Highly Elastic and >200% Reversibly Stretchable Down‐Conversion White Light‐Emitting Diodes Based on Quantum Dot Gel Emitters

Combining the characteristics of different materials offers exciting new opportunities for advanced applications in various fields. Herein, white light‐emitting diodes (WLEDs) with >200% reversible stretchability are fabricated using six‐color quantum dots (QDs) gel emitters. Stable aqueous‐phase...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Advanced optical materials 2020-04, Vol.8 (7), p.n/a
Hauptverfasser: Le, Thanh‐Hai, Choi, Yunseok, Kim, Semin, Lee, Unhan, Heo, Eunseo, Lee, Haney, Chae, Subin, Im, Won Bin, Yoon, Hyeonseok
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page n/a
container_issue 7
container_start_page
container_title Advanced optical materials
container_volume 8
creator Le, Thanh‐Hai
Choi, Yunseok
Kim, Semin
Lee, Unhan
Heo, Eunseo
Lee, Haney
Chae, Subin
Im, Won Bin
Yoon, Hyeonseok
description Combining the characteristics of different materials offers exciting new opportunities for advanced applications in various fields. Herein, white light‐emitting diodes (WLEDs) with >200% reversible stretchability are fabricated using six‐color quantum dots (QDs) gel emitters. Stable aqueous‐phase alloy core/shell QDs with high quantum yield are obtained via ligand exchange using a ternary solvent system. Transparent and highly stretchable gels with large pores are created by binary‐solvent‐based gelation at low temperatures. Importantly, the QDs and the gel originate from the same two solvents, which make the QDs highly compatible with the gelation process. Consequently, QDs of six different colors are incorporated into the gel without any property degradation. The excellent optical properties of the QDs in the liquid phase (e.g., 17% higher photoluminescence (PL) intensity) are retained in the gel phase. The QD gel (QDG) exhibits elastic deformation up to 200%, with uniform PL over the entire gel. A down‐conversion WLED built using the QDG emitter produces cool white light with a color temperature of 6100 K, a color rendering index of 94, and a luminous efficacy of 72 lm W−1. In addition, the performance of the QDG‐based WLED remains unchanged even after more than 1000 bending/stretching cycles. New down‐conversion white light‐emitting diodes with stretchable form factor are fabricated based on quantum dot gel emitters.
doi_str_mv 10.1002/adom.201901972
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2386112874</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2386112874</sourcerecordid><originalsourceid>FETCH-LOGICAL-c3172-ad0db54b6022708ace36c38019c23d74c89d07d3d7485af41b1625cc0b4bbd2e3</originalsourceid><addsrcrecordid>eNqFkEtLAzEUhYMoWGq3rgPicupN5r0RaltboVJ84XLIJGmbMo-aZCzd6T_wN_pLTFtRd0IgN5zvnEsOQqcEugSAXjBRl10KJHUnpgeoRUkaegRicvhnPkYdY5YA4B5-GsQt9D5W80WxwcOCGas4ZpXAlxTgHN_LV6mNyp34YLW0fMHyQuJBva4-3z76dbWT6wo_L5SVeOJyrBOGpbJWVXM8ULWQBl8xIwV22F3DKtuULsDikSzwDnQRJ-hoxgojO993Gz1dDx_7Y28yHd30exOP-ySmHhMg8jDII6A0hoRx6UfcT9x3OfVFHPAkFRCL7ZiEbBaQnEQ05BzyIM8FlX4bne1zV7p-aaSx2bJudOVWZtRPIkJoEgeO6u4prmtjtJxlK61KpjcZgWzbdLZtOvtp2hnSvWGtCrn5h856g-ntr_cLV8mEBA</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2386112874</pqid></control><display><type>article</type><title>Highly Elastic and &gt;200% Reversibly Stretchable Down‐Conversion White Light‐Emitting Diodes Based on Quantum Dot Gel Emitters</title><source>Wiley Online Library Journals Frontfile Complete</source><creator>Le, Thanh‐Hai ; Choi, Yunseok ; Kim, Semin ; Lee, Unhan ; Heo, Eunseo ; Lee, Haney ; Chae, Subin ; Im, Won Bin ; Yoon, Hyeonseok</creator><creatorcontrib>Le, Thanh‐Hai ; Choi, Yunseok ; Kim, Semin ; Lee, Unhan ; Heo, Eunseo ; Lee, Haney ; Chae, Subin ; Im, Won Bin ; Yoon, Hyeonseok</creatorcontrib><description>Combining the characteristics of different materials