Effect of CeO2-Fe2O3 coated SiO2 nanoparticles on the thermal stability and UV resistance of polyurethane films
In this study, CeO 2 -Fe 2 O 3 coated SiO 2 nanoparticles were prepared by a sol–gel process. One of the prepared nanoparticles was applied in a formulation of polyurethane film for automotive applications. The loading of nanoparticle was varied between 0.1% and 2.0%. First, these films' proper...
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| Veröffentlicht in: | Journal of polymer research 2021, Vol.28 (4), Article 139 |
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| container_title | Journal of polymer research |
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| creator | Dao, Ngoc Nhiem Nguyen, Thi Ha Chi Doan, Trung Dung Pham, Ngoc Chuc Nguyen, Quang Bac Duong, Thi Lim Pham, Ngo Nghia Nguyen, Vu Ngoc Mai Tran, Dai Lam |
| description | In this study, CeO
2
-Fe
2
O
3
coated SiO
2
nanoparticles were prepared by a sol–gel process. One of the prepared nanoparticles was applied in a formulation of polyurethane film for automotive applications. The loading of nanoparticle was varied between 0.1% and 2.0%. First, these films' properties were investigated by using FTIR and thermal gravimetric analysis. Next, these films were subjected to UV exposure testing. The structural changes were characterized by applying FTIR analysis and measuring water contact angle, gloss, and colour deviation. The results indicate that incorporating nanoparticles into the polymer matrix improves the UV-resistance properties of the polymer matrix. Additionally, the nanoparticles enhanced the polymer film's thermal stability until the temperature was 320 °C. Above this temperature, nanoparticles were catalytically active, which accelerated polymer's decomposition giving residue of lower weight percentage. Overall, polyurethane films with nanoparticle loading levels from 0.1 to 1.0 wt% gave the best UV-resistance performance. |
| doi_str_mv | 10.1007/s10965-021-02487-0 |
| format | Article |
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2
-Fe
2
O
3
coated SiO
2
nanoparticles were prepared by a sol–gel process. One of the prepared nanoparticles was applied in a formulation of polyurethane film for automotive applications. The loading of nanoparticle was varied between 0.1% and 2.0%. First, these films' properties were investigated by using FTIR and thermal gravimetric analysis. Next, these films were subjected to UV exposure testing. The structural changes were characterized by applying FTIR analysis and measuring water contact angle, gloss, and colour deviation. The results indicate that incorporating nanoparticles into the polymer matrix improves the UV-resistance properties of the polymer matrix. Additionally, the nanoparticles enhanced the polymer film's thermal stability until the temperature was 320 °C. Above this temperature, nanoparticles were catalytically active, which accelerated polymer's decomposition giving residue of lower weight percentage. Overall, polyurethane films with nanoparticle loading levels from 0.1 to 1.0 wt% gave the best UV-resistance performance.</description><identifier>ISSN: 1022-9760</identifier><identifier>EISSN: 1572-8935</identifier><identifier>DOI: 10.1007/s10965-021-02487-0</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Addition polymerization ; Cerium oxides ; Characterization and Evaluation of Materials ; Chemistry ; Chemistry and Materials Science ; Coating effects ; Contact angle ; Gloss ; Gravimetric analysis ; Industrial Chemistry/Chemical Engineering ; Nanoparticles ; Original Paper ; Polymer Sciences ; Polymers ; Polyurethane resins ; Silicon dioxide ; Sol-gel processes ; Thermal resistance ; Thermal stability</subject><ispartof>Journal of polymer research, 2021, Vol.28 (4), Article 139</ispartof><rights>The Polymer Society, Taipei 2021</rights><rights>The Polymer Society, Taipei 