One-pot synthesis of Mn3O4-coupled Ag2WO4 nanocomposite photocatalyst for enhanced photooxidative desulfurization of thiophene under visible light irradiation
The photooxidative desulfurization of thiophene (ThP) becomes a challenge in both industry and environmental remediation. Herein, we synthesize a visible-light-responsive Ag 2 WO 4 /Mn 3 O 4 nanocomposite by a one-pot strategy. Depiction of the produced photocatalysts exposed the suppression of the...
Gespeichert in:
| Veröffentlicht in: | Applied nanoscience 2020-05, Vol.10 (5), p.1545-1554 |
|---|---|
| Hauptverfasser: | , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 1554 |
|---|---|
| container_issue | 5 |
| container_start_page | 1545 |
| container_title | Applied nanoscience |
| container_volume | 10 |
| creator | Shawky, Ahmed Mohamed, R. M. Mkhalid, I. A. Awwad, Nasser S. Ibrahium, Hala A. |
| description | The photooxidative desulfurization of thiophene (ThP) becomes a challenge in both industry and environmental remediation. Herein, we synthesize a visible-light-responsive Ag
2
WO
4
/Mn
3
O
4
nanocomposite by a one-pot strategy. Depiction of the produced photocatalysts exposed the suppression of the surface structure and reduction of the bandgap energy by adding 15 wt% of Mn
3
O
4
to Ag
2
WO
4
. The obtained nanocomposite shows a complete photooxidation of ThP within 1 h under visible light illumination at a dose of 1.2 g L
−1
. The significance of photocatalytic performance of Ag
2
WO
4
/Mn
3
O
4
nanocomposite photocatalyst is referred to the enhancement of the visible light absorption and overthrow of the recombination of photogenerated charge carriers. The study opens the door for extensive use of nanocomposite photocatalysts as a novel functional material for the photooxidation of ThPs under visible light exposure. |
| doi_str_mv | 10.1007/s13204-019-01212-0 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2393609226</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2393609226</sourcerecordid><originalsourceid>FETCH-LOGICAL-c466t-419bf8d1671c55030c796f91f40416d67870b115490463906f795a6adf52d3ab3</originalsourceid><addsrcrecordid>eNp9kc1KxDAUhYsoKOoLuAq4rt78NDVLEf9AmY3iMmSaZJqhJjVJxfFhfFYzM6I7L4R7Q75zLuFU1QmGMwzQnidMCbAasCiHYFLDTnVAsIC6aXC7-zuD2K-OU1pCqYa1nDYH1dfMm3oMGaWVz71JLqFg0aOnM1Z3YRoHo9HlgrzMGPLKhy68jiG5bNDYhxw6ldWwShnZEJHxvfJd4TdP4cNpld27QdqkabBTdJ_lHvzaP_cujL3xBk1em4jeXXLzwaDBLfqMXIxKuw18VO1ZNSRz_NMPq-eb66eru_phdnt_dflQd4zzXDMs5vZCY97irvyTQtcKbgW2DBjmmrcXLcwxbpgAxqkAblvRKK60bYimak4Pq9Ot7xjD22RSlsswRV9WSkIF5SAI4YUiW6qLIaVorByje1VxJTHIdRRyG4UsUchNFBKKiG5FqcB-YeKf9T-qb92qjjk</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2393609226</pqid></control><display><type>article</type><title>One-pot synthesis of Mn3O4-coupled Ag2WO4 nanocomposite photocatalyst for enhanced photooxidative desulfurization of thiophene under visible light irradiation</title><source>Springer Nature - Complete Springer Journals</source><creator>Shawky, Ahmed ; Mohamed, R. M. ; Mkhalid, I. A. ; Awwad, Nasser S. ; Ibrahium, Hala A.</creator><creatorcontrib>Shawky, Ahmed ; Mohamed, R. M. ; Mkhalid, I. A. ; Awwad, Nasser S. ; Ibrahium, Hala A.</creatorcontrib><description>The photooxidative desulfurization of thiophene (ThP) becomes a challenge in both industry and environmental remediation. Herein, we synthesize a visible-light-responsive Ag
2
WO
4
/Mn
3
O
4
nanocomposite by a one-pot strategy. Depiction of the produced photocatalysts exposed the suppression of the surface structure and reduction of the bandgap energy by adding 15 wt% of Mn
3
O
4
to Ag
2
WO
4
. The obtained nanocomposite shows a complete photooxidation of ThP within 1 h under visible light illumination at a dose of 1.2 g L
−1
. The significance of photocatalytic performance of Ag
2
WO
4
/Mn
3
O
4
