Design and synthesis of an amide-containing crosslinked network based on Diels-Alder chemistry for fully recyclable aramid fabric reinforced composites
Fiber reinforced thermoset composites (FRPCs) have received tremendous attention because of their merits of light weight, high modulus and high strength. However, the efficient recycling of the waste during the manufacturing and service life of FRPCs is still great challenge. This paper reports a ne...
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| Veröffentlicht in: | Composites science and technology 2020-09, Vol.197, p.108280, Article 108280 |
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| creator | Zhou, Danling Huang, Hong Wang, Yan Yu, Junrong Hu, Zuming |
| description | Fiber reinforced thermoset composites (FRPCs) have received tremendous attention because of their merits of light weight, high modulus and high strength. However, the efficient recycling of the waste during the manufacturing and service life of FRPCs is still great challenge. This paper reports a newly designed dynamic crosslinked network based on Diels-Alder chemistry as matrix for fully recyclable aramid fabric reinforced composites. The DA network shows good thermomechanical properties owing to the incorporated aromatic amide bonds, and the overall performance can be readily tailored by adjusting the ratio of amide-containing component and flexible aliphatic component. The good reversibility of the DA network and highly efficient recovery of mechanical properties of recycled sample are confirmed. With optimized composition, the DA network exhibits good interfacial strength with aramid fiber that is comparable to that of widely used epoxy resin due to the interfacial hydrogen bonds among amide bonds between fiber and matrix. Moreover, the closed-loop recycling of both matrix and reinforced fabric without any other additive is also demonstrated. This paper presents the first report on recyclable aramid fiber reinforced composites and is expected to provide hints for future development of fully recyclable and high-performance FRPCs.
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| doi_str_mv | 10.1016/j.compscitech.2020.108280 |
| format | Article |
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[Display omitted]</description><subject>Aramid fiber reinforced plastics</subject><subject>Crosslinking</subject><subject>Crosslinking polymerization</subject><subject>Diels-Alder reaction</subject><subject>Epoxy resins</subject><subject>Fiber composites</subject><subject>Fiber reinforced composites</subject><subject>Fiber reinforced polymers</subject><subject>Hydrogen bonds</subject><subject>Interfacial strength</subject><subject>Mechanical properties</subject><subject>Polymer matrix composites</subject><subject>Polymer-matrix composites (PMCs)</subject><subject>Recovering</subject><subject>Recycling</subject><subject>Service life</subject><subject>Thermomechanical properties</subject><subject>Thermosetting resins</subject><subject>Weight reduction</subject><issn>0266-3538</issn><issn>1879-1050</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNqNUcFu1DAQtRCVupT-gxHnLHZix86x2kJBqsQFzpYzHne9zdqLnQXlS_jdOiwHjpxGM_Pmjd57hLzjbMsZ7z8ctpCOpwJhRthvW9auc91q9opsuFZDw5lkr8mGtX3fdLLT1-RNKQfGmJJDuyG_77GEp0htdLQscd7XttDk64DaY3DYQIqzDTHEJwo5lTKF-IyORpx_pfxMR1tqlyK9DziV5m5ymCns8RjKnBfqU6b-PE0LzQgLTHackNq8UlNvxxygLkKsMKg0q5ZUqpbyllx5OxW8_VtvyPdPH7_tPjePXx--7O4eGxBczo100HvQ46gGLpTrFNO8HZzWaLWUoJRFK3g3CrDAQTuPzCshobfdoLjH7oa8v_CecvpxxjKbQzrnWF-aVgglVdcJUVHDBfXHgYzenHI42rwYzsyagzmYf3Iwaw7mkkO93V1uqz34M2A2FYWxyg3Vktm4FP6D5QWAgJtp</recordid><startdate>20200908</startdate><enddate>20200908</enddate><creator>Zhou, Danling</creator><creator>Huang, Hong</creator><creator>Wang, Yan</creator><creator>Yu, Junrong</creator><creator>Hu, Zuming</creator><general>Elsevier Ltd</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope></search><sort><creationdate>20200908</creationdate><title>Design and synthesis of an amide-containing crosslinked network based on Diels-Alder chemistry for fully recyclable