offers exciting new opportunities for advanced applications in various fields. Herein, white light‐emitting diodes (WLEDs) with &gt;200% reversible stretchability are fabricated using six‐color quantum dots (QDs) gel emitters. Stable aqueous‐phase alloy core/shell QDs with high quantum yield are obtained via ligand exchange using a ternary solvent system. Transparent and highly stretchable gels with large pores are created by binary‐solvent‐based gelation at low temperatures. Importantly, the QDs and the gel originate from the same two solvents, which make the QDs highly compatible with the gelation process. Consequently, QDs of six different colors are incorporated into the gel without any property degradation. The excellent optical properties of the QDs in the liquid phase (e.g., 17% higher photoluminescence (PL) intensity) are retained in the gel phase. The QD gel (QDG) exhibits elastic deformation up to 200%, with uniform PL over the entire gel. A down‐conversion WLED built using the QDG emitter produces cool white light with a color temperature of 6100 K, a color rendering index of 94, and a luminous efficacy of 72 lm W−1. In addition, the performance of the QDG‐based WLED remains unchanged even after more than 1000 bending/stretching cycles. New down‐conversion white light‐emitting diodes with stretchable form factor are fabricated based on quantum dot gel emitters.</description><identifier>ISSN: 2195-1071</identifier><identifier>EISSN: 2195-1071</identifier><identifier>DOI: 10.1002/adom.201901972</identifier><language>eng</language><publisher>Weinheim: Wiley Subscription Services, Inc</publisher><subject>Color temperature ; Conversion ; Elastic deformation ; Emitters ; form factors ; Gelation ; Gels ; Liquid phases ; Low temperature ; Luminous efficacy ; Materials science ; mechanical reliability ; Optical properties ; Optics ; Photoluminescence ; Quantum dots ; Solvents ; Stretchability ; White light ; white light emitting diodes</subject><ispartof>Advanced optical materials, 2020-04, Vol.8 (7), p.n/a</ispartof><rights>2020 WILEY‐VCH Verlag GmbH &amp; Co. KGaA, Weinheim</rights><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c3172-ad0db54b6022708ace36c38019c23d74c89d07d3d7485af41b1625cc0b4bbd2e3</citedby><cites>FETCH-LOGICAL-c3172-ad0db54b6022708ace36c38019c23d74c89d07d3d7485af41b1625cc0b4bbd2e3</cites><orcidid>0000-0002-5403-1617</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fadom.201901972$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fadom.201901972$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27901,27902,45550,45551</link.rule.ids></links><search><creatorcontrib>Le, Thanh‐Hai</creatorcontrib><creatorcontrib>Choi, Yunseok</creatorcontrib><creatorcontrib>Kim, Semin</creatorcontrib><creatorcontrib>Lee, Unhan</creatorcontrib><creatorcontrib>Heo, Eunseo</creatorcontrib><creatorcontrib>Lee, Haney</creatorcontrib><creatorcontrib>Chae, Subin</creatorcontrib><creatorcontrib>Im, Won Bin</creatorcontrib><creatorcontrib>Yoon, Hyeonseok</creatorcontrib><title>Highly Elastic and &gt;200% Reversibly Stretchable Down‐Conversion White Light‐Emitting Diodes Based on Quantum Dot Gel Emitters</title><title>Advanced optical materials</title><description>Combining the characteristics of different materials offers exciting new opportunities for advanced applications in various fields. Herein, white light‐emitting diodes (WLEDs) with &gt;200% reversible stretchability are fabricated using six‐color quantum dots (QDs) gel emitters. Stable aqueous‐phase alloy core/shell QDs with high quantum yield are obtained via ligand exchange using a ternary solvent system. Transparent and highly stretchable gels with large pores are created by binary‐solvent‐based gelation at low temperatures. Importantly, the QDs and the gel originate from the same two solvents, which make the QDs highly