Two-dimensional modeling investigation of the modern methanol plate reactors

On the presumption that an axial-radial flow pattern (AR) can contribute to a more even distribution of fresh syngas over the catalyst bed, in this study, effects of AR pattern in a mega methanol plate reactor are studied, and the corresponding results are compared with that of fully axial (APR) or...

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Veröffentlicht in:Chemical engineering research & design 2020-10, Vol.162, p.212-227
Hauptverfasser: Eksiri, Z., Mozdianfard, M.R., Mirvakili, A., Rahimpour, M.R.
Format: Artikel
Sprache:eng
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Zusammenfassung:On the presumption that an axial-radial flow pattern (AR) can contribute to a more even distribution of fresh syngas over the catalyst bed, in this study, effects of AR pattern in a mega methanol plate reactor are studied, and the corresponding results are compared with that of fully axial (APR) or radial (RPR) ones. For this purpose, a two-dimensional mathematical model is developed for the AR, while this is one-dimensional for APR and RPR. Afterward, partial differential equations are solved with orthogonal collocation of finite elements method, and the modeling results are compared with industrial data, indicating a good agreement. Besides, the AR reactor is optimized (OAR) using differential evolution (DE) method in order to maximize methanol production. Results demonstrate that the AR can promote methanol production up to 6 and 3% relative to the APR and RPR, respectively. Moreover, in the OAR, 2% and 14°C increase in the feed flow rate and temperature, correspondingly, results in 3.5% improvement in the methanol production.
ISSN:0263-8762
1744-3563
DOI:10.1016/j.cherd.2020.08.009