Design, Identification, and Evolution of a Surface Ruthenium(II/III) Single Site for CO Activation

RuII compounds are widely used in catalysis, photocatalysis, and medical applications. They are usually obtained in a reductive environment as molecular O2 can oxidize RuII to RuIII and RuIV. Here we report the design, identification and evolution of an air‐stable surface [bipy‐RuII(CO)2Cl2] site th...

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Veröffentlicht in:	Angewandte Chemie 2021-01, Vol.133 (3), p.1232-1239
Hauptverfasser:	Kang, Liqun, Wang, Bolun, Thetford, Adam, Wu, Ke, Danaie, Mohsen, He, Qian, Gibson, Emma K., Sun, Ling‐Dong, Asakura, Hiroyuki, Catlow, C. Richard A., Wang, Feng Ryan
Format:	Artikel
Sprache:	eng
Schlagworte:	Carbon monoxide Catalysis Catalysts Chemistry Evolution heterogeneous catalysis Infrared spectroscopy Oxidation Ruthenium ruthenium(II/III) complexes single site surface coordination chemistry X-ray absorption spectroscopy
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