compatible with the gelation process. Consequently, QDs of six different colors are incorporated into the gel without any property degradation. The excellent optical properties of the QDs in the liquid phase (e.g., 17% higher photoluminescence (PL) intensity) are retained in the gel phase. The QD gel (QDG) exhibits elastic deformation up to 200%, with uniform PL over the entire gel. A down‐conversion WLED built using the QDG emitter produces cool white light with a color temperature of 6100 K, a color rendering index of 94, and a luminous efficacy of 72 lm W−1. In addition, the performance of the QDG‐based WLED remains unchanged even after more than 1000 bending/stretching cycles. New down‐conversion white light‐emitting diodes with stretchable form factor are fabricated based on quantum dot gel emitters.</description><subject>Color temperature</subject><subject>Conversion</subject><subject>Elastic deformation</subject><subject>Emitters</subject><subject>form factors</subject><subject>Gelation</subject><subject>Gels</subject><subject>Liquid phases</subject><subject>Low temperature</subject><subject>Luminous efficacy</subject><subject>Materials science</subject><subject>mechanical reliability</subject><subject>Optical properties</subject><subject>Optics</subject><subject>Photoluminescence</subject><subject>Quantum dots</subject><subject>Solvents</subject><subject>Stretchability</subject><subject>White light</subject><subject>white light emitting diodes</subject><issn>2195-1071</issn><issn>2195-1071</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNqFkEtLAzEUhYMoWGq3rgPicupN5r0RaltboVJ84XLIJGmbMo-aZCzd6T_wN_pLTFtRd0IgN5zvnEsOQqcEugSAXjBRl10KJHUnpgeoRUkaegRicvhnPkYdY5YA4B5-GsQt9D5W80WxwcOCGas4ZpXAlxTgHN_LV6mNyp34YLW0fMHyQuJBva4-3z76dbWT6wo_L5SVeOJyrBOGpbJWVXM8ULWQBl8xIwV22F3DKtuULsDikSzwDnQRJ-hoxgojO993Gz1dDx_7Y28yHd30exOP-ySmHhMg8jDII6A0hoRx6UfcT9x3OfVFHPAkFRCL7ZiEbBaQnEQ05BzyIM8FlX4bne1zV7p-aaSx2bJudOVWZtRPIkJoEgeO6u4prmtjtJxlK61KpjcZgWzbdLZtOvtp2hnSvWGtCrn5h856g-ntr_cLV8mEBA</recordid><startdate>20200401</startdate><enddate>20200401</enddate><creator>Le, Thanh‐Hai</creator><creator>Choi, Yunseok</creator><creator>Kim, Semin</creator><creator>Lee, Unhan</creator><creator>Heo, Eunseo</creator><creator>Lee, Haney</creator><creator>Chae, Subin</creator><creator>Im, Won Bin</creator><creator>Yoon, Hyeonseok</creator><general>Wiley Subscription Services, Inc</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-5403-1617</orcidid></search><sort><creationdate>20200401</creationdate><title>Highly Elastic and &gt;200% Reversibly Stretchable Down‐Conversion White Light‐Emitting Diodes Based on Quantum Dot Gel Emitters</title><author>Le, Thanh‐Hai ; Choi, Yunseok ; Kim, Semin ; Lee, Unhan ; Heo, Eunseo ; Lee, Haney ; Chae, Subin ; Im, Won Bin ; Yoon, Hyeonseok</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c3172-ad0db54b6022708ace36c38019c23d74c89d07d3d7485af41b1625cc0b4bbd2e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Color temperature</topic><topic>Conversion</topic><topic>Elastic deformation</topic><topic>Emitters</topic><topic>form factors</topic><topic>Gelation</topic><topic>Gels</topic><topic>Liquid phases</topic><topic>Low temperature</topic><topic>Luminous efficacy</topic><topic>Materials science</topic><topic>mechanical reliability</topic><topic>Optical properties</topic><topic>Optics</topic><topic>Photoluminescence</topic><topic>Quantum dots</topic><topic>Solvents</topic><topic>Stretchability</topic><topic>White light</topic><topic>white light emitting diodes</topic><toplevel>online_resources</toplevel><creatorcontrib>Le, Thanh‐Hai</creatorcontrib><creatorcontrib>Choi, Yunseok</creatorcontrib><creatorcontrib>Kim, Semin</creatorcontrib><creatorcontrib>Lee, Unhan</creatorcontrib><creatorcontrib>Heo, Eunseo</creatorcontrib><creatorcontrib>Lee, Haney</creatorcontrib><creatorcontrib>Chae, Subin</creatorcontrib><creatorcontrib>Im, Won