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c356t-b6ddd7e30c4d22797b5bce977714c954fc31aa10074d3b4639e7f7f7f3ee7a343</citedby><cites>FETCH-LOGICAL-c356t-b6ddd7e30c4d22797b5bce977714c954fc31aa10074d3b4639e7f7f7f3ee7a343</cites><orcidid>0000-0002-3638-9201</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10965-021-02487-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10965-021-02487-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27923,27924,41487,42556,51318</link.rule.ids></links><search><creatorcontrib>Dao, Ngoc Nhiem</creatorcontrib><creatorcontrib>Nguyen, Thi Ha Chi</creatorcontrib><creatorcontrib>Doan, Trung Dung</creatorcontrib><creatorcontrib>Pham, Ngoc Chuc</creatorcontrib><creatorcontrib>Nguyen, Quang Bac</creatorcontrib><creatorcontrib>Duong, Thi Lim</creatorcontrib><creatorcontrib>Pham, Ngo Nghia</creatorcontrib><creatorcontrib>Nguyen, Vu Ngoc Mai</creatorcontrib><creatorcontrib>Tran, Dai Lam</creatorcontrib><title>Effect of CeO2-Fe2O3 coated SiO2 nanoparticles on the thermal stability and UV resistance of polyurethane films</title><title>Journal of polymer research</title><addtitle>J Polym Res</addtitle><description>In this study, CeO
2
-Fe
2
O
3
coated SiO
2
nanoparticles were prepared by a sol–gel process. One of the prepared nanoparticles was applied in a formulation of polyurethane film for automotive applications. The loading of nanoparticle was varied between 0.1% and 2.0%. First, these films' properties were investigated by using FTIR and thermal gravimetric analysis. Next, these films were subjected to UV exposure testing. The structural changes were characterized by applying FTIR analysis and measuring water contact angle, gloss, and colour deviation. The results indicate that incorporating nanoparticles into the polymer matrix improves the UV-resistance properties of the polymer matrix. Additionally, the nanoparticles enhanced the polymer film's thermal stability until the temperature was 320 °C. Above this temperature, nanoparticles were catalytically active, which accelerated polymer's decomposition giving residue of lower weight percentage. Overall, polyurethane films with nanoparticle loading levels from 0.1 to 1.0 wt% gave the best UV-resistance performance.</description><subject>Addition polymerization</subject><subject>Cerium oxides</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Coating effects</subject><subject>Contact angle</subject><subject>Gloss</subject><subject>Gravimetric analysis</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Nanoparticles</subject><subject>Original Paper</subject><subject>Polymer Sciences</subject><subject>Polymers</subject><subject>Polyurethane resins</subject><subject>Silicon dioxide</subject><subject>Sol-gel processes</subject><subject>Thermal resistance</subject><subject>Thermal stability</subject><issn>1022-9760</issn><issn>1572-8935</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNp9UE1LAzEQXUTBWv0DngKeo_ncdI9SWhWEPWi9hmx2YrdskzVJD_337lrBmwyPGYb33jCvKG4puaeEqIdESVVKTBgdIRYKk7NiRqVieFFxeT7OhDFcqZJcFlcp7QiRUpWLWRFWzoHNKDi0hJrhNbCaIxtMhha9dTVD3vgwmJg720NCwaO8hQlxb3qUsmm6vstHZHyLNh8oQurGpbcwWQ6hPx4i5K3xgFzX79N1ceFMn-Dmt8-LzXr1vnzGr_XTy_LxFVsuy4ybsm1bBZxY0TKmKtXIxkKllKLCVlI4y6kx0-ui5Y0oeQXKTcUBlOGCz4u7k-8Qw9cBUta7cIh-PKmZJJwqLqQaWezEsjGkFMHpIXZ7E4-aEj2561OwegxW_wSrySjiJ1Eayf4T4p_1P6pvNR57Lw</recordid><startdate>2021</startdate><enddate>2021</enddate><creator>Dao, Ngoc Nhiem</creator><creator>Nguyen, Thi Ha Chi</creator><creator>Doan, Trung Dung</creator><creator>Pham, Ngoc Chuc</creator><creator>Nguyen, Quang Bac</creator><creator>Duong, Thi Lim</creator><creator>Pham, Ngo Nghia</creator><creator>Nguyen, Vu Ngoc Mai</creator><creator>Tran, Dai Lam</creator><general>Springer Netherlands</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope><orcidid>https://orcid.org/0000-0002-3638-9201</orcidid></search><sort><creationdate>2021</creationdate><title>Effect of CeO2-Fe2O3 coated SiO2 nanoparticles on the thermal stability