Oxyacetylene ablation resistance of continuous gradient ceramic–polymer composite
•A successful preparation of continuous gradient ceramic–polymer gradient composite with a thickness of 40 mm.•Studied the oxyacetylene ablation properties and mechanism of continuous gradient ceramic–polymer composite.•Put forward a novel structure concept for the integrated design of thermal prote...
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Veröffentlicht in: | Corrosion science 2021-02, Vol.179, p.109050, Article 109050 |
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creator | Hu, Zhaocai Meng, Songhe Yi, Fajun Li, Jinping Xu, Chenghai |
description | •A successful preparation of continuous gradient ceramic–polymer gradient composite with a thickness of 40 mm.•Studied the oxyacetylene ablation properties and mechanism of continuous gradient ceramic–polymer composite.•Put forward a novel structure concept for the integrated design of thermal protection system.
In this study, the ablation mechanism and ablation properties of continuous gradient ceramic–polymer composites were studied in an oxyacetylene environment, with the ablation heat flow being 2.38 MW/m2. The samples were prepared through six impregnation–crosslinking–pyrolysis cycles using a three-dimensional seven-directional carbon fiber preform. There were no noticeable ablation pits on the surface of ablated samples. The polysilazane coating and amorphous SiCN ceramics provided good protection for the surface of gradient material. The continuous gradient structure provides a new solution to the problems of thermal mismatch and thermal short-circuit, which are caused by the performance difference between materials. |
doi_str_mv | 10.1016/j.corsci.2020.109050 |
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In this study, the ablation mechanism and ablation properties of continuous gradient ceramic–polymer composites were studied in an oxyacetylene environment, with the ablation heat flow being 2.38 MW/m2. The samples were prepared through six impregnation–crosslinking–pyrolysis cycles using a three-dimensional seven-directional carbon fiber preform. There were no noticeable ablation pits on the surface of ablated samples. The polysilazane coating and amorphous SiCN ceramics provided good protection for the surface of gradient material. The continuous gradient structure provides a new solution to the problems of thermal mismatch and thermal short-circuit, which are caused by the performance difference between materials.</description><identifier>ISSN: 0010-938X</identifier><identifier>EISSN: 1879-0496</identifier><identifier>DOI: 10.1016/j.corsci.2020.109050</identifier><language>eng</language><publisher>Amsterdam: Elsevier Ltd</publisher><subject>A. Ceramic ; Ablation ; Amorphous materials ; B. SEM ; B. XRD ; C. High temperature corrosion ; C. Oxidation ; Carbon fibers ; Ceramic coatings ; Ceramics ; Crosslinking ; Fiber preforms ; Heat transmission ; Oxyacetylene ; Polymer matrix composites ; Polymers ; Polysilazane ; Pyrolysis ; Short circuits ; Thermal mismatch</subject><ispartof>Corrosion science, 2021-02, Vol.179, p.109050, Article 109050</ispartof><rights>2020</rights><rights>Copyright Elsevier BV Feb 2021</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c334t-2b75018e686eb64e8761a9018df39d54e8c15252c1b12569effb4d1607dee4f3</citedby><cites>FETCH-LOGICAL-c334t-2b75018e686eb64e8761a9018df39d54e8c15252c1b12569effb4d1607dee4f3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.corsci.2020.109050$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3548,27922,27923,45993</link.rule.ids></links><search><creatorcontrib>Hu, Zhaocai</creatorcontrib><creatorcontrib>Meng, Songhe</creatorcontrib><creatorcontrib>Yi, Fajun</creatorcontrib><creatorcontrib>Li, Jinping</creatorcontrib><creatorcontrib>Xu, Chenghai</creatorcontrib><title>Oxyacetylene ablation resistance of continuous gradient ceramic–polymer composite</title><title>Corrosion science</title><description>•A successful preparation of continuous gradient ceramic–polymer gradient composite with a thickness of 40 mm.•Studied the oxyacetylene ablation properties and mechanism of continuous gradient ceramic–polymer composite.•Put forward a novel structure concept for the integrated design of thermal protection system.