Bin</creatorcontrib><creatorcontrib>Yoon, Hyeonseok</creatorcontrib><collection>CrossRef</collection><collection>Electronics &amp; Communications Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Advanced optical materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Le, Thanh‐Hai</au><au>Choi, Yunseok</au><au>Kim, Semin</au><au>Lee, Unhan</au><au>Heo, Eunseo</au><au>Lee, Haney</au><au>Chae, Subin</au><au>Im, Won Bin</au><au>Yoon, Hyeonseok</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Highly Elastic and &gt;200% Reversibly Stretchable Down‐Conversion White Light‐Emitting Diodes Based on Quantum Dot Gel Emitters</atitle><jtitle>Advanced optical materials</jtitle><date>2020-04-01</date><risdate>2020</risdate><volume>8</volume><issue>7</issue><epage>n/a</epage><issn>2195-1071</issn><eissn>2195-1071</eissn><abstract>Combining the characteristics of different materials offers exciting new opportunities for advanced applications in various fields. Herein, white light‐emitting diodes (WLEDs) with &gt;200% reversible stretchability are fabricated using six‐color quantum dots (QDs) gel emitters. Stable aqueous‐phase alloy core/shell QDs with high quantum yield are obtained via ligand exchange using a ternary solvent system. Transparent and highly stretchable gels with large pores are created by binary‐solvent‐based gelation at low temperatures. Importantly, the QDs and the gel originate from the same two solvents, which make the QDs highly compatible with the gelation process. Consequently, QDs of six different colors are incorporated into the gel without any property degradation. The excellent optical properties of the QDs in the liquid phase (e.g., 17% higher photoluminescence (PL) intensity) are retained in the gel phase. The QD gel (QDG) exhibits elastic deformation up to 200%, with uniform PL over the entire gel. A down‐conversion WLED built using the QDG emitter produces cool white light with a color temperature of 6100 K, a color rendering index of 94, and a luminous efficacy of 72 lm W−1. In addition, the performance of the QDG‐based WLED remains unchanged even after more than 1000 bending/stretching cycles. New down‐conversion white light‐emitting diodes with stretchable form factor are fabricated based on quantum dot gel emitters.</abstract><cop>Weinheim</cop><pub>Wiley Subscription Services, Inc</pub><doi>10.1002/adom.201901972</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-5403-1617</orcidid></addata></record>
fulltext fulltext
identifier ISSN: 2195-1071
ispartof Advanced optical materials, 2020-04, Vol.8 (7), p.n/a
issn 2195-1071
2195-1071
language eng
recordid cdi_proquest_journals_2386112874
source Wiley Online Library Journals Frontfile Complete
subjects Color temperature
Conversion
Elastic deformation
Emitters
form factors
Gelation
Gels
Liquid phases
Low temperature
Luminous efficacy
Materials science
mechanical reliability
Optical properties
Optics
Photoluminescence
Quantum dots
Solvents
Stretchability
White light
white light emitting diodes
title Highly Elastic and >200% Reversibly Stretchable Down‐Conversion White Light‐Emitting Diodes Based on Quantum Dot Gel Emitters
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-11T14%3A05%3A07IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Highly%20Elastic%20and%20%3E200%25%20Reversibly%20Stretchable%20Down%E2%80%90Conversion%20White%20Light%E2%80%90Emitting%20Diodes%20Based%20on%20Quantum%20Dot%20Gel%20Emitters&rft.jtitle=Advanced%20optical%20materials&rft.au=Le,%20Thanh%E2%80%90Hai&rft.date=2020-04-01&rft.volume=8&rft.issue=7&rft.epage=n/a&rft.issn=2195-1071&rft.eissn=2195-1071&rft_id=info:doi/10.1002/adom.201901972&rft_dat=%3Cproquest_cross%3E2386112874%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2386112874&rft_id=info:pmid/&rfr_iscdi=true