Effects of spatially-varying substrate anchoring on instabilities and dewetting of thin nematic liquid crystal films
Partially wetting nematic liquid crystal (NLC) films on substrates are unstable to dewetting-type instabilities due to destabilizing solid/NLC interaction forces. These instabilities are modified by the nematic nature of the films, which influences the effective solid/NLC interaction. In this work,...
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description | Partially wetting nematic liquid crystal (NLC) films on substrates are unstable to dewetting-type instabilities due to destabilizing solid/NLC interaction forces. These instabilities are modified by the nematic nature of the films, which influences the effective solid/NLC interaction. In this work, we focus on the influence of imposed substrate anchoring on the instability development. The analysis is carried out within a long-wave formulation based on the Leslie-Ericksen description of NLC films. Linear stability analysis of the resulting equations shows that some features of the instability, such as emerging wavelengths, may not be influenced by the imposed substrate anchoring. Going further into the nonlinear regime, considered
via
large-scale GPU-based simulations, shows however that nonlinear effects may play an important role, in particular in the case of strong substrate anchoring anisotropy. Our simulations show that instability of the film develops in two stages: the first stage involves formation of ridges that are perpendicular to the local anchoring direction; and the second involves breakup of these ridges and formation of drops, whose final distribution is influenced by the anisotropy imposed by the substrate. Finally, we show that imposing more complex substrate anisotropy patterns allows us to reach basic understanding of the influence of substrate-imposed defects in director orientation on the instability evolution.
We investigate (theoretically and numerically) free surface evolution of nematic liquid crystal films in the presence of variable substrate anchoring. |
doi_str_mv | 10.1039/d0sm01416h |
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via
large-scale GPU-based simulations, shows however that nonlinear effects may play an important role, in particular in the case of strong substrate anchoring anisotropy. Our simulations show that instability of the film develops in two stages: the first stage involves formation of ridges that are perpendicular to the local anchoring direction; and the second involves breakup of these ridges and formation of drops, whose final distribution is influenced by the anisotropy imposed by the substrate. Finally, we show that imposing more complex substrate anisotropy patterns allows us to reach basic understanding of the influence of substrate-imposed defects in director orientation on the instability evolution.
We investigate (theoretically and numerically) free surface evolution of nematic liquid crystal films in the presence of variable substrate anchoring.</description><identifier>ISSN: 1744-683X</identifier><identifier>EISSN: 1744-6848</identifier><identifier>DOI: 10.1039/d0sm01416h</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Anchoring ; Anisotropy ; Crystal defects ; Drying ; Instability ; Liquid crystals ; Nematic crystals ; Ridges ; Stability ; Stability analysis ; Substrates ; Thin films ; Wavelengths ; Wetting</subject><ispartof>Soft matter, 2020-11, Vol.16 (44), p.1187-1197</ispartof><rights>Copyright Royal Society of Chemistry 2020</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c351t-9a9f28468795e93bff8942bac517303238bb083ce8afd69cb1242db7f09829a23</citedby><cites>FETCH-LOGICAL-c351t-9a9f28468795e93bff8942bac517303238bb083ce8afd69cb1242db7f09829a23</cites><orcidid>0000-0002-5052-0114 ; 0000-0002-7783-2126 ; 0000-0001-6966-9851</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Lam, Michael-Angelo Y.-H</creatorcontrib><creatorcontrib>Kondic, Lou</creatorcontrib><creatorcontrib>Cummings, Linda J</creatorcontrib><title>Effects of spatially-varying substrate anchoring on instabilities and dewetting of thin nematic liquid crystal films</title><title>Soft matter</title><description>Partially wetting nematic liquid crystal (NLC) films on substrates are unstable to dewetting-type instabilities due to destabilizing solid/NLC interaction forces. These instabilities are modified by the nematic nature of the films, which influences the effective solid/NLC interaction. In this work, we focus on the influence of imposed substrate anchoring on the instability development. The analysis is carried out within a long-wave formulation based on the Leslie-Ericksen description of NLC films. Linear stability analysis of the resulting equations shows that some features of the instability, such as emerging wavelengths, may not be influenced by the imposed substrate anchoring. Going further into the nonlinear regime, considered
via
large-scale GPU-based simulations, shows however that nonlinear effects may play an important role, in particular in the case of strong substrate anchoring anisotropy. Our simulations show that instability of the film develops in two stages: the first stage involves formation of ridges that are perpendicular to the local anchoring direction; and the second involves breakup of these ridges and formation of drops, whose final distribution is influenced by the anisotropy imposed by the substrate. Finally, we show that imposing more complex substrate anisotropy patterns allows us to reach basic understanding of the influence of substrate-imposed defects in director orientation on the instability evolution.
