Random lasing based on plasmonic enhancement from dye-doped capillary tubes with Ag-TiO2 composite nanostructure
•A typical Ag-TiO2 composite nanostructure with broadened plasmon resonance band has been successfully fabricated through solution reduction method.•The broaden LSPR band of the prepared hybrid nanostructure can sufficiently cover both the absorption and emission spectrum of dyes.•The random lasing...
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Veröffentlicht in: | Photonics and nanostructures 2020-12, Vol.42, p.100843, Article 100843 |
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Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | •A typical Ag-TiO2 composite nanostructure with broadened plasmon resonance band has been successfully fabricated through solution reduction method.•The broaden LSPR band of the prepared hybrid nanostructure can sufficiently cover both the absorption and emission spectrum of dyes.•The random lasing device based on the new nanostructure with lower threshold, sharper peak and higher intensity compared to the other devices prepared for reference is proposed.•The results further stimulate the consideration of the plasmon effect in random laser systems and help to design high-performance and cost-effective random laser device.
Plasmonics have allowed revolutionary progress in field of random lasers through improvement of the lasing property via surface plasmon resonance (SPR). However, localized surface plasmon resonance (LSPR) spectra of conventional metal nanostructures are too narrow to sufficiently cover both the absorption and emission spectra of dyes. Therefore, in this paper, we fabricate a typical Ag-TiO2 composite nanostructure by a solution-reduction method and dope it into a random-laser system with a dye solution. With the assistance of this new nanostructure with a broadened plasmon-resonance band, the random-lasing device shows a lower threshold, sharper peak, and higher intensity compared with devices with pure TiO2 nanoparticles (NPs) and mixtures of TiO2 and Ag NPs as scattering media. The results further stimulate consideration of the plasmon effects in random laser systems and help in the design of high-performance, cost-effective random laser devices. |
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ISSN: | 1569-4410 1569-4429 |
DOI: | 10.1016/j.photonics.2020.100843 |