In this study, the ablation mechanism and ablation properties of continuous gradient ceramic–polymer composites were studied in an oxyacetylene environment, with the ablation heat flow being 2.38 MW/m2. The samples were prepared through six impregnation–crosslinking–pyrolysis cycles using a three-dimensional seven-directional carbon fiber preform. There were no noticeable ablation pits on the surface of ablated samples. The polysilazane coating and amorphous SiCN ceramics provided good protection for the surface of gradient material. The continuous gradient structure provides a new solution to the problems of thermal mismatch and thermal short-circuit, which are caused by the performance difference between materials.</description><subject>A. Ceramic</subject><subject>Ablation</subject><subject>Amorphous materials</subject><subject>B. SEM</subject><subject>B. XRD</subject><subject>C. High temperature corrosion</subject><subject>C. Oxidation</subject><subject>Carbon fibers</subject><subject>Ceramic coatings</subject><subject>Ceramics</subject><subject>Crosslinking</subject><subject>Fiber preforms</subject><subject>Heat transmission</subject><subject>Oxyacetylene</subject><subject>Polymer matrix composites</subject><subject>Polymers</subject><subject>Polysilazane</subject><subject>Pyrolysis</subject><subject>Short circuits</subject><subject>Thermal mismatch</subject><issn>0010-938X</issn><issn>1879-0496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNp9kMtKxDAUhoMoOI6-gYuC644n6S3dCDJ4A2EWzsJdSNNTSWmbmqRid76Db-iTmKGuXR34-f5zOB8hlxQ2FGh-3W6UsU7pDQN2iErI4IisKC_KGNIyPyYrAApxmfDXU3LmXAsQSAor8rL7nKVCP3c4YCSrTnpthsii087LQWFkmkiZwethMpOL3qysNQ4-Umhlr9XP1_dourlHG6h-NE57PCcnjewcXvzNNdnf3-23j_Hz7uFpe_scqyRJfcyqIgPKMec5VnmKvMipLENSN0lZZyFQNGMZU7SiLMtLbJoqrWkORY2YNsmaXC1rR2veJ3RetGayQ7goWMo5sKRIeKDShVLWOGexEaPVvbSzoCAO9kQrFnviYE8s9kLtZqlheOBDoxWBwOCj1haVF7XR_y_4Bd-9fGM</recordid><startdate>202102</startdate><enddate>202102</enddate><creator>Hu, Zhaocai</creator><creator>Meng, Songhe</creator><creator>Yi, Fajun</creator><creator>Li, Jinping</creator><creator>Xu, Chenghai</creator><general>Elsevier Ltd</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SE</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>JG9</scope></search><sort><creationdate>202102</creationdate><title>Oxyacetylene ablation resistance of continuous gradient ceramic–polymer composite</title><author>Hu, Zhaocai ; Meng, Songhe ; Yi, Fajun ; Li, Jinping ; Xu, Chenghai</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c334t-2b75018e686eb64e8761a9018df39d54e8c15252c1b12569effb4d1607dee4f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>A. Ceramic</topic><topic>Ablation</topic><topic>Amorphous materials</topic><topic>B. SEM</topic><topic>B. XRD</topic><topic>C. High temperature corrosion</topic><topic>C. Oxidation</topic><topic>Carbon fibers</topic><topic>Ceramic coatings</topic><topic>Ceramics</topic><topic>Crosslinking</topic><topic>Fiber preforms</topic><topic>Heat transmission</topic><topic>Oxyacetylene</topic><topic>Polymer matrix composites</topic><topic>Polymers</topic><topic>Polysilazane</topic><topic>Pyrolysis</topic><topic>Short circuits</topic><topic>Thermal mismatch</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Hu, Zhaocai</creatorcontrib><creatorcontrib>Meng, Songhe</creatorcontrib><creatorcontrib>Yi, Fajun</creatorcontrib><creatorcontrib>Li, Jinping</creatorcontrib><creatorcontrib>Xu, Chenghai</creatorcontrib><collection>CrossRef</collection><collection>Corrosion Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><jtitle>Corrosion science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Hu, Zhaocai</au><au>Meng, Songhe</au><au>Yi, Fajun</au><au>Li, Jinping</au><au>Xu, Chenghai</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Oxyacetylene ablation resistance of continuous gradient ceramic–polymer composite</atitle><jtitle>Corrosion science</jtitle><date>2021-02</date><risdate>2021</risdate><volume>179</volume><spage>109050</spage><pages>109050-</pages><artnum>109050</artnum><issn>0010-938X</issn><eissn>1879-0496</eissn><abstract>•A successful preparation of continuous gradient ceramic–polymer gradient composite with a thickness of 40 mm.•Studied the oxyacetylene ablation properties and mechanism of continuous gradient ceramic–polymer composite.•Put forward a novel structure concept for the integrated design of thermal protection system.
In this study, the ablation mechanism and ablation properties of continuous gradient ceramic–polymer composites were studied in an oxyacetylene environment, with the ablation heat flow being 2.38 MW/m2. The samples were prepared through six impregnation–crosslinking–pyrolysis cycles using a three-dimensional seven-directional carbon fiber preform. There were no noticeable ablation pits on the surface of ablated samples. The polysilazane coating and amorphous SiCN ceramics provided good protection for the surface of gradient material. The continuous gradient structure provides a new solution to the problems of thermal mismatch and thermal short-circuit, which are caused by the performance difference between materials.</abstract><cop>Amsterdam</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.corsci.2020.109050</doi></addata></record> |
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subjects | A. Ceramic Ablation Amorphous materials B. SEM B. XRD C. High temperature corrosion C. Oxidation Carbon fibers Ceramic coatings Ceramics Crosslinking Fiber preforms Heat transmission Oxyacetylene Polymer matrix composites Polymers Polysilazane Pyrolysis Short circuits Thermal mismatch |
title | Oxyacetylene ablation resistance of continuous gradient ceramic–polymer composite |
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