Geochemical assessment and spatial analysis of heavy metals pollution around coal-fired power station
Coal-fired power stations are significant sources of soil contamination with heavy metals and a source of hazard to human health. The soil samples ( n = 25) selected in the area around Novocherkassk Power Station (Rostov Region, Russia) within a radius of up to 20 km revealed the enrichment with Pb...
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creator | Linnik, Vitaly G. Minkina, Tatiana M. Bauer, Tatiana V. Saveliev, Anatoly A. Mandzhieva, Saglara S. |
description | Coal-fired power stations are significant sources of soil contamination with heavy metals and a source of hazard to human health. The soil samples (
n
= 25) selected in the area around Novocherkassk Power Station (Rostov Region, Russia) within a radius of up to 20 km revealed the enrichment with Pb, Cu and Zn. The heavy metals (HM) content in soil is reduced in the following sequence: Mn > Cr > Zn > Ni > Cu > Pb > Co. The correlation diagrams of the HM total content in soils revealed a significant association between the following HM pairs: Cu–Pb, Ni–Cu, Cd–Ni, Cd–Cu (
r
≥ 0.7,
p
|
doi_str_mv | 10.1007/s10653-019-00361-z |
format | Article |
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n
= 25) selected in the area around Novocherkassk Power Station (Rostov Region, Russia) within a radius of up to 20 km revealed the enrichment with Pb, Cu and Zn. The heavy metals (HM) content in soil is reduced in the following sequence: Mn > Cr > Zn > Ni > Cu > Pb > Co. The correlation diagrams of the HM total content in soils revealed a significant association between the following HM pairs: Cu–Pb, Ni–Cu, Cd–Ni, Cd–Cu (
r
≥ 0.7,
p
< 0.001). The concentration coefficient (Kc) and the total pollution coefficient (Zc) were used to estimate anthropogenic pollution. The use of generalized additive model (GAM) to detect the dependence of HM distribution on factors revealed the significance of the source distance. The influence of wind rhumb on HM distribution has a complex nonlinear nature. A GAM shows a good performance for all data sets:
R
2
= 0.71, 81% deviance explained for Zn,
R
2
= 0.85, 91% deviance explained for Cd,
R
2
= 0.63, 70% deviance explained for Ni. Thus, GAM model reveals significant factors (Dist_km, rhumb) in forming pollution by heavy metals in studied impact zone and proved a valuable approach to assess the degree and sources of pollution in soils on a large scale.</description><identifier>ISSN: 0269-4042</identifier><identifier>EISSN: 1573-2983</identifier><identifier>DOI: 10.1007/s10653-019-00361-z</identifier><identifier>PMID: 31264040</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Additives ; Anthropogenic factors ; Cadmium ; Chromium ; Coal ; Coal - analysis ; Coal-fired power plants ; Contamination ; Copper ; Dependence ; Distribution ; Earth and Environmental Science ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental Monitoring ; Geochemistry ; Health hazards ; Heavy metals ; Human influences ; Humans ; Lead ; Manganese ; Metals ; Metals, Heavy - analysis ; Nickel ; Original Paper ; Pollution ; Pollution sources ; Power Plants ; Public Health ; Risk Assessment ; Russia ; Soil ; Soil contamination ; Soil Pollutants - analysis ; Soil pollution ; Soil Science & Conservation ; Spatial Analysis ; Terrestrial Pollution ; Wind ; Wind effects ; Zinc</subject><ispartof>Environmental geochemistry and health, 2020-12, Vol.42 (12), p.4087-4100</ispartof><rights>Springer Nature B.V. 2019</rights><rights>Environmental Geochemistry and Health is a copyright of Springer, (2019). All Rights Reserved.</rights><rights>Springer Nature B.V. 2019.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a426t-32d88990bdde8ada1fc99659bfcd74d3e0854c6fed08cea378d105acdcc99bd43</citedby><cites>FETCH-LOGICAL-a426t-32d88990bdde8ada1fc99659bfcd74d3e0854c6fed08cea378d105acdcc99bd43</cites><orcidid>0000-0001-6000-2209</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10653-019-00361-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10653-019-00361-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31264040$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Linnik, Vitaly G.</creatorcontrib><creatorcontrib>Minkina, Tatiana M.</creatorcontrib><creatorcontrib>Bauer, Tatiana V.</creatorcontrib><creatorcontrib>Saveliev, Anatoly A.</creatorcontrib><creatorcontrib>Mandzhieva, Saglara S.</creatorcontrib><title>Geochemical assessment and spatial analysis of heavy metals pollution around coal-fired power station</title><title>Environmental geochemistry and health</title><addtitle>Environ Geochem Health</addtitle><addtitle>Environ Geochem Health</addtitle><description>Coal-fired power stations are significant sources of soil contamination with heavy metals and a source of hazard to human health. The soil samples (
