Separation of CO2/N2 mixture by vacuum pressure swing adsorption (VPSA) using zeolite 13X type and carbon molecular sieve adsorbents

Separation of carbon dioxide in flue gases from the combustion equipment is one of the most serious concerns for industries and especially for the power plants which are the main producers of this pollutant gas. From the various separation methods, vacuum pressure swing adsorption (VPSA) process is...

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Veröffentlicht in:Heat and mass transfer 2020, Vol.56 (6), p.1985-1994
Hauptverfasser: Alibolandi, Mehdi, Sadrameli, Seyed Mojtaba, Rezaee, Fatemeh, Darian, Jafar Towfighi
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container_end_page 1994
container_issue 6
container_start_page 1985
container_title Heat and mass transfer
container_volume 56
creator Alibolandi, Mehdi
Sadrameli, Seyed Mojtaba
Rezaee, Fatemeh
Darian, Jafar Towfighi
description Separation of carbon dioxide in flue gases from the combustion equipment is one of the most serious concerns for industries and especially for the power plants which are the main producers of this pollutant gas. From the various separation methods, vacuum pressure swing adsorption (VPSA) process is attracted interest due to its lower energy consumption and high efficiency. A VPSA process was studied for the separation of a mixture of CO 2 /N 2 (80% N 2 and 20% CO 2 ). Experiments were performed in an eight-step, four-bed setup using zeolite 13X and carbon molecular sieve (CMS) as adsorbents. Experimental measurements by the bench-scale system have been obtained in a pressure range of 2.7–4.7 bar, cycle times of 360–600 s, the product flow rate of 1–3 (lit/min), and temperature 30 °C. The effects of pressure, cycle time, and product flow rate were investigated. With using 560 s for a cycle time at 3.7 bar, the maximum purity of 97.6% was obtained for zeolite 13X adsorbent.
doi_str_mv 10.1007/s00231-020-02823-y
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subjects Adsorbents
Carbon dioxide
Cycle time
Electric power generation
Energy consumption
Engineering
Engineering Thermodynamics
Flow velocity
Flue gas
Heat and Mass Transfer
Industrial Chemistry/Chemical Engineering
Industrial plants
Molecular sieves
Original Article
Pollutants
Power plants
Pressure effects
Pressure swing adsorption
Separation
Thermodynamics
Zeolites
title Separation of CO2/N2 mixture by vacuum pressure swing adsorption (VPSA) using zeolite 13X type and carbon molecular sieve adsorbents
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