks Metals Nanotechnology Plasma etching Porosity Precursors Renewable energy Review Article Single atom catalysts Ultrafines |
| title | Metal organic frameworks derived single atom catalysts for electrocatalytic energy conversion |
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