Preparation of graphene oxide-modified palygorskite nanocomposites for high-efficient removal of Co(II) from wastewater

Removing Co(II) from wastewater is urgent due to the threat to the environment and human health. In the work, the nanocomposite of graphene oxide-modified palygorskite (mPal-GO) is synthesized by cross-linking one-dimensional palygorskite (Pal) with two-dimensional material graphene oxide (GO), and...

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Veröffentlicht in:Environmental science and pollution research international 2021, Vol.28 (2), p.1919-1932
Hauptverfasser: Mou, Hongmei, Huang, Xiaofeng, Deng, Qiulin, Lei, Qin, Luo, Hong, Liang, Jianhao, Zhang, Xue, Zhang, Tinghong, Yao, Xingjun, Zhang, Lixiong
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container_end_page 1932
container_issue 2
container_start_page 1919
container_title Environmental science and pollution research international
container_volume 28
creator Mou, Hongmei
Huang, Xiaofeng
Deng, Qiulin
Lei, Qin
Luo, Hong
Liang, Jianhao
Zhang, Xue
Zhang, Tinghong
Yao, Xingjun
Zhang, Lixiong
description Removing Co(II) from wastewater is urgent due to the threat to the environment and human health. In the work, the nanocomposite of graphene oxide-modified palygorskite (mPal-GO) is synthesized by cross-linking one-dimensional palygorskite (Pal) with two-dimensional material graphene oxide (GO), and used to remove Co(II) from wastewater. Its structure is characterized by Fourier transformed infrared spectroscopy (FT-IR), X-ray diffraction (XRD), scanning electron microscopy (SEM), and Brunauer-Emmett-Teller (BET) surface area measurement. The parameters, such as mass ratio (GO:mPal), temperature, pH, and contact time, are carefully investigated. The results indicate that pseudo-second-order equation and Langmuir isotherm model are the best fitting one in the adsorption process of Co(II) onto mPal-GO. The maximum adsorption capacity achieves 16.9 mg/g at pH = 6.0 and T  = 298 K according to the Langmuir model analysis. Furthermore, mPal-GO can be reused more than 5 times with a slight decrease according to the adsorption-desorption cycle experiments. Finally, mPal-GO with the low-cost and easy separation is a promising candidate for removing of Co(II) from wastewater.
doi_str_mv 10.1007/s11356-020-07890-6
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In the work, the nanocomposite of graphene oxide-modified palygorskite (mPal-GO) is synthesized by cross-linking one-dimensional palygorskite (Pal) with two-dimensional material graphene oxide (GO), and used to remove Co(II) from wastewater. Its structure is characterized by Fourier transformed infrared spectroscopy (FT-IR), X-ray diffraction (XRD), scanning electron microscopy (SEM), and Brunauer-Emmett-Teller (BET) surface area measurement. The parameters, such as mass ratio (GO:mPal), temperature, pH, and contact time, are carefully investigated. The results indicate that pseudo-second-order equation and Langmuir isotherm model are the best fitting one in the adsorption process of Co(II) onto mPal-GO. The maximum adsorption capacity achieves 16.9 mg/g at pH = 6.0 and T  = 298 K according to the Langmuir model analysis. Furthermore, mPal-GO can be reused more than 5 times with a slight decrease according to the adsorption-desorption cycle experiments. 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In the work, the nanocomposite of graphene oxide-modified palygorskite (mPal-GO) is synthesized by cross-linking one-dimensional palygorskite (Pal) with two-dimensional material graphene oxide (GO), and used to remove Co(II) from wastewater. Its structure is characterized by Fourier transformed infrared spectroscopy (FT-IR), X-ray diffraction (XRD), scanning electron microscopy (SEM), and Brunauer-Emmett-Teller (BET) surface area measurement. The parameters, such as mass ratio (GO:mPal), temperature, pH, and contact time, are carefully investigated. The results indicate that pseudo-second-order equation and Langmuir isotherm model are the best fitting one in the adsorption process of Co(II) onto mPal-GO. The maximum adsorption capacity achieves 16.9 mg/g at pH = 6.0 and T  = 298 K according to the Langmuir model analysis. Furthermore, mPal-GO can be reused more than 5 times with a slight decrease according to the adsorption-desorption cycle experiments. Finally, mPal-GO with the low-cost and easy separation is a promising candidate for removing of Co(II) from wastewater.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>32862342</pmid><doi>10.1007/s11356-020-07890-6</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0002-7660-5589</orcidid></addata></record>
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subjects Adsorption
Aquatic Pollution
Atmospheric Protection/Air Quality Control/Air Pollution
Crosslinking
Earth and Environmental Science
Ecotoxicology
Environment
Environmental Chemistry
Environmental Health
Environmental science
Fourier analysis
Graphene
Graphite
Humans
Infrared spectroscopy
Kinetics
Magnesium Compounds
Nanocomposites
pH effects
Research Article
Scanning electron microscopy
Silicon Compounds
Spectroscopy, Fourier Transform Infrared
Two dimensional materials
Waste Water
Waste Water Technology
Wastewater
Wastewater treatment
Water Management
Water Pollutants, Chemical - analysis
Water Pollution Control
X-ray diffraction
title Preparation of graphene oxide-modified palygorskite nanocomposites for high-efficient removal of Co(II) from wastewater
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