n
= 25) selected in the area around Novocherkassk Power Station (Rostov Region, Russia) within a radius of up to 20 km revealed the enrichment with Pb, Cu and Zn. The heavy metals (HM) content in soil is reduced in the following sequence: Mn > Cr > Zn > Ni > Cu > Pb > Co. The correlation diagrams of the HM total content in soils revealed a significant association between the following HM pairs: Cu–Pb, Ni–Cu, Cd–Ni, Cd–Cu (
r
≥ 0.7,
p
< 0.001). The concentration coefficient (Kc) and the total pollution coefficient (Zc) were used to estimate anthropogenic pollution. The use of generalized additive model (GAM) to detect the dependence of HM distribution on factors revealed the significance of the source distance. The influence of wind rhumb on HM distribution has a complex nonlinear nature. A GAM shows a good performance for all data sets:
R
2
= 0.71, 81% deviance explained for Zn,
R
2
= 0.85, 91% deviance explained for Cd,
R
2
= 0.63, 70% deviance explained for Ni. Thus, GAM model reveals significant factors (Dist_km, rhumb) in forming pollution by heavy metals in studied impact zone and proved a valuable approach to assess the degree and sources of pollution in soils on a large scale.</description><subject>Additives</subject><subject>Anthropogenic factors</subject><subject>Cadmium</subject><subject>Chromium</subject><subject>Coal</subject><subject>Coal - analysis</subject><subject>Coal-fired power plants</subject><subject>Contamination</subject><subject>Copper</subject><subject>Dependence</subject><subject>Distribution</subject><subject>Earth and Environmental Science</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental Monitoring</subject><subject>Geochemistry</subject><subject>Health hazards</subject><subject>Heavy metals</subject><subject>Human influences</subject><subject>Humans</subject><subject>Lead</subject><subject>Manganese</subject><subject>Metals</subject><subject>Metals, Heavy - analysis</subject><subject>Nickel</subject><subject>Original Paper</subject><subject>Pollution</subject><subject>Pollution sources</subject><subject>Power Plants</subject><subject>Public Health</subject><subject>Risk Assessment</subject><subject>Russia</subject><subject>Soil</subject><subject>Soil contamination</subject><subject>Soil Pollutants - analysis</subject><subject>Soil pollution</subject><subject>Soil Science & Conservation</subject><subject>Spatial Analysis</subject><subject>Terrestrial Pollution</subject><subject>Wind</subject><subject>Wind effects</subject><subject>Zinc</subject><issn>0269-4042</issn><issn>1573-2983</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kEtP3DAQxy1UBNuFL8ChstSz2_EjDx8rVKASUi9wtrz2BIKSeOtJWi2fHi9L2xunkeb_mNGPsQsJXyRA85Uk1JUWIK0A0LUUz0dsJatGC2Vb_YGtQNVWGDDqlH0kegIA25j2hJ1qqeqyhxXDa0zhEcc--IF7IiQacZq5nyKnrZ_7_Xryw4564qnjj-h_7_iIsx-Ib9MwLHOfJu5zWkoiJD-Irs8Yi_YHM6fZ7_UzdtyVAJ6_zTW7v_p-d3kjbn9e_7j8diu8UfUstIptay1sYsTWRy-7YG1d2U0XYmOiRmgrE-oOI7QBvW7aKKHyIYbi20Sj1-zzoXeb068FaXZPacnlfXLKNFo3Riv7rktVoLWUheuaqYMr5ESUsXPb3I8-75wEt-fvDvxd4e9e-bvnEvr0Vr1sRoz_In-BF4M-GKhI0wPm_7ffqX0BmtaSyw</recordid><startdate>20201201</startdate><enddate>20201201</enddate><creator>Linnik, Vitaly G.</creator><creator>Minkina, Tatiana 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B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7ST</scope><scope>7UA</scope><scope>7X7</scope><scope>7XB</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>F1W</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>H97</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>L.G</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>PATMY</scope><scope>PCBAR</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0001-6000-2209</orcidid></search><sort><creationdate>20201201</creationdate><title>Geochemical assessment and spatial analysis of heavy metals pollution around coal-fired power station</title><author>Linnik, Vitaly G. ; Minkina, Tatiana M. ; Bauer, Tatiana V. ; Saveliev, Anatoly A. ; Mandzhieva, Saglara S.