nanocomposite photocatalyst is referred to the enhancement of the visible light absorption and overthrow of the recombination of photogenerated charge carriers. The study opens the door for extensive use of nanocomposite photocatalysts as a novel functional material for the photooxidation of ThPs under visible light exposure.</description><identifier>ISSN: 2190-5509</identifier><identifier>EISSN: 2190-5517</identifier><identifier>DOI: 10.1007/s13204-019-01212-0</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Chemistry and Materials Science ; Current carriers ; Desulfurizing ; Electromagnetic absorption ; Functional materials ; Light ; Light irradiation ; Manganese oxides ; Materials Science ; Membrane Biology ; Nanochemistry ; Nanocomposites ; Nanotechnology ; Nanotechnology and Microengineering ; Original Article ; Oxidation ; Photocatalysis ; Photocatalysts ; Photooxidation ; Surface structure</subject><ispartof>Applied nanoscience, 2020-05, Vol.10 (5), p.1545-1554</ispartof><rights>King Abdulaziz City for Science and Technology 2019</rights><rights>King Abdulaziz City for Science and Technology 2019.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c466t-419bf8d1671c55030c796f91f40416d67870b115490463906f795a6adf52d3ab3</citedby><cites>FETCH-LOGICAL-c466t-419bf8d1671c55030c796f91f40416d67870b115490463906f795a6adf52d3ab3</cites><orcidid>0000-0001-7590-8548</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s13204-019-01212-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s13204-019-01212-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Shawky, Ahmed</creatorcontrib><creatorcontrib>Mohamed, R. M.</creatorcontrib><creatorcontrib>Mkhalid, I. A.</creatorcontrib><creatorcontrib>Awwad, Nasser S.</creatorcontrib><creatorcontrib>Ibrahium, Hala A.</creatorcontrib><title>One-pot synthesis of Mn3O4-coupled Ag2WO4 nanocomposite photocatalyst for enhanced photooxidative desulfurization of thiophene under visible light irradiation</title><title>Applied nanoscience</title><addtitle>Appl Nanosci</addtitle><description>The photooxidative desulfurization of thiophene (ThP) becomes a challenge in both industry and environmental remediation. Herein, we synthesize a visible-light-responsive Ag
2
WO
4
/Mn
3
O
4
nanocomposite by a one-pot strategy. Depiction of the produced photocatalysts exposed the suppression of the surface structure and reduction of the bandgap energy by adding 15 wt% of Mn
3
O
4
to Ag
2
WO
4
. The obtained nanocomposite shows a complete photooxidation of ThP within 1 h under visible light illumination at a dose of 1.2 g L
−1
. The significance of photocatalytic performance of Ag
2
WO
4
/Mn
3
O
4
nanocomposite photocatalyst is referred to the enhancement of the visible light absorption and overthrow of the recombination of photogenerated charge carriers. The study opens the door for extensive use of nanocomposite photocatalysts as a novel functional material for the photooxidation of ThPs under visible light exposure.</description><subject>Chemistry and Materials Science</subject><subject>Current carriers</subject><subject>Desulfurizing</subject><subject>Electromagnetic absorption</subject><subject>Functional materials</subject><subject>Light</subject><subject>Light irradiation</subject><subject>Manganese oxides</subject><subject>Materials Science</subject><subject>Membrane Biology</subject><subject>Nanochemistry</subject><subject>Nanocomposites</subject><subject>Nanotechnology</subject><subject>Nanotechnology and Microengineering</subject><subject>Original Article</subject><subject>Oxidation</subject><subject>Photocatalysis</subject><subject>Photocatalysts</subject><subject>Photooxidation</subject><subject>Surface structure</subject><issn>2190-5509</issn><issn>2190-5517</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp9kc1KxDAUhYsoKOoLuAq4rt78NDVLEf9AmY3iMmSaZJqhJjVJxfFhfFYzM6I7L4R7Q75zLuFU1QmGMwzQnidMCbAasCiHYFLDTnVAsIC6aXC7-zuD2K-OU1pCqYa1nDYH1dfMm3oMGaWVz71JLqFg0aOnM1Z3YRoHo9HlgrzMGPLKhy68jiG5bNDYhxw6ldWwShnZEJHxvfJd4TdP4cNpld27QdqkabBTdJ_lHvzaP_cujL3xBk1em4jeXXLzwaDBLfqMXIxKuw18VO1ZNSRz_NMPq-eb66eru_phdnt_dflQd4zzXDMs5vZCY97irvyTQtcKbgW2DBjmmrcXLcwxbpgAxqkAblvRKK60bYimak4Pq9Ot7xjD22RSlsswRV9WSkIF5SAI4YUiW6qLIaVorByje1VxJTHIdRRyG4UsUchNFBKKiG5FqcB-YeKf9T-qb92qjjk</recordid><startdate>20200501</startdate><enddate>20200501</enddate><creator>Shawky, Ahmed</creator><creator>Mohamed, R. M.</creator><creator>Mkhalid, I. A.</creator><creator>Awwad, Nasser S.</creator><creator>Ibrahium, Hala A.</creator><general>Springer International Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-7590-8548</orcidid></search><sort><creationdate>20200501</creationdate><title>One-pot synthesis of Mn3O4-coupled Ag2WO4 nanocomposite photocatalyst for enhanced photooxidative desulfurization of thiophene under visible light irradiation</title><author>Shawky, Ahmed ; Mohamed, R. M. ; Mkhalid, I. A. ; Awwad, Nasser S. ; Ibrahium, Hala A.