Optimization of the Thermodynamic Properties of the Sm2O3–Y2O3–HfO2 System at High Temperatures by the Barker Method
The thermodynamic properties of the Sm 2 O 3 –Y 2 O 3 –HfO 2 system at 2500 K were modeled based on the generalized lattice theory of associated solutions using experimental data obtained by high-temperature mass spectrometry. A comparison was made between the results of the calculations of the ther...
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| Veröffentlicht in: | Russian journal of inorganic chemistry 2020-05, Vol.65 (5), p.773-780 |
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| container_title | Russian journal of inorganic chemistry |
| container_volume | 65 |
| creator | Shilov, A. L. Stolyarova, V. L. Vorozhtcov, V. A. Lopatin, S. I. Shugurov, S. M. |
| description | The thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system at 2500 K were modeled based on the generalized lattice theory of associated solutions using experimental data obtained by high-temperature mass spectrometry. A comparison was made between the results of the calculations of the thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system using two independent approaches to modeling based on this theory: from the experimental data on the properties of the ternary system and from the data on its boundary binary systems Sm
2
O
3
–Y
2
O
3
, Sm
2
O
3
–HfO
2
, and Y
2
O
3
–HfO
2
. It was shown that the chemical potentials of the components that were calculated in the studied ternary system using the above approaches much better fit the experimental data in the former case. |
| doi_str_mv | 10.1134/S0036023620050216 |
| format | Article |
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2
O
3
–Y
2
O
3
–HfO
2
system at 2500 K were modeled based on the generalized lattice theory of associated solutions using experimental data obtained by high-temperature mass spectrometry. A comparison was made between the results of the calculations of the thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system using two independent approaches to modeling based on this theory: from the experimental data on the properties of the ternary system and from the data on its boundary binary systems Sm
2
O
3
–Y
2
O
3
, Sm
2
O
3
–HfO
2
, and Y
2
O
3
–HfO
2
. It was shown that the chemical potentials of the components that were calculated in the studied ternary system using the above approaches much better fit the experimental data in the former case.</description><identifier>ISSN: 0036-0236</identifier><identifier>EISSN: 1531-8613</identifier><identifier>DOI: 10.1134/S0036023620050216</identifier><language>eng</language><publisher>Moscow: Pleiades Publishing</publisher><subject>Binary systems ; Chemistry ; Chemistry and Materials Science ; Hafnium oxide ; High temperature ; Inorganic Chemistry ; Lattice theory ; Mass spectrometry ; Optimization ; Ternary systems ; Thermodynamic properties ; Thermodynamics of Inorganic Compounds ; Yttrium oxide</subject><ispartof>Russian journal of inorganic chemistry, 2020-05, Vol.65 (5), p.773-780</ispartof><rights>Pleiades Publishing, Ltd. 2020</rights><rights>Pleiades Publishing, Ltd. 2020.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c2316-b9dced53e677bb8cd1d7c31f3b7e9d867eecd0af75fe19a74def13ffee983a103</citedby><cites>FETCH-LOGICAL-c2316-b9dced53e677bb8cd1d7c31f3b7e9d867eecd0af75fe19a74def13ffee983a103</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1134/S0036023620050216$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1134/S0036023620050216$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,777,781,27905,27906,41469,42538,51300</link.rule.ids></links><search><creatorcontrib>Shilov, A. L.</creatorcontrib><creatorcontrib>Stolyarova, V. L.</creatorcontrib><creatorcontrib>Vorozhtcov, V. A.</creatorcontrib><creatorcontrib>Lopatin, S. I.</creatorcontrib><creatorcontrib>Shugurov, S. M.</creatorcontrib><title>Optimization of the Thermodynamic Properties of the Sm2O3–Y2O3–HfO2 System at High Temperatures by the Barker Method</title><title>Russian journal of inorganic chemistry</title><addtitle>Russ. J. Inorg. Chem</addtitle><description>The thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system at 2500 K were modeled based on the generalized lattice theory of associated solutions using experimental data obtained by high-temperature mass spectrometry. A comparison was made between the results of the calculations of the thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system using two independent approaches to modeling based on this theory: from the experimental data on the properties of the ternary system and from the data on its boundary binary systems Sm
2
O
3
–Y
2
O
3
, Sm
2
O
3
–HfO
2
, and Y
2
O
3
–HfO
2