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a426t-32d88990bdde8ada1fc99659bfcd74d3e0854c6fed08cea378d105acdcc99bd43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Additives</topic><topic>Anthropogenic factors</topic><topic>Cadmium</topic><topic>Chromium</topic><topic>Coal</topic><topic>Coal - analysis</topic><topic>Coal-fired power plants</topic><topic>Contamination</topic><topic>Copper</topic><topic>Dependence</topic><topic>Distribution</topic><topic>Earth and Environmental Science</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental Monitoring</topic><topic>Geochemistry</topic><topic>Health hazards</topic><topic>Heavy metals</topic><topic>Human influences</topic><topic>Humans</topic><topic>Lead</topic><topic>Manganese</topic><topic>Metals</topic><topic>Metals, Heavy - analysis</topic><topic>Nickel</topic><topic>Original Paper</topic><topic>Pollution</topic><topic>Pollution sources</topic><topic>Power Plants</topic><topic>Public Health</topic><topic>Risk Assessment</topic><topic>Russia</topic><topic>Soil</topic><topic>Soil contamination</topic><topic>Soil Pollutants - analysis</topic><topic>Soil pollution</topic><topic>Soil Science & Conservation</topic><topic>Spatial Analysis</topic><topic>Terrestrial Pollution</topic><topic>Wind</topic><topic>Wind effects</topic><topic>Zinc</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Linnik, Vitaly G.</creatorcontrib><creatorcontrib>Minkina, Tatiana M.</creatorcontrib><creatorcontrib>Bauer, Tatiana 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M.</au><au>Bauer, Tatiana V.</au><au>Saveliev, Anatoly A.</au><au>Mandzhieva, Saglara S.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Geochemical assessment and spatial analysis of heavy metals pollution around coal-fired power station</atitle><jtitle>Environmental geochemistry and health</jtitle><stitle>Environ Geochem Health</stitle><addtitle>Environ Geochem Health</addtitle><date>2020-12-01</date><risdate>2020</risdate><volume>42</volume><issue>12</issue><spage>4087</spage><epage>4100</epage><pages>4087-4100</pages><issn>0269-4042</issn><eissn>1573-2983</eissn><abstract>Coal-fired power stations are significant sources of soil contamination with heavy metals and a source of hazard to human health. The soil samples (
n
= 25) selected in the area around Novocherkassk Power Station (Rostov Region, Russia) within a radius of up to 20 km revealed the enrichment with Pb, Cu and Zn. The heavy metals (HM) content in soil is reduced in the following sequence: Mn > Cr > Zn > Ni > Cu > Pb > Co. The correlation diagrams of the HM total content in soils revealed a significant association between the following HM pairs: Cu–Pb, Ni–Cu, Cd–Ni, Cd–Cu (
r
≥ 0.7,
p
< 0.001). The concentration coefficient (Kc) and the total pollution coefficient (Zc) were used to estimate anthropogenic pollution. The use of generalized additive model (GAM) to detect the dependence of HM distribution on factors revealed the significance of the source distance. The influence of wind rhumb on HM distribution has a complex nonlinear nature. A GAM shows a good performance for all data sets:
R
2
= 0.71, 81% deviance explained for Zn,
R
2
= 0.85, 91% deviance explained for Cd,
R
2
= 0.63, 70% deviance explained for Ni. Thus, GAM model reveals significant factors (Dist_km, rhumb) in forming pollution by heavy metals in studied impact zone and proved a valuable approach to assess the degree and sources of pollution in soils on a large scale.</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><pmid>31264040</pmid><doi>10.1007/s10653-019-00361-z</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0001-6000-2209</orcidid></addata></record> |
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subjects | Additives Anthropogenic factors Cadmium Chromium Coal Coal - analysis Coal-fired power plants Contamination Copper Dependence Distribution Earth and Environmental Science Environment Environmental Chemistry Environmental Health Environmental Monitoring Geochemistry Health hazards Heavy metals Human influences Humans Lead Manganese Metals Metals, Heavy - analysis Nickel Original Paper Pollution Pollution sources Power Plants Public Health Risk Assessment Russia Soil Soil contamination Soil Pollutants - analysis Soil pollution Soil Science & Conservation Spatial Analysis Terrestrial Pollution Wind Wind effects Zinc |
title | Geochemical assessment and spatial analysis of heavy metals pollution around coal-fired power station |
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