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c466t-419bf8d1671c55030c796f91f40416d67870b115490463906f795a6adf52d3ab3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Chemistry and Materials Science</topic><topic>Current carriers</topic><topic>Desulfurizing</topic><topic>Electromagnetic absorption</topic><topic>Functional materials</topic><topic>Light</topic><topic>Light irradiation</topic><topic>Manganese oxides</topic><topic>Materials Science</topic><topic>Membrane Biology</topic><topic>Nanochemistry</topic><topic>Nanocomposites</topic><topic>Nanotechnology</topic><topic>Nanotechnology and Microengineering</topic><topic>Original Article</topic><topic>Oxidation</topic><topic>Photocatalysis</topic><topic>Photocatalysts</topic><topic>Photooxidation</topic><topic>Surface structure</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shawky, Ahmed</creatorcontrib><creatorcontrib>Mohamed, R. M.</creatorcontrib><creatorcontrib>Mkhalid, I. A.</creatorcontrib><creatorcontrib>Awwad, Nasser S.</creatorcontrib><creatorcontrib>Ibrahium, Hala A.</creatorcontrib><collection>CrossRef</collection><jtitle>Applied nanoscience</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Shawky, Ahmed</au><au>Mohamed, R. M.</au><au>Mkhalid, I. A.</au><au>Awwad, Nasser S.</au><au>Ibrahium, Hala A.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>One-pot synthesis of Mn3O4-coupled Ag2WO4 nanocomposite photocatalyst for enhanced photooxidative desulfurization of thiophene under visible light irradiation</atitle><jtitle>Applied nanoscience</jtitle><stitle>Appl Nanosci</stitle><date>2020-05-01</date><risdate>2020</risdate><volume>10</volume><issue>5</issue><spage>1545</spage><epage>1554</epage><pages>1545-1554</pages><issn>2190-5509</issn><eissn>2190-5517</eissn><abstract>The photooxidative desulfurization of thiophene (ThP) becomes a challenge in both industry and environmental remediation. Herein, we synthesize a visible-light-responsive Ag
2
WO
4
/Mn
3
O
4
nanocomposite by a one-pot strategy. Depiction of the produced photocatalysts exposed the suppression of the surface structure and reduction of the bandgap energy by adding 15 wt% of Mn
3
O
4
to Ag
2
WO
4
. The obtained nanocomposite shows a complete photooxidation of ThP within 1 h under visible light illumination at a dose of 1.2 g L
−1
. The significance of photocatalytic performance of Ag
2
WO
4
/Mn
3
O
4
nanocomposite photocatalyst is referred to the enhancement of the visible light absorption and overthrow of the recombination of photogenerated charge carriers. The study opens the door for extensive use of nanocomposite photocatalysts as a novel functional material for the photooxidation of ThPs under visible light exposure.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s13204-019-01212-0</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0001-7590-8548</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 2190-5509 |
| ispartof | Applied nanoscience, 2020-05, Vol.10 (5), p.1545-1554 |
| issn | 2190-5509 2190-5517 |
| language | eng |
| recordid | cdi_proquest_journals_2393609226 |
| source | Springer Nature - Complete Springer Journals |
| subjects | Chemistry and Materials Science Current carriers Desulfurizing Electromagnetic absorption Functional materials Light Light irradiation Manganese oxides Materials Science Membrane Biology Nanochemistry Nanocomposites Nanotechnology Nanotechnology and Microengineering Original Article Oxidation Photocatalysis Photocatalysts Photooxidation Surface structure |
| title | One-pot synthesis of Mn3O4-coupled Ag2WO4 nanocomposite photocatalyst for enhanced photooxidative desulfurization of thiophene under visible light irradiation |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-31T02%3A41%3A56IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=One-pot%20synthesis%20of%20Mn3O4-coupled%20Ag2WO4%20nanocomposite%20photocatalyst%20for%20enhanced%20photooxidative%20desulfurization%20of%20thiophene%20under%20visible%20light%20irradiation&rft.jtitle=Applied%20nanoscience&rft.au=Shawky,%20Ahmed&rft.date=2020-05-01&rft.volume=10&rft.issue=5&rft.spage=1545&rft.epage=1554&rft.pages=1545-1554&rft.issn=2190-5509&rft.eissn=2190-5517&rft_id=info:doi/10.1007/s13204-019-01212-0&rft_dat=%3Cproquest_cross%3E2393609226%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2393609226&rft_id=info:pmid/&rfr_iscdi=true |