aramid fabric reinforced composites</title><author>Zhou, Danling ; Huang, Hong ; Wang, Yan ; Yu, Junrong ; Hu, Zuming</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c415t-5dc6fc8bb79147d3708129d88ea855c77aea413b4cac1c8dfe0f745c6a3971fe3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Aramid fiber reinforced plastics</topic><topic>Crosslinking</topic><topic>Crosslinking polymerization</topic><topic>Diels-Alder reaction</topic><topic>Epoxy resins</topic><topic>Fiber composites</topic><topic>Fiber reinforced composites</topic><topic>Fiber reinforced polymers</topic><topic>Hydrogen bonds</topic><topic>Interfacial strength</topic><topic>Mechanical properties</topic><topic>Polymer matrix composites</topic><topic>Polymer-matrix composites (PMCs)</topic><topic>Recovering</topic><topic>Recycling</topic><topic>Service life</topic><topic>Thermomechanical properties</topic><topic>Thermosetting resins</topic><topic>Weight reduction</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhou, Danling</creatorcontrib><creatorcontrib>Huang, Hong</creatorcontrib><creatorcontrib>Wang, Yan</creatorcontrib><creatorcontrib>Yu, Junrong</creatorcontrib><creatorcontrib>Hu, Zuming</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Composites science and technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhou, Danling</au><au>Huang, Hong</au><au>Wang, Yan</au><au>Yu, Junrong</au><au>Hu, Zuming</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Design and synthesis of an amide-containing crosslinked network based on Diels-Alder chemistry for fully recyclable aramid fabric reinforced composites</atitle><jtitle>Composites science and technology</jtitle><date>2020-09-08</date><risdate>2020</risdate><volume>197</volume><spage>108280</spage><pages>108280-</pages><artnum>108280</artnum><issn>0266-3538</issn><eissn>1879-1050</eissn><abstract>Fiber reinforced thermoset composites (FRPCs) have received tremendous attention because of their merits of light weight, high modulus and high strength. However, the efficient recycling of the waste during the manufacturing and service life of FRPCs is still great challenge. This paper reports a newly designed dynamic crosslinked network based on Diels-Alder chemistry as matrix for fully recyclable aramid fabric reinforced composites. The DA network shows good thermomechanical properties owing to the incorporated aromatic amide bonds, and the overall performance can be readily tailored by adjusting the ratio of amide-containing component and flexible aliphatic component. The good reversibility of the DA network and highly efficient recovery of mechanical properties of recycled sample are confirmed. With optimized composition, the DA network exhibits good interfacial strength with aramid fiber that is comparable to that of widely used epoxy resin due to the interfacial hydrogen bonds among amide bonds between fiber and matrix. Moreover, the closed-loop recycling of both matrix and reinforced fabric without any other additive is also demonstrated. This paper presents the first report on recyclable aramid fiber reinforced composites and is expected to provide hints for future development of fully recyclable and high-performance FRPCs.
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| ispartof | Composites science and technology, 2020-09, Vol.197, p.108280, Article 108280 |
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| source | Elsevier ScienceDirect Journals |
| subjects | Aramid fiber reinforced plastics Crosslinking Crosslinking polymerization Diels-Alder reaction Epoxy resins Fiber composites Fiber reinforced composites Fiber reinforced polymers Hydrogen bonds Interfacial strength Mechanical properties Polymer matrix composites Polymer-matrix composites (PMCs) Recovering Recycling Service life Thermomechanical properties Thermosetting resins Weight reduction |
| title | Design and synthesis of an amide-containing crosslinked network based on Diels-Alder chemistry for fully recyclable aramid fabric reinforced composites |
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