and UV resistance of polyurethane films</title><author>Dao, Ngoc Nhiem ; Nguyen, Thi Ha Chi ; Doan, Trung Dung ; Pham, Ngoc Chuc ; Nguyen, Quang Bac ; Duong, Thi Lim ; Pham, Ngo Nghia ; Nguyen, Vu Ngoc Mai ; Tran, Dai Lam</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c356t-b6ddd7e30c4d22797b5bce977714c954fc31aa10074d3b4639e7f7f7f3ee7a343</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Addition polymerization</topic><topic>Cerium oxides</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Coating effects</topic><topic>Contact angle</topic><topic>Gloss</topic><topic>Gravimetric analysis</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Nanoparticles</topic><topic>Original Paper</topic><topic>Polymer Sciences</topic><topic>Polymers</topic><topic>Polyurethane resins</topic><topic>Silicon dioxide</topic><topic>Sol-gel processes</topic><topic>Thermal resistance</topic><topic>Thermal stability</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Dao, Ngoc Nhiem</creatorcontrib><creatorcontrib>Nguyen, Thi Ha Chi</creatorcontrib><creatorcontrib>Doan, Trung Dung</creatorcontrib><creatorcontrib>Pham, Ngoc Chuc</creatorcontrib><creatorcontrib>Nguyen, Quang Bac</creatorcontrib><creatorcontrib>Duong, Thi Lim</creatorcontrib><creatorcontrib>Pham, Ngo Nghia</creatorcontrib><creatorcontrib>Nguyen, Vu Ngoc Mai</creatorcontrib><creatorcontrib>Tran, Dai Lam</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Journal of polymer research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Dao, Ngoc Nhiem</au><au>Nguyen, Thi Ha Chi</au><au>Doan, Trung Dung</au><au>Pham, Ngoc Chuc</au><au>Nguyen, Quang Bac</au><au>Duong, Thi Lim</au><au>Pham, Ngo Nghia</au><au>Nguyen, Vu Ngoc Mai</au><au>Tran, Dai Lam</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effect of CeO2-Fe2O3 coated SiO2 nanoparticles on the thermal stability and UV resistance of polyurethane films</atitle><jtitle>Journal of polymer research</jtitle><stitle>J Polym Res</stitle><date>2021</date><risdate>2021</risdate><volume>28</volume><issue>4</issue><artnum>139</artnum><issn>1022-9760</issn><eissn>1572-8935</eissn><abstract>In this study, CeO
2
-Fe
2
O
3
coated SiO
2
nanoparticles were prepared by a sol–gel process. One of the prepared nanoparticles was applied in a formulation of polyurethane film for automotive applications. The loading of nanoparticle was varied between 0.1% and 2.0%. First, these films' properties were investigated by using FTIR and thermal gravimetric analysis. Next, these films were subjected to UV exposure testing. The structural changes were characterized by applying FTIR analysis and measuring water contact angle, gloss, and colour deviation. The results indicate that incorporating nanoparticles into the polymer matrix improves the UV-resistance properties of the polymer matrix. Additionally, the nanoparticles enhanced the polymer film's thermal stability until the temperature was 320 °C. Above this temperature, nanoparticles were catalytically active, which accelerated polymer's decomposition giving residue of lower weight percentage. Overall, polyurethane films with nanoparticle loading levels from 0.1 to 1.0 wt% gave the best UV-resistance performance.</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><doi>10.1007/s10965-021-02487-0</doi><orcidid>https://orcid.org/0000-0002-3638-9201</orcidid></addata></record> |
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| subjects | Addition polymerization Cerium oxides Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Coating effects Contact angle Gloss Gravimetric analysis Industrial Chemistry/Chemical Engineering Nanoparticles Original Paper Polymer Sciences Polymers Polyurethane resins Silicon dioxide Sol-gel processes Thermal resistance Thermal stability |
| title | Effect of CeO2-Fe2O3 coated SiO2 nanoparticles on the thermal stability and UV resistance of polyurethane films |
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