. It was shown that the chemical potentials of the components that were calculated in the studied ternary system using the above approaches much better fit the experimental data in the former case.</description><subject>Binary systems</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Hafnium oxide</subject><subject>High temperature</subject><subject>Inorganic Chemistry</subject><subject>Lattice theory</subject><subject>Mass spectrometry</subject><subject>Optimization</subject><subject>Ternary systems</subject><subject>Thermodynamic properties</subject><subject>Thermodynamics of Inorganic Compounds</subject><subject>Yttrium oxide</subject><issn>0036-0236</issn><issn>1531-8613</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp1kL1OwzAcxC0EEqXwAGyWmAP-SOJkhAooUlGQWgamyIn_blJIXGxXIky8A2_Ik5ASEANiuuHudycdQseUnFLKw7M5ITwmjMeMkIgwGu-gEY04DZKY8l002trB1t9HB86tCAlDIpIResnWvm7qV-lr02Kjsa8ALyqwjVFdK5u6xHfWrMH6GtyPP29Yxj_e3h8GmeqM4XnnPDRYejytlxVeQNND0m9sjxXdF3Yh7SNYfAu-MuoQ7Wn55ODoW8fo_upyMZkGs-z6ZnI-C0rGaRwUqSpBRRxiIYoiKRVVouRU80JAqpJYAJSKSC0iDTSVIlSgKdcaIE24pISP0cnQu7bmeQPO5yuzsW0_mbOQpImIaCT6FB1SpTXOWdD52taNtF1OSb49OP9zcM-wgXF9tl2C_W3-H_oE8sx_WA</recordid><startdate>20200501</startdate><enddate>20200501</enddate><creator>Shilov, A. L.</creator><creator>Stolyarova, V. L.</creator><creator>Vorozhtcov, V. A.</creator><creator>Lopatin, S. I.</creator><creator>Shugurov, S. M.</creator><general>Pleiades Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20200501</creationdate><title>Optimization of the Thermodynamic Properties of the Sm2O3–Y2O3–HfO2 System at High Temperatures by the Barker Method</title><author>Shilov, A. L. ; Stolyarova, V. L. ; Vorozhtcov, V. A. ; Lopatin, S. I. ; Shugurov, S. M.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c2316-b9dced53e677bb8cd1d7c31f3b7e9d867eecd0af75fe19a74def13ffee983a103</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Binary systems</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Hafnium oxide</topic><topic>High temperature</topic><topic>Inorganic Chemistry</topic><topic>Lattice theory</topic><topic>Mass spectrometry</topic><topic>Optimization</topic><topic>Ternary systems</topic><topic>Thermodynamic properties</topic><topic>Thermodynamics of Inorganic Compounds</topic><topic>Yttrium oxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shilov, A. L.</creatorcontrib><creatorcontrib>Stolyarova, V. L.</creatorcontrib><creatorcontrib>Vorozhtcov, V. A.</creatorcontrib><creatorcontrib>Lopatin, S. I.</creatorcontrib><creatorcontrib>Shugurov, S. M.</creatorcontrib><collection>CrossRef</collection><jtitle>Russian journal of inorganic chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Shilov, A. L.</au><au>Stolyarova, V. L.</au><au>Vorozhtcov, V. A.</au><au>Lopatin, S. I.</au><au>Shugurov, S. M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Optimization of the Thermodynamic Properties of the Sm2O3–Y2O3–HfO2 System at High Temperatures by the Barker Method</atitle><jtitle>Russian journal of inorganic chemistry</jtitle><stitle>Russ. J. Inorg. Chem</stitle><date>2020-05-01</date><risdate>2020</risdate><volume>65</volume><issue>5</issue><spage>773</spage><epage>780</epage><pages>773-780</pages><issn>0036-0236</issn><eissn>1531-8613</eissn><abstract>The thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system at 2500 K were modeled based on the generalized lattice theory of associated solutions using experimental data obtained by high-temperature mass spectrometry. A comparison was made between the results of the calculations of the thermodynamic properties of the Sm
2
O
3
–Y
2
O
3
–HfO
2
system using two independent approaches to modeling based on this theory: from the experimental data on the properties of the ternary system and from the data on its boundary binary systems Sm
2
O
3
–Y
2
O
3
, Sm
2
O
3
–HfO
2
, and Y
2
O
3
–HfO
2
. It was shown that the chemical potentials of the components that were calculated in the studied ternary system using the above approaches much better fit the experimental data in the former case.</abstract><cop>Moscow</cop><pub>Pleiades Publishing</pub><doi>10.1134/S0036023620050216</doi><tpages>8</tpages></addata></record> |
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| issn | 0036-0236 1531-8613 |
| language | eng |
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| source | SpringerLink Journals |
| subjects | Binary systems Chemistry Chemistry and Materials Science Hafnium oxide High temperature Inorganic Chemistry Lattice theory Mass spectrometry Optimization Ternary systems Thermodynamic properties Thermodynamics of Inorganic Compounds Yttrium oxide |
| title | Optimization of the Thermodynamic Properties of the Sm2O3–Y2O3–HfO2 System at High Temperatures by the Barker Method |
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