We investigate (theoretically and numerically) free surface evolution of nematic liquid crystal films in the presence of variable substrate anchoring.</description><subject>Anchoring</subject><subject>Anisotropy</subject><subject>Crystal defects</subject><subject>Drying</subject><subject>Instability</subject><subject>Liquid crystals</subject><subject>Nematic crystals</subject><subject>Ridges</subject><subject>Stability</subject><subject>Stability analysis</subject><subject>Substrates</subject><subject>Thin films</subject><subject>Wavelengths</subject><subject>Wetting</subject><issn>1744-683X</issn><issn>1744-6848</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNpd0c1LwzAYBvAiCur04l0IeBGhmq-2yVH8BsWDCt5KmiYuI21n3lTZf2-2yQRPCXl_eQh5suyI4HOCmbxoMXSYcFJOt7I9UnGel4KL7c2eve9m-wAzjJlIai-LN9YaHQENFsFcRae8X-RfKixc_4FgbCAGFQ1SvZ4OYXk29Mj1EFXjvIvOQBq1qDXfJsbV2KI4dT3qTZfSNPLuc3Qt0mGR7nhkne_gINuxyoM5_F0n2dvtzevVff74fPdwdfmYa1aQmEslLRW8FJUsjGSNtUJy2ihdkIphRploGiyYNkLZtpS6IZTTtqksloJKRdkkO13nzsPwORqIdedAG-9Vb4YRasoLznFVsiLRk390NoyhT69LqqQySbkMPFsrHQaAYGw9D65Ln1UTXC8LqK_xy9OqgPuEj9c4gN64v4LYD77dg_8</recordid><startdate>20201118</startdate><enddate>20201118</enddate><creator>Lam, Michael-Angelo Y.-H</creator><creator>Kondic, Lou</creator><creator>Cummings, Linda J</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QO</scope><scope>7QQ</scope><scope>7SC</scope><scope>7SE</scope><scope>7SP</scope><scope>7SR</scope><scope>7TA</scope><scope>7TB</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>JG9</scope><scope>JQ2</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>P64</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-5052-0114</orcidid><orcidid>https://orcid.org/0000-0002-7783-2126</orcidid><orcidid>https://orcid.org/0000-0001-6966-9851</orcidid></search><sort><creationdate>20201118</creationdate><title>Effects of spatially-varying substrate anchoring on instabilities and dewetting of thin nematic liquid crystal films</title><author>Lam, Michael-Angelo Y.-H ; Kondic, Lou ; Cummings, Linda J</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c351t-9a9f28468795e93bff8942bac517303238bb083ce8afd69cb1242db7f09829a23</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Anchoring</topic><topic>Anisotropy</topic><topic>Crystal defects</topic><topic>Drying</topic><topic>Instability</topic><topic>Liquid crystals</topic><topic>Nematic crystals</topic><topic>Ridges</topic><topic>Stability</topic><topic>Stability analysis</topic><topic>Substrates</topic><topic>Thin films</topic><topic>Wavelengths</topic><topic>Wetting</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lam, Michael-Angelo Y.-H</creatorcontrib><creatorcontrib>Kondic, Lou</creatorcontrib><creatorcontrib>Cummings, Linda J</creatorcontrib><collection>CrossRef</collection><collection>Aluminium Industry Abstracts</collection><collection>Biotechnology Research Abstracts</collection><collection>Ceramic Abstracts</collection><collection>Computer and Information Systems Abstracts</collection><collection>Corrosion Abstracts</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Materials Business File</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Copper Technical Reference Library</collection><collection>Materials Research Database</collection><collection>ProQuest Computer Science Collection</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Computer and Information Systems Abstracts Academic</collection><collection>Computer and Information Systems Abstracts Professional</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Soft matter</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lam, Michael-Angelo Y.-H</au><au>Kondic, Lou</au><au>Cummings, Linda J</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of spatially-varying substrate anchoring on instabilities and dewetting of thin nematic liquid crystal films</atitle><jtitle>Soft matter</jtitle><date>2020-11-18</date><risdate>2020</risdate><volume>16</volume><issue>44</issue><spage>1187</spage><epage>1197</epage><pages>1187-1197</pages><issn>1744-683X</issn><eissn>1744-6848</eissn><abstract>Partially wetting nematic liquid crystal (NLC) films on substrates are unstable to dewetting-type instabilities due to destabilizing solid/NLC interaction forces. These instabilities are modified by the nematic nature of the films, which influences the effective solid/NLC interaction. In this work, we focus on the influence of imposed substrate anchoring on the instability development. The analysis is carried out within a long-wave formulation based on the Leslie-Ericksen description of NLC films. Linear stability analysis of the resulting equations shows that some features of the instability, such as emerging wavelengths, may not be influenced by the imposed substrate anchoring. Going further into the nonlinear regime, considered
via
large-scale GPU-based simulations, shows however that nonlinear effects may play an important role, in particular in the case of strong substrate anchoring anisotropy. Our simulations show that instability of the film develops in two stages: the first stage involves formation of ridges that are perpendicular to the local anchoring direction; and the second involves breakup of these ridges and formation of drops, whose final distribution is influenced by the anisotropy imposed by the substrate. Finally, we show that imposing more complex substrate anisotropy patterns allows us to reach basic understanding of the influence of substrate-imposed defects in director orientation on the instability evolution.
We investigate (theoretically and numerically) free surface evolution of nematic liquid crystal films in the presence of variable substrate anchoring.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d0sm01416h</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-5052-0114</orcidid><orcidid>https://orcid.org/0000-0002-7783-2126</orcidid><orcidid>https://orcid.org/0000-0001-6966-9851</orcidid></addata></record> |
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subjects | Anchoring Anisotropy Crystal defects Drying Instability Liquid crystals Nematic crystals Ridges Stability Stability analysis Substrates Thin films Wavelengths Wetting |
title | Effects of spatially-varying substrate anchoring on instabilities and dewetting of thin nematic liquid crystal films |
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